New insights into thallium(I) behaviors at birnessite surfaces: Effects of an organic buffer and goethite
文献类型：期刊论文
| 作者 | Zhuang, Wen3,6; Zhu, Tianqiang2,3; Li, Feng2,3; Jing, Chuanyong3; Ying, Samantha C.1; Abernathy, Macon J.1,8; Song, Jinming7 ; Yin, Hui4,5
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| 刊名 | JOURNAL OF HAZARDOUS MATERIALS
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| 出版日期 | 2024-12-05 |
| 卷号 | 480页码:11 |
| 关键词 | Thallium Manganese (hydr)oxide Competitive adsorption Good's buffer |
| ISSN号 | 0304-3894 |
| DOI | 10.1016/j.jhazmat.2024.136340 |
| 通讯作者 | Zhuang, Wen(wzhuang@sdu.edu.cn) ; Yin, Hui(yinhui666@mail.hzau.edu.cn) |
| 英文摘要 | Understanding the environmental behavior of thallium (Tl) is crucial due to its high toxicity and increasing anthropogenic presence. This study investigated the adsorption and redox behaviors of Tl(I) with acid birnessite (AcBi) in the presence of 1,4-piperazine-diethanesulfonic acid (PIPES) and goethite under diffusion-limited conditions using Donnan reactors in aerobic and anaerobic environments. Our findings indicate that Tl(I) preferentially adsorbs onto AcBi, with capacities 20 to 100 times higher than onto goethite, even when AcBi is partial reduced by PIPES. No net Tl(I) oxidation occurred in the Donnan reactors, likely due to complex electron transfer processes between Tl(I), birnessite, and PIPES. Any Tl(III) generated from Tl(I) oxidation by birnessite was rapidly reduced back to Tl(I) by PIPES. This was confirmed in batch experiments where reduced Tl(III) on birnessite surfaces and in Tl(III) salts. These findings highlight the need to assess the impact of Good's buffers on redox reactions involving manganese oxides and Tl, while also providing insights into the competitive retention of Tl on manganese and iron (hydr)oxides, with implications for Tl mobility and bioavailability in natural environments. |
| WOS关键词 | HEXAGONAL BIRNESSITE ; ISOTOPE COMPOSITIONS ; MANGANESE OXIDES ; METAL-IONS ; OXIDATION ; SORPTION ; SEDIMENTS ; NANOPARTICLES ; ENRICHMENT ; SPECIATION |
| 资助项目 | Laoshan Laboratory Science and Technology Innovation Project[LSKJ202205003] ; Natural Science Foundations of China[42077015] |
| WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:001349179500001 |
| 出版者 | ELSEVIER |
| 源URL | [http://ir.qdio.ac.cn/handle/337002/199405]  |
| 专题 | 海洋研究所_海洋生态与环境科学重点实验室 |
| 通讯作者 | Zhuang, Wen; Yin, Hui |
| 作者单位 | 1.Univ Calif Riverside, Dept Environm Sci, Environm Toxicol Program, Riverside, CA 92521 USA 2.Shandong Univ, Inst Ecoenvironm Forens, Qingdao 266237, Shandong, Peoples R China 3.Shandong Univ, Sch Environm Sci & Engn, Qingdao 266237, Shandong, Peoples R China 4.Huazhong Agr Univ, Coll Resources & Environm, Key Lab Arable Land Conservat Middle & Lower Reach, Minist Agr & Rural Affairs, Wuhan 430070, Hubei, Peoples R China 5.Huazhong Agr Univ, State Environm Protect Key Lab Soil Hlth & Green, Wuhan 430070, Peoples R China 6.Shandong Univ, Inst Marine Sci & Technol, Qingdao 266237, Shandong, Peoples R China 7.Chinese Acad Sci, Key Lab Marine Ecol & Environm Sci, Inst Oceanol, Qingdao 266071, Shandong, Peoples R China 8.Stanford Univ, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA |
| 推荐引用方式 GB/T 7714 | Zhuang, Wen,Zhu, Tianqiang,Li, Feng,et al. New insights into thallium(I) behaviors at birnessite surfaces: Effects of an organic buffer and goethite[J]. JOURNAL OF HAZARDOUS MATERIALS,2024,480:11. |
| APA | Zhuang, Wen.,Zhu, Tianqiang.,Li, Feng.,Jing, Chuanyong.,Ying, Samantha C..,...&Yin, Hui.(2024).New insights into thallium(I) behaviors at birnessite surfaces: Effects of an organic buffer and goethite.JOURNAL OF HAZARDOUS MATERIALS,480,11. |
| MLA | Zhuang, Wen,et al."New insights into thallium(I) behaviors at birnessite surfaces: Effects of an organic buffer and goethite".JOURNAL OF HAZARDOUS MATERIALS 480(2024):11. |
入库方式： OAI收割
来源：海洋研究所
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