Membrane Electrode Assembly Degradation Modeling of Proton Exchange Membrane Fuel Cells: A Review
文献类型：期刊论文
| 作者 | Dafalla, Ahmed Mohmed1,2,3; Wei, Lin1,2,3; Habte, Bereket Tsegai1,2,3; Guo, Jian1,2,3; Jiang, Fangming1,2,3 |
| 刊名 | ENERGIES
 |
| 出版日期 | 2022-12-01 |
| 卷号 | 15期号:23页码:26 |
| 关键词 | PEMFC membrane electrode assembly proton exchange membrane gas diffusion layer catalyst layer durability degradation modeling real-time monitoring physical-based mechanistic models |
| DOI | 10.3390/en15239247 |
| 通讯作者 | Jiang, Fangming(jiangfm@ms.giec.ac.cn) |
| 英文摘要 | Proton exchange membrane fuel cells (PEMFCs) have been recognized as a promising power generation source for a wide range of automotive, stationary, and portable electronic applications. However, the durability of PEMFCs remains as one of the key barriers to their wide commercialization. The membrane electrode assembly (MEA) as a central part of a PEMFC, which consists of a proton exchange membrane with a catalyst layer (CL) and gas diffusion layer (GDL) on each side, is subject to failure and degradation in long-running and cycling load conditions. The real-time monitoring of the degradation evolution process through experimental techniques is challenging. Therefore, different numerical modeling approaches were proposed in the literature to assist the understanding of the degradation mechanisms in PEMFCs. To provide modeling progress in the addressed field, this paper briefly discusses the different degradation mechanisms occurring in the MEA. In particular, we present a detailed review of MEA degradation modeling research work, with special attention paid to the physical-based models (mechanistic models). Following the most recent relevant literature, the results showed that the combination of microstructure component models with macro-scale comprehensive PEMFC models provides a better understanding of degradation mechanisms when compared to single-scale degradation models. In this sense, it is concluded that in order to develop an accurate and efficient predictive degradation model, the different relevant scales ranging from nano- to macro-sized scales should be considered, and coupling techniques for multiscale modeling have to be advanced. Finally, the paper summarizes the degradation models for different MEA components. It is highlighted that the GDL chemical degradation models that describe damage accumulation are relatively limited. The paper provides a useful reference for the recent developments in the MEA degradation modeling of PEMFCs. |
| WOS关键词 | GAS-DIFFUSION LAYER ; COLD START PERFORMANCE ; CATHODE CATALYST LAYER ; FATIGUE-CRACK GROWTH ; INHOMOGENEOUS COMPRESSION ; CHEMICAL DEGRADATION ; MECHANICAL DEGRADATION ; MICROSTRUCTURE CHANGES ; PLATINUM DISSOLUTION ; TRANSPORT-PROPERTIES |
| 资助项目 | National Natural Science Foundation of China[52006226] ; CAS-VPST Silk Road Science Fund[182344KYSB20210007] ; Guangzhou Science and Technology Plan[202102020356] ; New Energy Technology Co., Ltd. |
| WOS研究方向 | Energy & Fuels |
| 语种 | 英语 |
| WOS记录号 | WOS:000897557100001 |
| 出版者 | MDPI |
| 资助机构 | National Natural Science Foundation of China ; CAS-VPST Silk Road Science Fund ; Guangzhou Science and Technology Plan ; New Energy Technology Co., Ltd. |
| 源URL | [http://ir.giec.ac.cn/handle/344007/38078]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Jiang, Fangming |
| 作者单位 | 1.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 3.CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China |
| 推荐引用方式 GB/T 7714 | Dafalla, Ahmed Mohmed,Wei, Lin,Habte, Bereket Tsegai,et al. Membrane Electrode Assembly Degradation Modeling of Proton Exchange Membrane Fuel Cells: A Review[J]. ENERGIES,2022,15(23):26. |
| APA | Dafalla, Ahmed Mohmed,Wei, Lin,Habte, Bereket Tsegai,Guo, Jian,&Jiang, Fangming.(2022).Membrane Electrode Assembly Degradation Modeling of Proton Exchange Membrane Fuel Cells: A Review.ENERGIES,15(23),26. |
| MLA | Dafalla, Ahmed Mohmed,et al."Membrane Electrode Assembly Degradation Modeling of Proton Exchange Membrane Fuel Cells: A Review".ENERGIES 15.23(2022):26. |
入库方式： OAI收割
来源：广州能源研究所
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