Cooperative production of monophenolic chemicals and carbon adsorption materials from cascade pyrolysis of acid hydrolysis lignin
文献类型：期刊论文
| 作者 | Xu, Ying2,3,4; Fan, Zhiqiang3; Li, Xianchun3; Yang, Shaoqi2; Wang, Jin2; Zheng, Anqing2; Shu, Riyang1 |
| 刊名 | BIORESOURCE TECHNOLOGY
 |
| 出版日期 | 2024-05-01 |
| 卷号 | 399页码:8 |
| 关键词 | Lignin Hydrolysis residues Phenols Pyrolysis char Adsorption capacity |
| ISSN号 | 0960-8524 |
| DOI | 10.1016/j.biortech.2024.130557 |
| 通讯作者 | Zheng, Anqing(zhengaq@ms.giec.ac.cn) ; Shu, Riyang(shuriyang@gdut.edu.cn) |
| 英文摘要 | A novel cascade pyrolysis upgrading process for acid hydrolysis lignin (AHL), consisting of pyrolysis, catalytic upgrading of pyrolysis vapors, and pyrolysis char, was developed to improve the yield of value-added products (monophenolic chemicals and carbon materials). Pyrolysis of AHL at 450 degrees C and subsequent catalytic upgrading of pyrolysis vapors over Ni/H-ZSM-5 boosted the concentration of monophenolic chemicals in pyrolysis liquids by 58%. The carbon material prepared from pyrolysis char using KOH as activating agent exhibited a large specific surface area of 2902.5 m2/g and a large total pore volume of 1.45 cm3/g, thus affording good adsorption capacity for methylene blue (824.87 mg/g) and iodine (2333.17 mg/g). Moreover, the cascade pyrolysis upgrading of AHL achieved a yield of 68.52% desired products, which was much higher than the reported results (single production of monophenols and pyrolysis char). In summary, this work provides a potential reference for efficient utilization of lignin in large-scale applications. |
| WOS关键词 | ACTIVATED CARBON ; KOH ACTIVATION ; DEPOLYMERIZATION ; PRETREATMENT ; MECHANISM ; RELEVANCE |
| 资助项目 | National Natural Science Foundation of China[22178340] ; Young Elite Scientists Sponsorship Program by CAST[2022QNRC001] ; Guangdong Natural Science Foundation[2023A1515030159] ; Guangzhou Basic and Applied Basic Research Foundation[202201010630] |
| WOS研究方向 | Agriculture ; Biotechnology & Applied Microbiology ; Energy & Fuels |
| 语种 | 英语 |
| WOS记录号 | WOS:001221433800001 |
| 出版者 | ELSEVIER SCI LTD |
| 资助机构 | National Natural Science Foundation of China ; Young Elite Scientists Sponsorship Program by CAST ; Guangdong Natural Science Foundation ; Guangzhou Basic and Applied Basic Research Foundation |
| 源URL | [http://ir.giec.ac.cn/handle/344007/41646]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Zheng, Anqing; Shu, Riyang |
| 作者单位 | 1.Guangdong Univ Technol, Sch Mat & Energy, Guangdong Prov Key Lab Funct Soft Condensed Matter, Guangzhou 510006, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 3.Univ Sci & Technol Liaoning, Coll Chem Engn, Anshan 114000, Peoples R China 4.Jimei Univ, Coll Mech Equipment & Mech Engn, Fujian Prov Clean Combust & Energy Utilizat Res Ct, Fujian Prov Key Lab Energy Clean Utilizat & Dev, Xiamen 316021, Peoples R China |
| 推荐引用方式 GB/T 7714 | Xu, Ying,Fan, Zhiqiang,Li, Xianchun,et al. Cooperative production of monophenolic chemicals and carbon adsorption materials from cascade pyrolysis of acid hydrolysis lignin[J]. BIORESOURCE TECHNOLOGY,2024,399:8. |
| APA | Xu, Ying.,Fan, Zhiqiang.,Li, Xianchun.,Yang, Shaoqi.,Wang, Jin.,...&Shu, Riyang.(2024).Cooperative production of monophenolic chemicals and carbon adsorption materials from cascade pyrolysis of acid hydrolysis lignin.BIORESOURCE TECHNOLOGY,399,8. |
| MLA | Xu, Ying,et al."Cooperative production of monophenolic chemicals and carbon adsorption materials from cascade pyrolysis of acid hydrolysis lignin".BIORESOURCE TECHNOLOGY 399(2024):8. |
入库方式： OAI收割
来源：广州能源研究所
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