Preparation of carbon materials by vapor deposition with Fe3+-Modified nickel foam from biomass pyrolysis gas
文献类型：期刊论文
| 作者 | Lan, Weijuan2; Zhou, Yunlong2; Liu, Jiaxin2; Wang, Yingxian2; Jin, Xin2; Yin, Dongxue2; Ji, Jiangtao2; Yang, Gaixiu1; Zhang, Huan3 |
| 刊名 | JOURNAL OF THE ENERGY INSTITUTE
 |
| 出版日期 | 2024-10-01 |
| 卷号 | 116页码:7 |
| 关键词 | Fe 3+-modified nickel foam Biomass Pyrolysis gas Chemical vapor deposition Carbon materials |
| ISSN号 | 1743-9671 |
| DOI | 10.1016/j.joei.2024.101756 |
| 通讯作者 | Lan, Weijuan(lwj@haust.edu.cn) ; Jin, Xin(jx.771@haust.edu.cn) |
| 英文摘要 | Biomass carbon materials have attracted attention in various fields due to their excellent properties. In this study, CH4 derived from biomass pyrolysis was utilized as a carbon source gas to synthesize carbon materials by chemical vapor deposition (CVD) in a two-stage reactor with purification system, with Fe3+-loaded nickel foam as the substrate under an argon atmosphere, using a self-designed experimental platform. The reaction process was optimized by examining the effects of the catalyst type, reaction temperature, reaction time, and gas flow rate on the structure and morphology of the carbon materials. The optimal preparation condition was to use FeCl3 ethanol solution as catalyst, with CH4 flow rate of 50 ml/min at 1000 degrees C for 25 min. The high quality carbon materials with uniform diameters (250-500 nm) were obtained on nickel foam substrate. The carbon materials obtained under optimal conditions were characterized and analyzed to investigate their excellent properties. Surface morphology and structure of as-formed carbon materials were characterized by SEM. The analysis of the XRD spectra and the Raman spectroscopy showed that the graphite diffraction peak (002) at 26.6 degrees, the calculated intensity ratios for ID/IG and I2D/IG were 0.257 and 0.545, respectively, indicated high degree of graphitization and purity of the carbon materials. Furthermore, the growth mechanism of carbon materials on the nickel foam substrate was discussed. |
| WOS关键词 | NANOTUBES ; NANOMATERIALS |
| 资助项目 | Key R & D Projects in Henan Province[241111321700] ; Major Science and Technology Projects in Henan Province[231100110200] |
| WOS研究方向 | Energy & Fuels |
| 语种 | 英语 |
| WOS记录号 | WOS:001276872500001 |
| 出版者 | ELSEVIER SCI LTD |
| 资助机构 | Key R & D Projects in Henan Province ; Major Science and Technology Projects in Henan Province |
| 源URL | [http://ir.giec.ac.cn/handle/344007/42468]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Lan, Weijuan; Jin, Xin |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510610, Peoples R China 2.Henan Univ Sci & Technol, Sch Agr Equipment Engn, Luoyang 471003, Peoples R China 3.Henan Agr Univ, Key Lab New Mat & Facil Rural Renewable Energy MOA, Zhengzhou 450002, Peoples R China |
| 推荐引用方式 GB/T 7714 | Lan, Weijuan,Zhou, Yunlong,Liu, Jiaxin,et al. Preparation of carbon materials by vapor deposition with Fe3+-Modified nickel foam from biomass pyrolysis gas[J]. JOURNAL OF THE ENERGY INSTITUTE,2024,116:7. |
| APA | Lan, Weijuan.,Zhou, Yunlong.,Liu, Jiaxin.,Wang, Yingxian.,Jin, Xin.,...&Zhang, Huan.(2024).Preparation of carbon materials by vapor deposition with Fe3+-Modified nickel foam from biomass pyrolysis gas.JOURNAL OF THE ENERGY INSTITUTE,116,7. |
| MLA | Lan, Weijuan,et al."Preparation of carbon materials by vapor deposition with Fe3+-Modified nickel foam from biomass pyrolysis gas".JOURNAL OF THE ENERGY INSTITUTE 116(2024):7. |
入库方式： OAI收割
来源：广州能源研究所
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