Unveiling the role of lignin feature on bio-ethanol and xylose derived from poplar during combined alkali/ethanol synergistic pretreatment
文献类型：期刊论文
| 作者 | Fan, Meishan4,5; Lei, Ming3; Liu, Zhu4; Li, Jun1,2; Zhang, Hongdan5; Xie, Jun5; Chen, Yong5 |
| 刊名 | INDUSTRIAL CROPS AND PRODUCTS
 |
| 出版日期 | 2024-07-01 |
| 卷号 | 213页码:11 |
| 关键词 | NaOH catalyzed ethanol pretreatment Bioethanol Xylose Lignin |
| ISSN号 | 0926-6690 |
| DOI | 10.1016/j.indcrop.2024.118408 |
| 通讯作者 | Zhang, Hongdan(hdzhang@scau.edu.cn) ; Xie, Jun(xiejun@scau.edu.cn) |
| 英文摘要 | This study adopted a mixed experimental research design to investigate the effects of alkali and alkali-catalyzed ethanol pretreatment of poplar wood under different NaOH loadings on the pretreatment liquid, pretreatment solids, and polysaccharide conversion, with a particular emphasis on the utility of the lignin for subsequent conversion. Specifically, NaOH catalyzed ethanol pretreatment at 10% NaOH loading resulted in the removal of more than 80% lignin with >80% carbohydrates remaining in the residual solids. Simultaneous saccharification fermentation of this pretreated residue resulted in 29.09 g/L (72.84%) and 14.86 g/L (69.26%) of ethanol and xylose, respectively, following a fermentation period of 72 h. Then, an integrated evaluation of the lignin characterization in raw and pretreated residues was carried out to emphasize their influence on ethanol and xylose yield by two-dimensional heteronuclear single quantum coherence (2D-HSQC) NMR and gel permeation chromatography (GPC) analysis. The results showed that most of the side-chain structures were oxidized and the aryl-ether bond was dissociated with the synergistic influence of NaOH and ethanol treatment, accompanied by low molecular weight lignin obtained in the solid fraction. Overall, NaOH catalyzed ethanol pretreatment offered a strategy for selective biomass fractionation into carbohydrates conversion and lignin valorization with a high yield. |
| WOS关键词 | ORGANOSOLV PRETREATMENT ; BIOMASS RECALCITRANCE ; HYDROGEN-PEROXIDE ; INSIGHTS ; VARIANTS ; ALKALI |
| 资助项目 | National Key Research and Development Program of China[2021YFC2101602] ; National Key Research and Development Program of China[2021YFC2101603] ; National Natural Science Foundation of China[21978108] ; National Natural Science Foundation of China[42271269] ; Guangdong Basic and Applied Basic Research Foundation[2019A1515011624] |
| WOS研究方向 | Agriculture |
| 语种 | 英语 |
| WOS记录号 | WOS:001224017800001 |
| 出版者 | ELSEVIER |
| 资助机构 | National Key Research and Development Program of China ; National Natural Science Foundation of China ; Guangdong Basic and Applied Basic Research Foundation |
| 源URL | [http://ir.giec.ac.cn/handle/344007/41789]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Zhang, Hongdan; Xie, Jun |
| 作者单位 | 1.Sun Yat Sen Univ, Sch Int Relat, Guangzhou, Peoples R China 2.Deakin Univ, Fac Business & Law, Burwood, Australia 3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 4.Shaoguan Univ, Henry Fok Sch Biol & Agr, Guangdong Prov Key Lab Utilizat & Conservat Food &, Shaoguan 512005, Peoples R China 5.South China Agr Univ, Guangdong Engn Technol Res Ctr Agr & Forestry Biom, Key Lab Energy Plants Resource & Utilizat, Inst Biomass Engn,Minist Agr & Rural Affairs, Guangzhou 510642, Peoples R China |
| 推荐引用方式 GB/T 7714 | Fan, Meishan,Lei, Ming,Liu, Zhu,et al. Unveiling the role of lignin feature on bio-ethanol and xylose derived from poplar during combined alkali/ethanol synergistic pretreatment[J]. INDUSTRIAL CROPS AND PRODUCTS,2024,213:11. |
| APA | Fan, Meishan.,Lei, Ming.,Liu, Zhu.,Li, Jun.,Zhang, Hongdan.,...&Chen, Yong.(2024).Unveiling the role of lignin feature on bio-ethanol and xylose derived from poplar during combined alkali/ethanol synergistic pretreatment.INDUSTRIAL CROPS AND PRODUCTS,213,11. |
| MLA | Fan, Meishan,et al."Unveiling the role of lignin feature on bio-ethanol and xylose derived from poplar during combined alkali/ethanol synergistic pretreatment".INDUSTRIAL CROPS AND PRODUCTS 213(2024):11. |
入库方式： OAI收割
来源：广州能源研究所
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