Acid-promoted hydrothermal on Chinese herbal residue toward upgradation and denitrogenation capabilities
文献类型：期刊论文
| 作者 | Bi, Hao2,4; Wang, Zhiwei1; Zhan, Hao1,3; Leng, Lijian1; Zeng, Zhiyong1; Wang, Xinming; Liu, Huacai2; Yin, Xiuli2; Wu, Chuangzhi2 |
| 刊名 | FUEL PROCESSING TECHNOLOGY
 |
| 出版日期 | 2022-12-15 |
| 卷号 | 238页码:12 |
| 关键词 | Chinese herbal residue Acid-promoted hydrothermal Upgradation Denitrogenation Solid biofuel |
| ISSN号 | 0378-3820 |
| DOI | 10.1016/j.fuproc.2022.107518 |
| 通讯作者 | Zhan, Hao(isaaczhanhao@163.com) ; Liu, Huacai(liuhc@ms.giec.ac.cn) |
| 英文摘要 | Chinese herbal residue (CHR) is an association of renewable resource and hazardous waste, and high nitrogen content and low energy density are two primary obstacles to its efficient and clean thermal utilization. In this paper, acid-promoted hydrothermal was employed to probe the feasibility on CHR toward enhanced solid biofuel concerning upgradation and denitrogenation. A more excellent hydrothermal promoter (H2SO4) was demonstrated to upgrade and denitrogenate CHR with better energy (1.125) and nitrogen densities (0.586) at optimal conditions (160 degrees C, 0.5 N H2SO4), which could be attributed to the improved removal of oxygen, amino and ash during acid-promoted hydrothermal. Compared to raw feedstock or the conventional hydrochar, the acid-promoted hydrochar had enhanced compositional characteristics with higher heating value (21.00 kJ.mol(-1)), lower nitrogen (1.44 wt%) and ash (11.03 wt%) contents, thus showing more stable combustion flame with a higher comprehensive combustion index of 4.861 x 10(-8), a higher combustion stability index of 4979.342, lower combustion alkali index of 0.026, and less nitrogen gaseous pollutant emission. Thus, acid-promoted hydrothermal would be a promising way to convert CHR into much cleaner and higher-grade solid biofuel. |
| WOS关键词 | INDUSTRIAL BIOWASTES ; SEWAGE-SLUDGE ; COMBUSTION BEHAVIOR ; CHEMICAL-PROPERTIES ; CARBONIZATION HTC ; BIOMASS WASTE ; TG-FTIR ; PYROLYSIS ; CONVERSION ; NITROGEN |
| 资助项目 | National Natural Science Foundation of China[51906247] ; Guangdong Basic and Applied Basic Research Foundation[2020A1515011336] ; Science and Technology Planning Project of Guangdong Province of China[2021A0505030054] ; Science and Technology Program of Guangzhou[202002030421] |
| WOS研究方向 | Chemistry ; Energy & Fuels ; Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000892775800007 |
| 出版者 | ELSEVIER |
| 资助机构 | National Natural Science Foundation of China ; Guangdong Basic and Applied Basic Research Foundation ; Science and Technology Planning Project of Guangdong Province of China ; Science and Technology Program of Guangzhou |
| 源URL | [http://ir.giec.ac.cn/handle/344007/37963]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Zhan, Hao; Liu, Huacai |
| 作者单位 | 1.Sch Energy Sci & Engn, Cent South Univ, Changsha 410083, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangdong Key Lab New & Renewable Energy Res & De, Guangzhou 510640, Peoples R China 3.Chinese Acad Sci, Guangzhou Inst Geochemistry, State Key Lab Organ Geochemistry, Guangdong Key Lab Environm Protect & Resources Ut, Guangzhou 510640, Peoples R China 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Bi, Hao,Wang, Zhiwei,Zhan, Hao,et al. Acid-promoted hydrothermal on Chinese herbal residue toward upgradation and denitrogenation capabilities[J]. FUEL PROCESSING TECHNOLOGY,2022,238:12. |
| APA | Bi, Hao.,Wang, Zhiwei.,Zhan, Hao.,Leng, Lijian.,Zeng, Zhiyong.,...&Wu, Chuangzhi.(2022).Acid-promoted hydrothermal on Chinese herbal residue toward upgradation and denitrogenation capabilities.FUEL PROCESSING TECHNOLOGY,238,12. |
| MLA | Bi, Hao,et al."Acid-promoted hydrothermal on Chinese herbal residue toward upgradation and denitrogenation capabilities".FUEL PROCESSING TECHNOLOGY 238(2022):12. |
入库方式： OAI收割
来源：广州能源研究所
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