Hydrogen-rich syngas production by catalytic cracking of polypropylene over activated carbon based monometallic and bimetallic Fe/Ni catalysts
文献类型：期刊论文
| 作者 | Wang, Shuxiao1,2,3,4; Sun, Yibo2,3,4; Shan, Rui2,3,4; Gu, Jing2,3,4; Huhe, Taoli1,2; Ling, Xiang1; Yuan, Haoran2,3,4,6; Chen, Yong1,2,3,4,5,7 |
| 刊名 | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
 |
| 出版日期 | 2023-07-22 |
| 卷号 | 48期号:62页码:23821-23830 |
| 关键词 | H2 production Catalytic reforming Pyrolysis Plastic Carbon nanotubes |
| ISSN号 | 0360-3199 |
| DOI | 10.1016/j.ijhydene.2023.03.230 |
| 通讯作者 | Yuan, Haoran(yuanhr@ms.giec.ac.cn) ; Chen, Yong(chenyong@ms.giec.ac.cn) |
| 英文摘要 | The aim of this study is to efficiently produce hydrogen-rich syngas. The thermal con-version experiment of polypropylene was carried out in a two-stage pyrolytic-catalytic device. Activated carbon based catalyst was developed, the catalytic performance of monomial and bimetallic catalysts was explored, and the influence of metal addition ratio in bimetallic catalysts on hydrogen production performance was analyzed. The micro-scopic morphology and structural characterization of the unreacted and spent catalyst were analyzed, and the effect of active substance in catalyst on the reaction performance was described. Under optimized reaction conditions, bimetallic catalyst 5Fe-10Ni had excellent catalytic activity, large hydrogen yield (136.32 mmol/gPP) and high carbon depo-sition quality. For this high performance catalyst, the catalyst stability was verified by 10 cycles of recycling experiments. The method of hydrogen production from waste plastic cracking in this paper will provide new ideas for high value utilization of plastic and hydrogen production.& COPY; 2023 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved. |
| WOS关键词 | FE-NI ; WASTE PLASTICS ; GASIFICATION ; COPRODUCTION ; CONVERSION ; PYROLYSIS ; NANOTUBES ; BIOMASS ; TAR |
| 资助项目 | National Key R amp; D Program of China[2022YFC3902402] ; CAS Project for Young Scientists in Basic Research[YSBR-044] ; National Natural Science Funds of China[51976223] ; Guangdong Basic and Applied Basic Research Foundation[2021B1515020068] |
| WOS研究方向 | Chemistry ; Electrochemistry ; Energy & Fuels |
| 语种 | 英语 |
| WOS记录号 | WOS:001039774700001 |
| 出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
| 资助机构 | National Key R amp; D Program of China ; CAS Project for Young Scientists in Basic Research ; National Natural Science Funds of China ; Guangdong Basic and Applied Basic Research Foundation |
| 源URL | [http://ir.giec.ac.cn/handle/344007/39236]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Yuan, Haoran; Chen, Yong |
| 作者单位 | 1.Nanjing Tech Univ, Nanjing 211816, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 3.CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 4.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China 5.Changzhou Univ, Changzhou 213164, Peoples R China 6.Chinese Acad Sci, Guangzhou Inst Energy Convers, 2 Nengyuan Rd, Guangzhou 510640, Guangdong, Peoples R China 7.Nanjing Tech Univ, 30 Puzhu South Rd, Nanjing 211816, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Shuxiao,Sun, Yibo,Shan, Rui,et al. Hydrogen-rich syngas production by catalytic cracking of polypropylene over activated carbon based monometallic and bimetallic Fe/Ni catalysts[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2023,48(62):23821-23830. |
| APA | Wang, Shuxiao.,Sun, Yibo.,Shan, Rui.,Gu, Jing.,Huhe, Taoli.,...&Chen, Yong.(2023).Hydrogen-rich syngas production by catalytic cracking of polypropylene over activated carbon based monometallic and bimetallic Fe/Ni catalysts.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,48(62),23821-23830. |
| MLA | Wang, Shuxiao,et al."Hydrogen-rich syngas production by catalytic cracking of polypropylene over activated carbon based monometallic and bimetallic Fe/Ni catalysts".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 48.62(2023):23821-23830. |
入库方式： OAI收割
来源：广州能源研究所
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