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A Unified Strategy for Transition-Metal-Free Synthesis of Benzothienopyridines, Benzoselenopyridines, and Benzotelluropyridines and Related Analogues

文献类型：期刊论文

作者Wen, Zhaoyue7; Wu, Jianlian7; Wang, Chun7; Shen, Bingjie6; Fu, Mingyue7; Zheng, Xinni5; Lu, Cheng4; Chen, Wei7; Chen, Tie-Gen1,2,3
刊名ORGANIC LETTERS
出版日期2025-06-02
卷号27期号:23页码:6047-6053
ISSN号1523-7060
DOI10.1021/acs.orglett.5c01557
通讯作者Lu, Cheng(luchengjy@ust.hk) ; Chen, Wei(chenweicstq@163.com) ; Chen, Tie-Gen(chentiegen@simm.ac.cn)
英文摘要A transition-metal-free, unified synthetic approach has been developed for the efficient construction of benzothienopyridines, benzoselenopyridines, and benzotelluropyridines. This versatile methodology facilitates the formation of C-S, C-Se, and C-Te bonds through the cyclization reaction of readily available dihalogenated pyridyl biaryls with chalcogen sources (thiourea, elemental sulfur, selenium, or tellurium). Significantly, the derivatized products exhibit promising potential as building blocks for benzochalcogenophene-fused pyridine architectures and functional materials for organic optoelectronic applications, particularly in organic light-emitting diodes.
WOS关键词ANTICONFLICT ACTIVITY ; SULFIDE ; CONSTRUCTION ; THIOUREA
资助项目The 100 Talents Program of the Chinese Academy of Sciences ; Zhongshan Municipal Bureau of Science and Technology[2021B2014] ; Zhongshan Municipal Bureau of Science and Technology[CXTD2022013] ; Shanghai Rising-Star Program[21QA1411000] ; National Natural Science Foundation of China[22371303]
WOS研究方向Chemistry
语种英语
WOS记录号WOS:001500761000001
出版者AMER CHEMICAL SOC
源URL[http://119.78.100.183/handle/2S10ELR8/318219]  
专题中国科学院上海药物研究所
通讯作者Lu, Cheng; Chen, Wei; Chen, Tie-Gen
作者单位1.Southern Med Univ, Sch Pharmaceut Sci, Guangzhou 510515, Peoples R China
2.Chinese Acad Sci, Shanghai Inst Mat Med, Shanghai 201203, Peoples R China
3.Chinese Acad Sci, Zhongshan Inst Drug Discovery, Shanghai Inst Mat Med, Zhongshan 528400, Peoples R China
4.Hong Kong Univ Sci & Technol, Dept Chem, Hong Kong 999077, Peoples R China
5.Chinese Acad Sci, Zhongshan Inst Drug Discovery, Shanghai Inst Mat Med, Zhongshan 528400, Peoples R China
6.Southern Med Univ, Sch Pharmaceut Sci, Guangzhou 510515, Peoples R China
7.Southwest Jiaotong Univ, Sichuan Engn Res Ctr Biomimet Synth Nat Drugs, Sch Life Sci & Engn, Chengdu 610031, Peoples R China
推荐引用方式
GB/T 7714		 Wen, Zhaoyue,Wu, Jianlian,Wang, Chun,et al. A Unified Strategy for Transition-Metal-Free Synthesis of Benzothienopyridines, Benzoselenopyridines, and Benzotelluropyridines and Related Analogues[J]. ORGANIC LETTERS,2025,27(23):6047-6053.
APA Wen, Zhaoyue.,Wu, Jianlian.,Wang, Chun.,Shen, Bingjie.,Fu, Mingyue.,...&Chen, Tie-Gen.(2025).A Unified Strategy for Transition-Metal-Free Synthesis of Benzothienopyridines, Benzoselenopyridines, and Benzotelluropyridines and Related Analogues.ORGANIC LETTERS,27(23),6047-6053.
MLA Wen, Zhaoyue,et al."A Unified Strategy for Transition-Metal-Free Synthesis of Benzothienopyridines, Benzoselenopyridines, and Benzotelluropyridines and Related Analogues".ORGANIC LETTERS 27.23(2025):6047-6053.

入库方式： OAI收割

来源：上海药物研究所

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