中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Selective Hydrogenation of 5-Hydroxymethylfurfural to 2,5-bis(hydroxymethyl)furan by Pt/Ni@C Catalyst

文献类型:期刊论文

作者Xu, Xian4; Lan, Ling4; Xu, Jiangong3; Liang, Zheng2; Tan, Jin1; Wang, Haiyong2; Qiu, Songbai4
刊名CATALYSIS LETTERS
出版日期2024-06-03
页码11
关键词Biomass HMF BHMF Hydrogenation Biomass based monomers
ISSN号1011-372X
DOI10.1007/s10562-024-04717-8
通讯作者Wang, Haiyong(wanghy@ms.giec.ac.cn) ; Qiu, Songbai(qiusb@gdut.edu.cn)
英文摘要The development of biodegradable materials from biomass is a crucial strategy for leveraging biomass resources. A key component in this process is 2,5-bis(hydroxymethyl)furan (BHMF), a significant biomass-derived platform chemical. However, producing BHMF with high selectivity through the selective hydrogenation of 5-hydroxymethylfurfural, while avoiding the creation of unwanted byproducts, is a complex challenge. In our research, we have developed a novel catalyst featuring a magnetic core. This catalyst, which consists of platinum loaded onto a graphene-like shell, has been applied to the catalytic hydrogenation of HMF in an aqueous environment. Under the optimized conditions of 373 K, 3 MPa H2, and 1 h reaction time, a BHMF yield exceeding 99% was achieved. This method presents a promising and effective approach for the high-value conversion of biomass waste into polymer materials and pharmaceutical chemicals.
WOS关键词TRANSFORMATION ; CHEMICALS ; LIGNIN ; CARBON ; 2,5-DIHYDROXYMETHYLFURAN ; 2,5-DIFORMYLFURAN ; ESTERIFICATION ; CONVERSION ; REDUCTION ; POLYMERS
资助项目the Science and Technology Plan Project of Zhaoqing City[52006225] ; National Natural Science Foundation of China ; Youth Innovation Promotion Association, CAS[2021GDKLPRB05] ; Guang-dong Provincial Key Laboratory of Plant Resources Biorefinery[2022040302004] ; Science and Technology Plan Project of Zhaoqing City
WOS研究方向Chemistry
语种英语
WOS记录号WOS:001237085800003
出版者SPRINGER
资助机构the Science and Technology Plan Project of Zhaoqing City ; National Natural Science Foundation of China ; Youth Innovation Promotion Association, CAS ; Guang-dong Provincial Key Laboratory of Plant Resources Biorefinery ; Science and Technology Plan Project of Zhaoqing City
源URL[http://ir.giec.ac.cn/handle/344007/41943]  
专题中国科学院广州能源研究所
通讯作者Wang, Haiyong; Qiu, Songbai
作者单位1.Zhaoqing Univ, Sch Environm & Chem Engn, Zhaoqing 526061, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
3.Xinxiang Med Coll, Affiliated Hosp 3, Xinxiang 453200, Peoples R China
4.Guangdong Univ Technol, Sch Chem Engn & Light Ind, Guangzhou 510006, Peoples R China
推荐引用方式
GB/T 7714
Xu, Xian,Lan, Ling,Xu, Jiangong,et al. Selective Hydrogenation of 5-Hydroxymethylfurfural to 2,5-bis(hydroxymethyl)furan by Pt/Ni@C Catalyst[J]. CATALYSIS LETTERS,2024:11.
APA Xu, Xian.,Lan, Ling.,Xu, Jiangong.,Liang, Zheng.,Tan, Jin.,...&Qiu, Songbai.(2024).Selective Hydrogenation of 5-Hydroxymethylfurfural to 2,5-bis(hydroxymethyl)furan by Pt/Ni@C Catalyst.CATALYSIS LETTERS,11.
MLA Xu, Xian,et al."Selective Hydrogenation of 5-Hydroxymethylfurfural to 2,5-bis(hydroxymethyl)furan by Pt/Ni@C Catalyst".CATALYSIS LETTERS (2024):11.

入库方式: OAI收割

来源:广州能源研究所

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