Scalable synthesis of Co2C-covered NiTe (Co2C-NiTe) nanosheets as an efficient electrocatalyst for HER & OER in an alkaline medium
文献类型：期刊论文
| 作者 | Munawar, Tauseef2; Bashir, Ambreen3; El-Marghany, Adel4; Shen, Lisha2; Tu, Zhiming2; Fatima, Saman3; Abid, Abdul Ghafoor1; Khan, Shoukat Alim5; Koc, Muammer5; Yan, Chang-Feng2 |
| 刊名 | FUEL
 |
| 出版日期 | 2024-11-01 |
| 卷号 | 375页码:13 |
| 关键词 | Interface engineering Electronic interaction Hydrogen evolution Oxygen evolution Alkaline water splitting Co2C-NiTe |
| ISSN号 | 0016-2361 |
| DOI | 10.1016/j.fuel.2024.132445 |
| 通讯作者 | Yan, Chang-Feng(yancf@ms.giec.ac.cn) ; Iqbal, Faisal(faisal.iqbal@iub.edu.pk) |
| 英文摘要 | To tackle global carbon conditions, renewable energy-powered electrochemical water splitting is a promising energy conversion device that can enhance the sustainable hydrogen output of the next generation. Regarding large-scale water splitting, novel non-noble metal-based heterostructures focus on constructing highly efficient electrocatalysts with unique interfaces toward hydrogen and oxygen evolution reactions. In this work, to facilitate the limited number of defects in the pure Co2C and NiTe electrocatalysts, we report that NiTe nanoflakes are coupled with a dispersed nanosheet network of the Co2C to develop a Co2C-NiTe composite by interface engineering strategy using a hydrothermal approach. XRD, IV, BET, TEM, XPS, and EDX mapping technologies investigated the 3D structure of as-grown Co2C-NiTe/SS. Electrochemical test results revealed that our bestperforming electrocatalyst delivers a 10 mAcm-2 with low overpotentials of 279 mV and 227 mV for oxidation and reduction reactions, respectively. Remarkably, this catalyst achieves good stability, reaching up to 90 h in one mol alkaline medium. We showed that this excellent activity of Co2C-NiTe is primarily due to the abundant interfacial area and stable anchoring sites, which improve the adsorption-desorption energy for hydroxide/oxyhydroxide species and thereby provide a fast electron transfer rate for OER/HER. In addition, a synergistic effect of Co2C with NiTe presents high electrical conductivity over counterpart electrocatalysts. |
| WOS关键词 | CARBON-PASTE ELECTRODE ; NANOPARTICLES EXPERIMENTAL-DESIGN ; HIGHLY EFFICIENT ; HETEROJUNCTION ; OXIDATION ; NANORODS |
| 资助项目 | King Saud University, Riyadh, Saudi Arabia[RSPD2024R667] |
| WOS研究方向 | Energy & Fuels ; Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:001279342900001 |
| 出版者 | ELSEVIER SCI LTD |
| 资助机构 | King Saud University, Riyadh, Saudi Arabia |
| 源URL | [http://ir.giec.ac.cn/handle/344007/42483]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Yan, Chang-Feng; Iqbal, Faisal |
| 作者单位 | 1.Chinese Acad Sci, Fujian Inst Res Struct Matter, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Energy Convers, 2,Nengyuan Rd, Guangzhou 510640, Peoples R China 3.Islamia Univ Bahawalpur, Inst Phys, Bahawalpur 63100, Pakistan 4.King Saud Univ, Coll Sci, Dept Chem, POB 2455, Riyadh 11451, Saudi Arabia 5.Hamad Bin Khalifa Univ, Qatar Fdn, Coll Sci & Engn, Div Sustainable Dev, Doha, Qatar |
| 推荐引用方式 GB/T 7714 | Munawar, Tauseef,Bashir, Ambreen,El-Marghany, Adel,et al. Scalable synthesis of Co2C-covered NiTe (Co2C-NiTe) nanosheets as an efficient electrocatalyst for HER & OER in an alkaline medium[J]. FUEL,2024,375:13. |
| APA | Munawar, Tauseef.,Bashir, Ambreen.,El-Marghany, Adel.,Shen, Lisha.,Tu, Zhiming.,...&Iqbal, Faisal.(2024).Scalable synthesis of Co2C-covered NiTe (Co2C-NiTe) nanosheets as an efficient electrocatalyst for HER & OER in an alkaline medium.FUEL,375,13. |
| MLA | Munawar, Tauseef,et al."Scalable synthesis of Co2C-covered NiTe (Co2C-NiTe) nanosheets as an efficient electrocatalyst for HER & OER in an alkaline medium".FUEL 375(2024):13. |
入库方式： OAI收割
来源：广州能源研究所
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