Chemical recycling of plastic wastes via homogeneous catalysis: A review
文献类型：期刊论文
| 作者 | Chen, Xueru1,2; Cheng, Leilei1,2; Gu, Jing1,2; Yuan, Haoran1,2; Chen, Yong1,2 |
| 刊名 | CHEMICAL ENGINEERING JOURNAL
 |
| 出版日期 | 2024 |
| 卷号 | 479页码:22 |
| 关键词 | Homogeneous catalyst Catalysis mechanism Chemical recycling Chemical depolymerization Closed-loop recovery |
| ISSN号 | 1385-8947 |
| DOI | 10.1016/j.cej.2023.147853 |
| 通讯作者 | Yuan, Haoran(yuanhr@ms.giec.ac.cn) |
| 英文摘要 | Improper disposal of plastic wastes causes serious negative impacts on the ecosystem. These plastic wastes are considered to be a rich carbon resource, and the use of homogeneous catalytic chemical recycling methods has enabled the high-value recovery of plastic wastes under mild conditions to obtain liquid fuels (alkane, cycloalkane and aromatic hydrocarbon etc.), high-value chemicals (terephthalic acid, bisphenol A and diols), and plastic monomers (bis(hydroxyalkyl) terephthalate). This review summarizes recent advances in homogeneous catalysis of plastic polymers for the preparation of high-value chemicals. The bond breaking mechanism of plastics using different homogeneous catalysts and the relationship between catalyst active sites and catalytic performance are systematically discussed in each section. Finally, we evaluate the current homogeneous catalytic chemical recycling routes for plastic wastes. Chemical recycling through homogeneous catalysis is a bright way to realize the circular economy of plastic wastes. |
| WOS关键词 | ANHYDRIDE-CURED EPOXY ; FIBER-REINFORCED COMPOSITES ; CONTAINING IONIC LIQUIDS ; CARBON-FIBER ; POLYETHYLENE TEREPHTHALATE ; SUPERCRITICAL WATER ; SELECTIVE CLEAVAGE ; RESIN COMPOSITES ; CYCLIC CARBONATES ; DEGRADATION |
| 资助项目 | CAS Project for Young Scientists in Basic Research[YSBR-044] |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:001135323300001 |
| 出版者 | ELSEVIER SCIENCE SA |
| 资助机构 | CAS Project for Young Scientists in Basic Research |
| 源URL | [http://ir.giec.ac.cn/handle/344007/40584]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Yuan, Haoran |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 2.Univ Sci & Technol China, Sch Energy Sci & Engn, Hefei 230026, Peoples R China |
| 推荐引用方式 GB/T 7714 | Chen, Xueru,Cheng, Leilei,Gu, Jing,et al. Chemical recycling of plastic wastes via homogeneous catalysis: A review[J]. CHEMICAL ENGINEERING JOURNAL,2024,479:22. |
| APA | Chen, Xueru,Cheng, Leilei,Gu, Jing,Yuan, Haoran,&Chen, Yong.(2024).Chemical recycling of plastic wastes via homogeneous catalysis: A review.CHEMICAL ENGINEERING JOURNAL,479,22. |
| MLA | Chen, Xueru,et al."Chemical recycling of plastic wastes via homogeneous catalysis: A review".CHEMICAL ENGINEERING JOURNAL 479(2024):22. |
入库方式： OAI收割
来源：广州能源研究所
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