Wood-Structured Nanomaterials as Highly Efficient, Self-Standing Electrocatalysts for Water Splitting
文献类型：期刊论文
| 作者 | Huang, Jianlin1; Shi, Zhikai1; Mao, Chengwei1; Yang, Gaixiu2; Chen, Yan1 |
| 刊名 | SMALL
 |
| 出版日期 | 2024-06-04 |
| 页码 | 22 |
| 关键词 | hierarchically porous structures hydrogen evolution reactions oxygen evolution reactions self-standing electrocatalysts wood-structured electrocatalysts |
| ISSN号 | 1613-6810 |
| DOI | 10.1002/smll.202402511 |
| 通讯作者 | Huang, Jianlin(jianlinhuang@scut.edu.cn) ; Yang, Gaixiu(yanggx@ms.giec.ac.cn) ; Chen, Yan(escheny@scut.edu.cn) |
| 英文摘要 | Electrocatalytic water splitting (EWS) driven by renewable energy is widely considered an environmentally friendly and sustainable approach for generating hydrogen (H-2), an ideal energy carrier for the future. However, the efficiency and economic viability of large-scale water electrolysis depend on electrocatalysts that can efficiently accelerate the electrochemical reactions taking place at the two electrodes. Wood-derived nanomaterials are well-suited for serving as EWS catalysts because of their hierarchically porous structure with high surface area and low tortuosity, compositional tunability, cost-effectiveness, and self-standing integral electrode configuration. Here, recent advancements in the design and synthesis of wood-structured nanomaterials serving as advanced electrocatalysts for water splitting are summarized. First, the design principles and corresponding strategies toward highly effective wood-structured electrocatalysts (WSECs) are emphasized. Then, a comprehensive overview of current findings on WSECs, encompassing diverse structural designs and functionalities such as supported-metal nanoparticles (NPs), single-atom catalysts (SACs), metal compounds, and heterostructured electrocatalysts based on engineered wood hosts are presented. Subsequently, the application of these WSECs in various aspects of water splitting, including the hydrogen evolution reaction (HER), oxygen evolution reaction (OER), overall water splitting (OWS), and hybrid water electrolysis (HWE) are explored. Finally, the prospects, challenges, and opportunities associated with the broad application of WSECs are briefly discussed. This review aims to provide a comprehensive understanding of the ongoing developments in water-splitting catalysts, along with outlining design principles for the future development of WSECs. |
| WOS关键词 | EVOLUTION REACTION ; ENERGY-CONVERSION ; OXYGEN REDUCTION ; HYDROGEN ; NANOPARTICLES ; CARBON ; MEMBRANE ; ELECTROOXIDATION ; CELLULOSE ; ELECTRODE |
| 资助项目 | Guangzhou Municipal Science and Technology Project[22076049] ; Guangzhou Municipal Science and Technology Project[52176214] ; National Natural Science Foundation of China[2024YFE0101500] ; National Key Research and Development Program of China[2024A1515010333] ; Guangdong Basic and Applied Basic Research Foundation[202201010063] ; Guangzhou Science and Technology Program[2020345] ; Youth Innovation Promotion Association CAS |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| 语种 | 英语 |
| WOS记录号 | WOS:001239099400001 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 资助机构 | Guangzhou Municipal Science and Technology Project ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; Guangdong Basic and Applied Basic Research Foundation ; Guangzhou Science and Technology Program ; Youth Innovation Promotion Association CAS |
| 源URL | [http://ir.giec.ac.cn/handle/344007/42100]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Huang, Jianlin; Yang, Gaixiu; Chen, Yan |
| 作者单位 | 1.South China Univ Technol, Sch Environm & Energy, Guangdong Prov Key Lab Solid Wastes Pollut Control, Guangzhou 510006, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy Guangdong Prov Key La, Guangzhou 510640, Peoples R China |
| 推荐引用方式 GB/T 7714 | Huang, Jianlin,Shi, Zhikai,Mao, Chengwei,et al. Wood-Structured Nanomaterials as Highly Efficient, Self-Standing Electrocatalysts for Water Splitting[J]. SMALL,2024:22. |
| APA | Huang, Jianlin,Shi, Zhikai,Mao, Chengwei,Yang, Gaixiu,&Chen, Yan.(2024).Wood-Structured Nanomaterials as Highly Efficient, Self-Standing Electrocatalysts for Water Splitting.SMALL,22. |
| MLA | Huang, Jianlin,et al."Wood-Structured Nanomaterials as Highly Efficient, Self-Standing Electrocatalysts for Water Splitting".SMALL (2024):22. |
入库方式： OAI收割
来源：广州能源研究所
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