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Synthesis of MS2 (M = Mo, W) thin films by chemical solution deposition

文献类型：期刊论文

作者Huan, Jie1,4; Zhu, Lili1; Li, Changdian1,4; Chen, Qian1,4; Zheng, Ruobing1,4; He, Yuandi1,4; Gong, Chengzhuan1,4; Wei, Renhuai1; Zhu, Xuebin1; Sun, Yuping1,2,3
刊名INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
出版日期2024-08-19
卷号79
关键词Mo1-xWxS2 Thin film Chemical solution deposition Hydrogen evolution reaction
ISSN号0360-3199
DOI10.1016/j.ijhydene.2024.07.113
通讯作者Zhu, Lili(llzhu@issp.ac.cn) ; Zhu, Xuebin(xbzhu@issp.ac.cn)
英文摘要MoS2 and WS2 as typical two-dimensional transition metal dichalcogenides have been investigated since of rich physicochemical properties. To deposit MoS2 and WS2 thin films, chemical solution deposition as a facile route had been used showing the advantages of high component controllability, low cost, sequential processing of device, easy preparation of large-size films and facile preparation of films on irregular substrates. Here, Mo1-xWxS2 (0 <= x <= 1) thin films were successfully prepared by chemical solution deposition method. The phases as well as microstructures were investigated using field emission scanning electron microscope, atomic force microscopy, transmission electron microscopy, Raman and x-ray photoelectron spectroscopy measurements. The prepared Mo1-xWxS2 thin films are used as hydrogen evolution reaction (HER) catalyst electrodes for water splitting. The Mo03W07S2 thin film catalyst shows an overpotential of 345 mV at a current density of 10 mA cm(-2) and the corresponding Tafel slope of 169 mV dec(-1) in 0.5 M sulfuric acid. The results will provide a facile method to deposit MX2 thin films.
WOS关键词HYDROGEN EVOLUTION REACTION ; MONOLAYER MOS2 ; WAFER-SCALE ; NANOSHEETS ; GROWTH ; LAYERS ; EXFOLIATION ; CATALYSTS ; DIODES
资助项目National Natural Science Foundation of China, China[52272251]
WOS研究方向Chemistry ; Electrochemistry ; Energy & Fuels
语种英语
WOS记录号WOS:001268940400001
出版者PERGAMON-ELSEVIER SCIENCE LTD
资助机构National Natural Science Foundation of China, China
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/137181]  
专题中国科学院合肥物质科学研究院
通讯作者Zhu, Lili; Zhu, Xuebin
作者单位1.Chinese Acad Sci, Key Lab Mat Phys, Inst Solid State Phys, HFIPS, Hefei 230031, Peoples R China
2.Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Peoples R China
3.Chinese Acad Sci, High Magnet Field Lab, HFIPS, Hefei 230031, Peoples R China
4.Univ Sci & Technol China, Hefei 230026, Peoples R China
推荐引用方式
GB/T 7714		 Huan, Jie,Zhu, Lili,Li, Changdian,et al. Synthesis of MS2 (M = Mo, W) thin films by chemical solution deposition[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2024,79.
APA Huan, Jie.,Zhu, Lili.,Li, Changdian.,Chen, Qian.,Zheng, Ruobing.,...&Sun, Yuping.(2024).Synthesis of MS2 (M = Mo, W) thin films by chemical solution deposition.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,79.
MLA Huan, Jie,et al."Synthesis of MS2 (M = Mo, W) thin films by chemical solution deposition".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 79(2024).

入库方式： OAI收割

来源：合肥物质科学研究院

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