中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Reactive particle-laden flow in industrial-scale supercritical water gasification reactor: Modeling and study on flow patterns

文献类型:期刊论文

作者Wang, Yingdong1; Ou, Zhisong2; Jin, Hui1; Shang, Fei1; Guo, Shenghui1
刊名POWDER TECHNOLOGY
出版日期2024-07-01
卷号443页码:13
关键词Thermally integrated supercritical water gasification reactor Flow pattern Reactive particle-laden flow Porous media model
ISSN号0032-5910
DOI10.1016/j.powtec.2024.119946
英文摘要Coal gasification in supercritical water (SCW) is a highly complicated reactive particle-laden flow process, which couples multiphase flow hydrodynamics, conjugate heat transfers, and complex chemical reactions. A quantitative understanding is the key issue for reactor design and optimization. In this study, the Eulerian-Eulerian model is used to describe the particles-SCW flow in a novel industrial-scale thermally integrated supercritical water gasification (TISCWG) reactor with conjugate heat transfer boundary conditions and porous media model. The sophisticated chemical reactions are using a species transport model with a seven-step lumped kinetics. Four zones of the TISCWG reactor and four typical flow patterns in the gasification chamber are firstly revealed as 1) the bottom accumulation region with the nonhomogeneous solids distribution and back-mixing of particles, 2) the upper developed fluidization region with the SCW and coal particles moving in a plug-flow regime in the center and a downward annular gravity-driven flow near the wall, 3) the jet-affected region strongly affected by the vortexes near the nozzle and presented as a trans-critical jet regime and 4) the dilute region where dilute solids slow down and fall back into the gasification zone. Flow in the gasification chamber is strongly affected by the heat transfer with the preheat zone, as reflected by an annular gravity-driven flow film flowing downwards near the gasification wall. A funnel-shaped structure promotes a more uniform distribution of solids in the accumulation region rather than a cylindrical structure. The effect of flow patterns on coal gasification processes is also studied. Volatile pyrohydrolysis reactions depend on the time-varying solids distribution and the gaseous products at the system outlet with a typical H 2 mole fraction of 61.42% and CO 2 of 34.98%.
资助项目National Key Research and Development Program of China[2020YFA0714400] ; Shaanxi Science & Technology Co-ordination & Innovation Project[2024GX-YBXM- 518] ; National Natural Science Foundation of China[52300183] ; National Funding Program for Postdoctoral Researchers ; Special Research Assistant Program of the Chinese Academy of Science
WOS研究方向Engineering
语种英语
WOS记录号WOS:001251423000001
出版者ELSEVIER
源URL[http://119.78.100.198/handle/2S6PX9GI/41761]  
专题中科院武汉岩土力学所
通讯作者Jin, Hui
作者单位1.Xi An Jiao Tong Univ, State Key Lab Multiphase Flow Power Engn SKLMF, Xian 710049, Shaanxi, Peoples R China
2.Chinese Acad Sci, Inst Rock & Soil Mech, Xiaohongshan 2, Wuhan 430071, Peoples R China
推荐引用方式
GB/T 7714
Wang, Yingdong,Ou, Zhisong,Jin, Hui,et al. Reactive particle-laden flow in industrial-scale supercritical water gasification reactor: Modeling and study on flow patterns[J]. POWDER TECHNOLOGY,2024,443:13.
APA Wang, Yingdong,Ou, Zhisong,Jin, Hui,Shang, Fei,&Guo, Shenghui.(2024).Reactive particle-laden flow in industrial-scale supercritical water gasification reactor: Modeling and study on flow patterns.POWDER TECHNOLOGY,443,13.
MLA Wang, Yingdong,et al."Reactive particle-laden flow in industrial-scale supercritical water gasification reactor: Modeling and study on flow patterns".POWDER TECHNOLOGY 443(2024):13.

入库方式: OAI收割

来源:武汉岩土力学研究所

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