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A novelty catalytic reforming of tire pyrolysis oil for hydrogen-rich syngas

文献类型：期刊论文

作者Wang, Fengchao1; Gao, Ningbo2; Quan, Cui2; Liu, Huacai1; Li, Weizhen1; Yuan, Hongyou1; Yin, Xiuli1
刊名ENERGY CONVERSION AND MANAGEMENT
出版日期2024-01-15
卷号300页码:10
关键词Catalytic reforming Pyrolysis char Pyrolysis oil Nickel Bottom ash
ISSN号0196-8904
DOI10.1016/j.enconman.2023.117925
通讯作者Gao, Ningbo(nbogao@xjtu.edu.cn) ; Yin, Xiuli(xlyin@ms.giec.ac.cn)
英文摘要Pyrolysis oil and pyrolysis char from waste tires have been reported with poor quality but could be a source and catalyst for generating hydrogen-rich syngas, respectively. In this study, the influence of two-layer catalysts on the catalytic reforming syngas distribution derived from side wall rubber pyrolysis oil (SWRPO) was explored. The side wall rubber pyrolysis char (SWRC), as a catalyst and carrier support of nickel, was used as the first-layer catalyst, and the calcined bottom ash (CBA) from oil sludge combustion was used as the secondary catalyst. Steam was used as an activator to activate SWRC and improve the concentration of CO and H-2 in catalytic reforming syngas. Different analysis methods (BET, XRD, SEM, and Raman) were employed to characterize the properties of catalysts. Consequently, the yield and LHV of syngas increased from 0.05 g.(-1)(goil) and 2.03 kJ.g(-1) to 0.42 g.g(oil)(-1) and 11.32 kJ.g(-1), respectively. The H-2 concentration increased from 20.38 vol% to 44.68 vol% in syngas with two-layer catalysts, and the H-2 selectivity reached 0.16. The yield of carbon deposit increased to 0.57 g.g(oil)(-1) with the SWRPO total conversion of 95.55 %. The lifetime of two-layer catalysts reached 17 h with a stability conversion process of SWRPO.
WOS关键词IN-SITU ; TAR ; WASTE ; CHAR ; HUSK
资助项目National Natural Science Foundation of China[52376207] ; National Natural Science Foundation of China[52276211] ; Sci-ence and Technology Exchange Project of China Ministry of Science and Technology ; Strategic Priority Research Program of Chinese Academy of Sciences[XDA29010400]
WOS研究方向Thermodynamics ; Energy & Fuels ; Mechanics
语种英语
WOS记录号WOS:001129553600001
出版者PERGAMON-ELSEVIER SCIENCE LTD
资助机构National Natural Science Foundation of China ; Sci-ence and Technology Exchange Project of China Ministry of Science and Technology ; Strategic Priority Research Program of Chinese Academy of Sciences
源URL[http://ir.giec.ac.cn/handle/344007/40621]  
专题中国科学院广州能源研究所
通讯作者Gao, Ningbo; Yin, Xiuli
作者单位1.Chinese Acad Sci, CAS Key Lab Renewable Energy, Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
2.Xi An Jiao Tong Univ, Sch Energy & Power Engn, Xian 710049, Peoples R China
推荐引用方式
GB/T 7714		 Wang, Fengchao,Gao, Ningbo,Quan, Cui,et al. A novelty catalytic reforming of tire pyrolysis oil for hydrogen-rich syngas[J]. ENERGY CONVERSION AND MANAGEMENT,2024,300:10.
APA Wang, Fengchao.,Gao, Ningbo.,Quan, Cui.,Liu, Huacai.,Li, Weizhen.,...&Yin, Xiuli.(2024).A novelty catalytic reforming of tire pyrolysis oil for hydrogen-rich syngas.ENERGY CONVERSION AND MANAGEMENT,300,10.
MLA Wang, Fengchao,et al."A novelty catalytic reforming of tire pyrolysis oil for hydrogen-rich syngas".ENERGY CONVERSION AND MANAGEMENT 300(2024):10.

入库方式： OAI收割

来源：广州能源研究所

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