Prioritizing pollution sources and targeted potentially toxic elements in soils using a probabilistic source-specific eco-health risk assessment from micro and macro perspectives
文献类型：期刊论文
| 作者 | Guo, Guanghui1,2; Chen, Shiqi1,2; Zhang, Jinlong1,2; Lei, Mei1,2 |
| 刊名 | JOURNAL OF HAZARDOUS MATERIALS
 |
| 出版日期 | 2025-10-15 |
| 卷号 | 498页码:139909 |
| 关键词 | Soil potentially toxic elements Eco-health risk SEM-EDS Geo-detector model Monte Carlo simulation |
| ISSN号 | 0304-3894 |
| DOI | 10.1016/j.jhazmat.2025.139909 |
| 产权排序 | 1 |
| 文献子类 | Article |
| 英文摘要 | Soil potentially toxic elements (PTEs) pose significant ecological and health risks in mining areas with multiple pollution sources. However, accurate identification of priority pollution sources and PTEs remained unclear. To address this gap, this study developed an comprehensive framework integrating positive matrix factorization (PMF), geo-detector model (GDM), scanning electron microscopy and energy-dispersive spectroscopy (SEM-EDS) with probabilistic eco-health risk assessment. PMF model assisted with SEM-EDS and GDM revealed four potential sources: Cr (89.27 %) and Ni (88.34 %) were predominantly contributed by electroplating activities; As (86.26 %) was primarily attributed to gold leaching activities; Pb (84.60 %), Cd (65.14 %), and Zn (64.05 %) mainly originated from Pb/Zn smelting activities; while Cu (74.02 %) principally came from copper mining activities. Regarding ecological risk, Pb/Zn smelting accounting for 53.09 % of total risk was identified as the highest contributor, primarily driven by Cd (88.05 %) due to its high toxicity. While non-carcinogenic risks were acceptable for all population groups, carcinogenic risks reached cautionary level. Gold leaching activities, strongly linked to As, constituted the largest contributor to carcinogenic risks (children: 47.38 %; adult females: 49.45 %; adult males: 48.89 %). These findings enhance the accuracy of source-specific eco-health risk quanti-fication for soil PTEs, providing actionable insights for optimized risk management under resource constraints. |
| URL标识 | 查看原文 |
| WOS关键词 | UNCERTAINTY ; EXPOSURE ; METALS |
| WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:001583113300003 |
| 出版者 | ELSEVIER |
| 源URL | [http://ir.igsnrr.ac.cn/handle/311030/217511]  |
| 专题 | 资源利用与环境修复重点实验室_外文论文 |
| 通讯作者 | Guo, Guanghui |
| 作者单位 | 1.Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Beijing 100101, Peoples R China; 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Guo, Guanghui,Chen, Shiqi,Zhang, Jinlong,et al. Prioritizing pollution sources and targeted potentially toxic elements in soils using a probabilistic source-specific eco-health risk assessment from micro and macro perspectives[J]. JOURNAL OF HAZARDOUS MATERIALS,2025,498:139909. |
| APA | Guo, Guanghui,Chen, Shiqi,Zhang, Jinlong,&Lei, Mei.(2025).Prioritizing pollution sources and targeted potentially toxic elements in soils using a probabilistic source-specific eco-health risk assessment from micro and macro perspectives.JOURNAL OF HAZARDOUS MATERIALS,498,139909. |
| MLA | Guo, Guanghui,et al."Prioritizing pollution sources and targeted potentially toxic elements in soils using a probabilistic source-specific eco-health risk assessment from micro and macro perspectives".JOURNAL OF HAZARDOUS MATERIALS 498(2025):139909. |
入库方式： OAI收割
来源：地理科学与资源研究所
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