中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
CO2 seepage & breakthrough process and multifactorial influence mechanisms on it in unsaturated low-permeability sandstones

文献类型:期刊论文

作者Li, Yi2,3; Wang, Yao3; Dan, Wendong3; Li, Qi2; Hu, Zhikai3; Zhao, Jiaqi3; He, Li3; Diao, Yujie1
刊名JOURNAL OF HYDROLOGY
出版日期2025-10-01
卷号659页码:18
关键词Initial pressure difference Confining pressure CO2 geo-sequestration CO2 breakthrough pressure CO2 phase
ISSN号0022-1694
DOI10.1016/j.jhydrol.2025.133331
英文摘要CO2 breakthrough pressure is a key indicator for studying CO2 percolation behavior and assessing the sealing capacity of caprocks, which is critical for ensuring the safety and effectiveness of CO2 geo-sequestration. However, existing research on how CO2 phase, initial pressure difference, and confining pressure influence CO2 breakthrough pressure is limited, with inconsistent and unreliable conclusions. To address this gap, this study investigated the mechanisms behind CO2 breakthrough pressure using natural low-permeability unsaturated sandstone as the experimental material. A total of 27 CO2 breakthrough pressure experiments were conducted under various CO2 phases, initial pressure difference, and confining pressures using a step-by-step methodology. The results showed that there was no fixed or predictable relationship between breakthrough pressure and CO2 phase. However, in the presence of a single CO2 phase, the breakthrough pressure declined exponentially as the pressure increases. The influence of pressure on breakthrough pressure was attributed to the combined effect of CO2-H2O interfacial tension (IFT), contact angle of CO2-H2O-rock system, and two-phase viscosity ratio. The study clarifies interactions influencing CO2 breakthrough pressure under varying conditions and elucidates the role of CO2 phase behavior. These findings provide experimental data to improve assessments of CO2 sequestration safety and caprock integrity, enabling more accurate evaluations of geological storage potential.
资助项目Open Research Fund of State Key Laboratory of Geomechanics and Geotechnical Engineering Safety, Institute of Rock and Soil Mechanics, Chinese Academy of Sciences[SKLGME021010] ; National Natural Science Foundation of China[41702251]
WOS研究方向Engineering ; Geology ; Water Resources
语种英语
WOS记录号WOS:001478425900001
出版者ELSEVIER
源URL[http://119.78.100.198/handle/2S6PX9GI/35867]  
专题中科院武汉岩土力学所
通讯作者Li, Yi; He, Li
作者单位1.China Geol Survey, Key Lab Carbon Dioxide Geol Storage, Ctr Hydrogeol & Environm Geol Survey, Baoding 071051, Hebei, Peoples R China
2.Chinese Acad Sci, Inst Rock & Soil Mech, State Key Lab Geomech & Geotech Engn Safety, Wuhan 430071, Peoples R China
3.Tianjin Univ, Sch Civil Engn, Key Lab Coast Civil Struct Safety, Minist Educ, Tianjin 300350, Peoples R China
推荐引用方式
GB/T 7714
Li, Yi,Wang, Yao,Dan, Wendong,et al. CO2 seepage & breakthrough process and multifactorial influence mechanisms on it in unsaturated low-permeability sandstones[J]. JOURNAL OF HYDROLOGY,2025,659:18.
APA Li, Yi.,Wang, Yao.,Dan, Wendong.,Li, Qi.,Hu, Zhikai.,...&Diao, Yujie.(2025).CO2 seepage & breakthrough process and multifactorial influence mechanisms on it in unsaturated low-permeability sandstones.JOURNAL OF HYDROLOGY,659,18.
MLA Li, Yi,et al."CO2 seepage & breakthrough process and multifactorial influence mechanisms on it in unsaturated low-permeability sandstones".JOURNAL OF HYDROLOGY 659(2025):18.

入库方式: OAI收割

来源:武汉岩土力学研究所

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