中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
High-efficient stabilization and solidification of municipal solid waste incineration fly ash by synergy of alkali treatment and supersulfated cement

文献类型:期刊论文

作者Cao, Wenxiang3; Lv, Xuesen3; Ban, Jiaxing3; Lu, Jian-Xin3; Liu, Ze2; Chen, Zhen1; Poon, Chi Sun3
刊名ENVIRONMENTAL POLLUTION
出版日期2024-08-15
卷号355页码:10
关键词Incineration fly ash Supersulfated cement Alkali treatment Heavy metals Stabilization and solidification
ISSN号0269-7491
DOI10.1016/j.envpol.2024.124261
英文摘要Municipal solid waste incineration fly ash (IFA) designated as hazardous waste poses risks to environment and human health. This study introduces a novel approach for the stabilization and solidification (S/S) of IFA: a combined approach involving alkali treatment and immobilization in low-carbon supersulfated cement (SSC). The impact of varying temperatures of alkali solution on the chemical and mineralogical compositions, as well as the pozzolanic reactivity of IFA, and the removal efficiency of heavy metals and metallic aluminum (Al) were examined. The physical characteristics, hydration kinetics and effectiveness of SSC in immobilizing IFA were also analyzed. Results showed that alkali treatment at 25 degrees C effectively eliminated heavy metals like manganese (Mn), barium (Ba), nickel (Ni), and chromium (Cr) to safe levels and totally removed the metallic Al, while enhancing the pozzolanic reactivity of IFA. By incorporating the alkali-treated IFA and filtrate, the density, compressive strength and hydration reaction of SSC were improved, resulting in higher hydration degree, finer pore structure, and denser microstructure compared to untreated IFA. The rich presence of calcium-aluminosilicate-hydrate (C(A)-S-H) and ettringite (AFt) in SSC facilitated the efficient stabilization and solidification of heavy metals, leading to a significant decrease in their leaching potential. The use of SSC for treating Ca(OH)2- and 25 degrees Ctreated IFA could achieve high strength and high-efficient immobilization.
资助项目General Research Fund of the Hong Kong Research Grants Council Research Centre for Resources Engineering towards Carbon Neutrality (BBEK)[B-Q80K] ; Start-up Fund under the Strategic Hiring Scheme[BDS6]
WOS研究方向Environmental Sciences & Ecology
语种英语
WOS记录号WOS:001247550700001
出版者ELSEVIER SCI LTD
源URL[http://119.78.100.198/handle/2S6PX9GI/41707]  
专题中科院武汉岩土力学所
通讯作者Lu, Jian-Xin
作者单位1.Chinese Acad Sci, Inst Rock & Soil Mech, State Key Lab Geomech & Geotech Engn, Wuhan 430071, Peoples R China
2.China Univ Min & Technol Beijing, Sch Chem & Environm Engn, Beijing 100083, Peoples R China
3.Hong Kong Polytech Univ, Dept Civil & Environm Engn, Hong Kong, Peoples R China
推荐引用方式
GB/T 7714
Cao, Wenxiang,Lv, Xuesen,Ban, Jiaxing,et al. High-efficient stabilization and solidification of municipal solid waste incineration fly ash by synergy of alkali treatment and supersulfated cement[J]. ENVIRONMENTAL POLLUTION,2024,355:10.
APA Cao, Wenxiang.,Lv, Xuesen.,Ban, Jiaxing.,Lu, Jian-Xin.,Liu, Ze.,...&Poon, Chi Sun.(2024).High-efficient stabilization and solidification of municipal solid waste incineration fly ash by synergy of alkali treatment and supersulfated cement.ENVIRONMENTAL POLLUTION,355,10.
MLA Cao, Wenxiang,et al."High-efficient stabilization and solidification of municipal solid waste incineration fly ash by synergy of alkali treatment and supersulfated cement".ENVIRONMENTAL POLLUTION 355(2024):10.

入库方式: OAI收割

来源:武汉岩土力学研究所

浏览0
下载0
收藏0
其他版本

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。