Phase Transition Characteristics of Hydrate Formation Process in Microscale Pores
文献类型：期刊论文
| 作者 | Deng, Yu2,3,4; Kou, Xuan2,3; Li, Xiao-Sen2,3,4; Xu, Rui1,2,3; Chen, Zhao-Yang2,3,4; Wang, Yi2,3,4 |
| 刊名 | ENERGY & FUELS
 |
| 出版日期 | 2024-06-03 |
| 卷号 | 38期号:12页码:10914-10925 |
| ISSN号 | 0887-0624 |
| DOI | 10.1021/acs.energyfuels.4c01535 |
| 通讯作者 | Li, Xiao-Sen(lixs@ms.giec.ac.cn) ; Wang, Yi(wangyi@ms.giec.ac.cn) |
| 英文摘要 | Gas hydrates are ubiquitous in nature, with their formation within microscale pores involving intricate physical and chemical process. Recent advancements in visualization methods have propelled further investigations into the formation mechanisms of gas hydrates. The exploration of characteristics pertaining to the hydrate formation process through visual data has emerged as a prominent research avenue. However, it is still difficult to directly point out the relationship between the visual phenomenon and mechanism with a systematic approach. This article focuses on discerning significant temporal changes and categorizes phase transition features of microscale pore hydrate formation into two distinct yet conceptually clear domains: distribution probability and phase transition probability. Then, a statistical discussion of these probabilities has been proposed. Distribution probability elucidates the structural performance and physical attributes of hydrates at the microscale, while phase transition probability offers insights into visualizing kinetic parameters of hydrate reactions, which are conventionally challenging to gauge using traditional sensors. These probabilities linked visual information to physical information. It enabled the quantitative statistical evaluation of various factors during the phase transition process of hydrates, moving beyond a mere visual qualitative analysis. In essence, this innovative methodology furnishes hitherto unexplored concepts and a systematic framework for investigating microscale interface reactions and illuminating their internal mechanisms and evolutionary principles. |
| WOS关键词 | GAS HYDRATE |
| 资助项目 | Special Project for Marine Economy Development of Guangdong Province[52122602] ; Special Project for Marine Economy Development of Guangdong Province[52127815] ; Special Project for Marine Economy Development of Guangdong Province[52306286] ; National Natural Science Foundation of China[2019B030302004] ; National Natural Science Foundation of China[2020B0301030003] ; Fundamental Research & Applied Fundamental Research Major Project of Guangdong Province[2022M723160] ; China Postdoctoral Science Foundation[2019BT02L278] ; Guangdong Special Support Program Local Innovation and Entrepreneurship Team Project[[2022]43] ; Guangdong Special Support Program Local Innovation and Entrepreneurship Team Project[[2022]45] ; Special Project for Marine Economy Development of Guangdong Province |
| WOS研究方向 | Energy & Fuels ; Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:001239418700001 |
| 出版者 | AMER CHEMICAL SOC |
| 资助机构 | Special Project for Marine Economy Development of Guangdong Province ; National Natural Science Foundation of China ; Fundamental Research & Applied Fundamental Research Major Project of Guangdong Province ; China Postdoctoral Science Foundation ; Guangdong Special Support Program Local Innovation and Entrepreneurship Team Project ; Special Project for Marine Economy Development of Guangdong Province |
| 源URL | [http://ir.giec.ac.cn/handle/344007/42018]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Li, Xiao-Sen; Wang, Yi |
| 作者单位 | 1.Univ Chinese Acad Sci, Beijing 100083, Peoples R China 2.Chinese Acad Sci, Key Lab Gas Hydrate, Guangzhou 510640, Peoples R China 3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 4.Univ Sci & Technol China, Sch Energy Sci & Engn, Hefei 230026, Anhui, Peoples R China |
| 推荐引用方式 GB/T 7714 | Deng, Yu,Kou, Xuan,Li, Xiao-Sen,et al. Phase Transition Characteristics of Hydrate Formation Process in Microscale Pores[J]. ENERGY & FUELS,2024,38(12):10914-10925. |
| APA | Deng, Yu,Kou, Xuan,Li, Xiao-Sen,Xu, Rui,Chen, Zhao-Yang,&Wang, Yi.(2024).Phase Transition Characteristics of Hydrate Formation Process in Microscale Pores.ENERGY & FUELS,38(12),10914-10925. |
| MLA | Deng, Yu,et al."Phase Transition Characteristics of Hydrate Formation Process in Microscale Pores".ENERGY & FUELS 38.12(2024):10914-10925. |
入库方式： OAI收割
来源：广州能源研究所
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