Mild organosolv pretreatment of sugarcane bagasse with acetone/phenoxyethanol/water for enhanced sugar production
文献类型：期刊论文
| 作者 | Li, Wuhuan2,6; Tan, Xuesong6; Miao, Changlin6; Zhang, Zhanying1; Wang, Yunxuan3; Ragauskas, Arthur J.3,4,5; Zhuang, Xinshu2,6 |
| 刊名 | GREEN CHEMISTRY
 |
| 出版日期 | 2023-02-06 |
| 卷号 | 25期号:3页码:1169-1178 |
| ISSN号 | 1463-9262 |
| DOI | 10.1039/d2gc04404h |
| 通讯作者 | Tan, Xuesong(tanxs@ms.giec.ac.cn) ; Zhuang, Xinshu(zhuangxs@ms.giec.ac.cn) |
| 英文摘要 | This study conducted mild organosolv pretreatment of sugarcane bagasse with acetone/phenoxyethanol/water (APW) solutions to improve sugar production in the subsequent enzymatic hydrolysis step. The Box-Behnken design was used to optimize pretreatment conditions based on lignin removal. Further examination of the data revealed that lignin removal was positively correlated (R-2 > 0.95) with the combined severity factor (CSF). Pretreatment under the optimal conditions (125 degrees C-120 min, 0.17 M H2SO4, liquid-solid ratio of 15) led to 98.1% lignin removal and 74.5% cellulose digestibility compared to a low digestibility of 9.3% with raw sugarcane bagasse (SCB). Moreover, the APW process showed effective fractionation of pine, corn stalk and bamboo, and lignin removal was over 90%. The recovered lignin was characterized by 2D-HSQC NMR and P-31 NMR, suggesting that the pretreatment resulted in breakage of beta-O-4, total phenolic OH and H-units increased. However, the enzymatic hydrolysis efficiency (EHE) of samples with a lower lignin content (<4%) varied significantly. Correlations between various substrate-related factors of the pretreated SCB and EHE were analyzed to understand this observation. The results showed that the surface area of cellulose, lateral order index, CrI, and specific surface area were the predominant factors for enzymatic hydrolysis rather than lignin properties. |
| WOS关键词 | DILUTE-ACID PRETREATMENT ; ENZYMATIC-HYDROLYSIS ; LIGNOCELLULOSIC BIOMASS ; ALKALINE PRETREATMENT ; SURFACE-AREA ; HOT-WATER ; LIGNIN ; FRACTIONATION ; INSIGHTS ; POROSITY |
| 资助项目 | International Science and Technology Innovation Cooperation Program of the National Key Research and Development Plan of China[2021YFE0114400] ; National Natural Science Foundation of China[51976221] ; Guangdong Basic and Applied Basic Research Foundation[2022A1515012078] ; University of Tennessee, Knoxville |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics |
| 语种 | 英语 |
| WOS记录号 | WOS:000919849400001 |
| 出版者 | ROYAL SOC CHEMISTRY |
| 资助机构 | International Science and Technology Innovation Cooperation Program of the National Key Research and Development Plan of China ; National Natural Science Foundation of China ; Guangdong Basic and Applied Basic Research Foundation ; University of Tennessee, Knoxville |
| 源URL | [http://ir.giec.ac.cn/handle/344007/38334]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Tan, Xuesong; Zhuang, Xinshu |
| 作者单位 | 1.Queensland Univ Technol, Fac Engn, Fac Sci, Ctr Agr & Bioecon, Brisbane, Qld 4000, Australia 2.Univ Sci & Technol China, Sch Energy Sci & Engn, Hefei 230026, Peoples R China 3.Univ Tennessee Knoxville, Dept Chem & Biomol Engn, Knoxville, TN USA 4.Oak Ridge Natl Lab, Joint Inst Biol Sci, Biosci Div, Oak Ridge, TN USA 5.Univ Tennessee, Inst Agr, Ctr Renewable Carbon, Dept Forestry Wildlife & Fisheries, Knoxville, TN USA 6.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China |
| 推荐引用方式 GB/T 7714 | Li, Wuhuan,Tan, Xuesong,Miao, Changlin,et al. Mild organosolv pretreatment of sugarcane bagasse with acetone/phenoxyethanol/water for enhanced sugar production[J]. GREEN CHEMISTRY,2023,25(3):1169-1178. |
| APA | Li, Wuhuan.,Tan, Xuesong.,Miao, Changlin.,Zhang, Zhanying.,Wang, Yunxuan.,...&Zhuang, Xinshu.(2023).Mild organosolv pretreatment of sugarcane bagasse with acetone/phenoxyethanol/water for enhanced sugar production.GREEN CHEMISTRY,25(3),1169-1178. |
| MLA | Li, Wuhuan,et al."Mild organosolv pretreatment of sugarcane bagasse with acetone/phenoxyethanol/water for enhanced sugar production".GREEN CHEMISTRY 25.3(2023):1169-1178. |
入库方式： OAI收割
来源：广州能源研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。