In Situ Ca- and Mg- Codoped Biochar Derived from Tobacco Stem for Phosphate Adsorption and Desorption
文献类型：期刊论文
| 作者 | Tu, Panfeng1; Cen, Yingyuan1; Deng, Lansheng2; Huang, Baoyuan2; Li, Juan1; Li, Yongquan1; Deng, Lifang2; Yuan, Haoran2,3 |
| 刊名 | CHEMISTRYSELECT
 |
| 出版日期 | 2024-04-04 |
| 卷号 | 9期号:13页码:13 |
| 关键词 | in situ Ca and Mg co-doped biochar tobacco stems phosphate adsorption and desorption |
| ISSN号 | 2365-6549 |
| DOI | 10.1002/slct.202304674 |
| 通讯作者 | Deng, Lifang(nannandeng@163.com) |
| 英文摘要 | Phosphorus is an important element for plant growth. The efficient use and recovery of phosphorus is crucial due to limited phosphate resource reserves. This study explored the potential application of an in situ Ca and Mg co-doped biochar derived from tobacco stem to reclaim and reuse phosphate from aqueous solutions. We performed various batch adsorption experiments and industrial analysis based on different parameters. The findings indicate that biochar prepared using the raw material particle size range of 0.85-2 mm and pyrolyzed at 800 degrees C presented good pore structure and specific surface area. Ca and Mg elements in biochar exhibited great influence on its phosphate adsorption property. The maximum phosphate adsorption capacity of the tobacco stem-based biochar was 54.66 mg/g, and the experimental data agreed with the Langmuir equation, suggesting monolayer adsorption. The adsorption process conformed to the pseudo-second-order kinetic equation, indicating that chemisorption was the dominant adsorption process and that the adsorption was controlled by intra-particle diffusion. Furthermore, phosphate adsorbed on tobacco stem-based in situ Ca and Mg co-doped biochar was released under acidic, alkaline, and neutral conditions. Therefore, in situ Ca and Mg co-doped biochar prepared from tobacco stems is a potential environmentally friendly and low-cost adsorbent for phosphorus recovery. |
| WOS关键词 | AQUEOUS-SOLUTION ; RECOVERY ; COMPOSITE ; REMOVAL ; BEADS |
| 资助项目 | National Natural Science Foundation of China ; Basic and Applied Basic Research Foundation of Guangdong Province[2022A1515010941] ; Science and technology plan projects of Guangzhou[202206010069] ; Meizhou Science and Technology Project[2021A0304001] ; Key-Area Research and Development Program of Guangdong Province[2020B020215003] ; [42377211] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:001195339700001 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 资助机构 | National Natural Science Foundation of China ; Basic and Applied Basic Research Foundation of Guangdong Province ; Science and technology plan projects of Guangzhou ; Meizhou Science and Technology Project ; Key-Area Research and Development Program of Guangdong Province |
| 源URL | [http://ir.giec.ac.cn/handle/344007/41336]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Deng, Lifang |
| 作者单位 | 1.Zhongkai Univ Agr & Engn, Guangzhou 510225, Peoples R China 2.South China Agr Univ, Inst Biomass Engn, Guangzhou 510642, Peoples R China 3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China |
| 推荐引用方式 GB/T 7714 | Tu, Panfeng,Cen, Yingyuan,Deng, Lansheng,et al. In Situ Ca- and Mg- Codoped Biochar Derived from Tobacco Stem for Phosphate Adsorption and Desorption[J]. CHEMISTRYSELECT,2024,9(13):13. |
| APA | Tu, Panfeng.,Cen, Yingyuan.,Deng, Lansheng.,Huang, Baoyuan.,Li, Juan.,...&Yuan, Haoran.(2024).In Situ Ca- and Mg- Codoped Biochar Derived from Tobacco Stem for Phosphate Adsorption and Desorption.CHEMISTRYSELECT,9(13),13. |
| MLA | Tu, Panfeng,et al."In Situ Ca- and Mg- Codoped Biochar Derived from Tobacco Stem for Phosphate Adsorption and Desorption".CHEMISTRYSELECT 9.13(2024):13. |
入库方式： OAI收割
来源：广州能源研究所
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