Efficient degradation of bisphenol A and amino black 10B by magnetic composite Fe3O4@MOF-74 as catalyst
文献类型：期刊论文
| 作者 | Hu, Xiaohan2; Tian, Ye2; Liu, Junshen2; Xu, Wenlong2; Niu, Yuzhong2; Zhang, Beibei2; Sun, Changmei2; Sun, Xiyan1 |
| 刊名 | ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY
 |
| 出版日期 | 2024-10-01 |
| 卷号 | 284页码:12 |
| 关键词 | MOFs Catalyst Catalyst Degradation Amino black 10B Bisphenol A |
| ISSN号 | 0147-6513 |
| DOI | 10.1016/j.ecoenv.2024.116926 |
| 通讯作者 | Zhang, Beibei(zhbb0302@163.com) ; Sun, Changmei(sunchangmei0535@126.com) ; Sun, Xiyan(xysun@yic.ac.cn) |
| 英文摘要 | Metal-organic frameworks (MOFs) exhibit high chemical stability and porosity, and have been widely applied in various fields including selective adsorption and separation, sensors, and catalysis. When combined with Fe3O4, they effectively address issues such as aggregation of Fe3O4 particles and the difficulty in recovering MOFs as catalysts. Therefore, in this study, we used a simple solvothermal method as a catalyst to synthesize a high specific surface area magnetic composite Fe3O4@MOF-74, which was used to catalyze the degradation of bisphenol A (BPA) and amino black 10B in wastewater. We activated Na2S2O8 to generate radicals for oxidizing and degrading BPA and amino black 10B. Experimental results showed that at 35 degrees C, with Fe3O4@MOF-74 (Fe3O4: MOF-74=1:1) concentration of 0.2 g/L and Na2S2O8 concentration of 2 g/L, the catalytic effect is efficient and economical. Meanwhile, removal rates of BPA and amino black 10B exceeded 95.58 % over a broad pH range (pH 3-9). Furthermore, even after multiple cycles of use, Fe3O4@MOF-74 maintained catalytic degradation rates of BPA and amino black 10B above 93.24 % and 95.01 %, respectively. Additionally, in water samples, removal rates of BPA and amino black 10B exceeded 91.55 %. This study provides a new and efficient catalyst material for wastewater treatment, which is expected to play an important role in environmental remediation. |
| WOS关键词 | ACTIVATED PERSULFATE OXIDATION ; WATER ; PEROXYMONOSULFATE ; KINETICS ; REMOVAL ; OXIDE ; NANOCOMPOSITE ; NANOPARTICLES ; ADSORPTION ; BEHAVIOR |
| WOS研究方向 | Environmental Sciences & Ecology ; Toxicology |
| 语种 | 英语 |
| WOS记录号 | WOS:001358544900001 |
| 资助机构 | Natural Science Foundation of Shandong Province ; National Natural Science Foundation of China ; Youth Innovation Technology Support Program of Universities in Shandong Province ; Project of Yantai Science and Tech-nology Innovation Development Plan |
| 源URL | [http://ir.yic.ac.cn/handle/133337/38204]  |
| 专题 | 中国科学院牟平海岸带环境综合试验站 |
| 通讯作者 | Zhang, Beibei; Sun, Changmei; Sun, Xiyan |
| 作者单位 | 1.Chinese Acad Sci, Muping Coastal Environm Res Stn, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China 2.Ludong Univ, Sch Chem & Mat Sci, Yantai 264025, Peoples R China |
| 推荐引用方式 GB/T 7714 | Hu, Xiaohan,Tian, Ye,Liu, Junshen,et al. Efficient degradation of bisphenol A and amino black 10B by magnetic composite Fe3O4@MOF-74 as catalyst[J]. ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY,2024,284:12. |
| APA | Hu, Xiaohan.,Tian, Ye.,Liu, Junshen.,Xu, Wenlong.,Niu, Yuzhong.,...&Sun, Xiyan.(2024).Efficient degradation of bisphenol A and amino black 10B by magnetic composite Fe3O4@MOF-74 as catalyst.ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY,284,12. |
| MLA | Hu, Xiaohan,et al."Efficient degradation of bisphenol A and amino black 10B by magnetic composite Fe3O4@MOF-74 as catalyst".ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY 284(2024):12. |
入库方式： OAI收割
来源：烟台海岸带研究所
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