Two-dimensional Pt@g-C3N4/ReS2 Van Der Waals Heterostructure for photocatalytic hydrogen evolution with direct Z-scheme
文献类型：期刊论文
| 作者 | Wang, Hong-Yao4; Yang, Chuan-Lu4,5; Li, Xiaohu2,3,5 ; Liu, Yuliang4; Zhao, Wenkai4; Gao, Feng1
|
| 刊名 | CHEMICAL PHYSICS LETTERS
 |
| 出版日期 | 2025-07-01 |
| 卷号 | 870页码:142101 |
| 关键词 | Heterostructure Photocatalytic Direct Z -scheme Solar-to-hydrogen Gibbs free energy |
| ISSN号 | 0009-2614 |
| DOI | 10.1016/j.cplett.2025.142101 |
| 产权排序 | 3 |
| 英文摘要 | To overcome the limitations of the Pt@g-C3N4 monolayer in driving the oxygen evolution reaction (OER), we construct a photocatalytic Z-scheme with Pt@g-C3N4/ReS2 heterojunction. Band edge arrangement satisfies the requirements for hydrogen evolution reaction (HER) and OER, with a solar-to-hydrogen efficiency of 15.31 %. Nonadiabatic molecular dynamics simulation indicates that the reduction and oxidation activities of OER and HER can be efficiently protected. The Gibbs free energies indicate that the heterostructure can spontaneously drive HER, while OER requires a cocatalyst or sacrificial agent. These findings demonstrate the potential of Pt@g-C3N4/ReS2 heterojunctions as promising candidates for photocatalytic water splitting applications. |
| WOS关键词 | TOTAL-ENERGY CALCULATIONS ; VISIBLE-LIGHT ; CHARGE SEPARATION ; EFFICIENT ; HETEROJUNCTION ; DYNAMICS ; G-C3N4 |
| 资助项目 | National Natural Science Foundation of China[12374232] ; National Natural Science Foundation of China[12473025] |
| WOS研究方向 | Chemistry ; Physics |
| 语种 | 英语 |
| WOS记录号 | WOS:001476200700001 |
| 出版者 | ELSEVIER |
| 资助机构 | National Natural Science Foundation of China |
| 源URL | [http://ir.xao.ac.cn/handle/45760611-7/7721]  |
| 专题 | 天体化学研究团组 |
| 通讯作者 | Yang, Chuan-Lu |
| 作者单位 | 1.Southern Univ & A&M Coll, Dept Phys, Baton Rouge, LA 70813 USA 2.Xinjiang Key Lab Radio Astrophys, Urumqi 830011, Xinjiang, Peoples R China 3.Chinese Acad Sci, Key Lab Radio Astron & Technol, Beijing 100101, Peoples R China 4.Ludong Univ, Sch Phys & Optoelect Engn, Yantai 264025, Peoples R China 5.Chinese Acad Sci, Xinjiang Astron Observ, Urumqi 830011, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Hong-Yao,Yang, Chuan-Lu,Li, Xiaohu,et al. Two-dimensional Pt@g-C3N4/ReS2 Van Der Waals Heterostructure for photocatalytic hydrogen evolution with direct Z-scheme[J]. CHEMICAL PHYSICS LETTERS,2025,870:142101. |
| APA | Wang, Hong-Yao,Yang, Chuan-Lu,Li, Xiaohu,Liu, Yuliang,Zhao, Wenkai,&Gao, Feng.(2025).Two-dimensional Pt@g-C3N4/ReS2 Van Der Waals Heterostructure for photocatalytic hydrogen evolution with direct Z-scheme.CHEMICAL PHYSICS LETTERS,870,142101. |
| MLA | Wang, Hong-Yao,et al."Two-dimensional Pt@g-C3N4/ReS2 Van Der Waals Heterostructure for photocatalytic hydrogen evolution with direct Z-scheme".CHEMICAL PHYSICS LETTERS 870(2025):142101. |
入库方式： OAI收割
来源：新疆天文台
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。