中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Design of MOF-Based Solar Evaporators With Hierarchical Microporous/Nanobridged/Nanogranular Structures for Rapid Interfacial Solar Evaporation and Fresh Water Collection

文献类型:期刊论文

作者Li, Lingxiao1,2; Chen, Kai1; Zhang, Jiaren1; Zhang, Junping1,2
刊名ChemSusChem
出版日期2024
卷号17期号:24页码:e202401224
关键词Interfacial solar evaporation Silicone nanofilaments Superhydrophilic Metal-organic frameworks Solar desalination
DOI10.1002/cssc.202401224
英文摘要

Interfacial solar evaporation (ISE) holds considerable promise to solve fresh water shortage, but it is challenging to achieve high evaporation rate (Reva) and fresh water yield in close system. Here, we report design and preparation of MOF-based solar evaporators with hierarchical microporous/nanobridged/nanogranular structures for rapid ISE and fresh water collection in close system. The evaporators are fabricated by growing silicone nanofilaments with variable length as nanobridges on a microporous silicone sponge followed by grafting with polydopamine nanoparticles and Cu-MOF nanocrystals. Integration of the unique structure and excellent photothermal composites endows the evaporators with high Reva of 3.5–20 wt % brines (3.60–2.90 kg m−2 h−1 in open system and 2.38–1.44 kg m−2 h−1 in close system) under simulated 1 sun, high Reva under natural sunlight, excellent salt resistance and high fresh water yield, which surpass most state-of-the-art evaporators. Moreover, when combined with a superhydrophilic cover, the evaporators show much higher average Reva of real seawater, remarkable fresh water yield and excellent long-term stability over one month continuous ISE under natural sunlight. The findings here will promote the development of advanced evaporators via microstructure engineering and their real-world ISE applications.

语种英语
源URL[http://ir.licp.cn/handle/362003/31431]  
专题兰州化学物理研究所_环境材料与生态化学研究发展中心
兰州化学物理研究所_OSSO国家重点实验室
通讯作者Zhang, Junping
作者单位1.Research Center of Resource Chemistry and Energy Materials, and State KeyLaboratory for Oxo Synthesis and Selective Oxidation, Lanzhou Institute ofChemical Physics, Chinese Academy of Sciences, Lanzhou, P. R. China
2.Center of Materials Science and Optoelectronics Engineering, University ofChinese Academy of Sciences, Beijing, P. R. China
推荐引用方式
GB/T 7714
Li, Lingxiao,Chen, Kai,Zhang, Jiaren,et al. Design of MOF-Based Solar Evaporators With Hierarchical Microporous/Nanobridged/Nanogranular Structures for Rapid Interfacial Solar Evaporation and Fresh Water Collection[J]. ChemSusChem,2024,17(24):e202401224.
APA Li, Lingxiao,Chen, Kai,Zhang, Jiaren,&Zhang, Junping.(2024).Design of MOF-Based Solar Evaporators With Hierarchical Microporous/Nanobridged/Nanogranular Structures for Rapid Interfacial Solar Evaporation and Fresh Water Collection.ChemSusChem,17(24),e202401224.
MLA Li, Lingxiao,et al."Design of MOF-Based Solar Evaporators With Hierarchical Microporous/Nanobridged/Nanogranular Structures for Rapid Interfacial Solar Evaporation and Fresh Water Collection".ChemSusChem 17.24(2024):e202401224.

入库方式: OAI收割

来源:兰州化学物理研究所

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