Fractionation of poplar through solid acid pretreatment assisted by mild alkali-1-butanol immersion to effectively produce xylose, glucose, and solid lignin
文献类型:期刊论文
| 作者 | Chen, Yang1,2; Qi, Wei1; Shakeel, Usama1; Liang, Cuiyi1; Wang, Wen1; Hu, Yunzi1; Wang, Zhongming1; Yuan, Zhenhong1; Shen, Fei2; Wang, Qiong1 |
| 刊名 | BIOMASS CONVERSION AND BIOREFINERY
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| 出版日期 | 2023-06-16 |
| 页码 | 19 |
| 关键词 | Lignocellulose pretreatment Solid acid catalyst Xylose Glucose Enzymatic hydrolysis |
| ISSN号 | 2190-6815 |
| DOI | 10.1007/s13399-023-04378-4 |
| 通讯作者 | Shen, Fei(fishen@sicau.edu.cn) ; Wang, Qiong(wangqiong@ms.giec.ac.cn) |
| 英文摘要 | The efficient fractionation and recovery of lignocellulosic biomass (LCB) constituents, hemicellulose, cellulose, and lignin, are ideal for LCB utilization. In this study, we prepared a solid acid catalyst (SPS120-40) with high acid density using polystyrene resin (PS) as precursor. The synthesized catalyst was characterized by XPS, C-13 NMR, TG-FTIR-MS, and so on to investigate its structural properties and thermal stability. During process optimization using FeCl3- assisted SPS120-40, a total of 78.9% xylose yield with 96.6% monosaccharide selectivity was achieved. Moreover, the catalyst showed extraordinary catalytic activity until five runs without significant loss in xylose yield. The pretreated residue was further treated with NaOH-1-butanol to effectively remove the lignin deposited on the residue surface and eventually 89.5% hydrolysis rate was obtained. At the same time, 64.4% lignin was obtained in the residue of enzymatic hydrolysis. This work provides important guidance for utilizing the whole components of lignocellulose. |
| WOS关键词 | ENZYMATIC SACCHARIFICATION ; HYDROTHERMAL PRETREATMENT ; POLYSTYRENE MICROSPHERES ; LIGNOCELLULOSIC BIOMASS ; SUGARCANE BAGASSE ; HYDROLYSIS ; CELLULOSE ; CONVERSION ; CHEMISTRY ; MECHANISM |
| 资助项目 | National Key Research and Development Program of China[2019YFB1503801] ; National Natural Science Foundation of China[51976224] ; National Natural Science Foundation of China[52006227] ; Key Fundamental Research Project of Guangdong-Guangxi Joint Funding[2020B1515420005] ; Youth Innovation Promotion Association, CAS[2021351] ; Guangzhou Science and Technology Program[202201010563] |
| WOS研究方向 | Energy & Fuels ; Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:001163748400001 |
| 出版者 | SPRINGER HEIDELBERG |
| 资助机构 | National Key Research and Development Program of China ; National Natural Science Foundation of China ; Key Fundamental Research Project of Guangdong-Guangxi Joint Funding ; Youth Innovation Promotion Association, CAS ; Guangzhou Science and Technology Program |
| 源URL | [http://ir.giec.ac.cn/handle/344007/41190] ![]() |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Shen, Fei; Wang, Qiong |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 2.Sichuan Agr Univ, Inst Ecol & Environm Sci, Environm Coll, Chengdu 611130, Sichuan, Peoples R China |
| 推荐引用方式 GB/T 7714 | Chen, Yang,Qi, Wei,Shakeel, Usama,et al. Fractionation of poplar through solid acid pretreatment assisted by mild alkali-1-butanol immersion to effectively produce xylose, glucose, and solid lignin[J]. BIOMASS CONVERSION AND BIOREFINERY,2023:19. |
| APA | Chen, Yang.,Qi, Wei.,Shakeel, Usama.,Liang, Cuiyi.,Wang, Wen.,...&Wang, Qiong.(2023).Fractionation of poplar through solid acid pretreatment assisted by mild alkali-1-butanol immersion to effectively produce xylose, glucose, and solid lignin.BIOMASS CONVERSION AND BIOREFINERY,19. |
| MLA | Chen, Yang,et al."Fractionation of poplar through solid acid pretreatment assisted by mild alkali-1-butanol immersion to effectively produce xylose, glucose, and solid lignin".BIOMASS CONVERSION AND BIOREFINERY (2023):19. |
入库方式: OAI收割
来源:广州能源研究所
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