Novel Fenton-like degradation via generation of hydrogen peroxide using CoAl-LDH/porous g-C3N4 catalyst
文献类型：期刊论文
| 作者 | Qi, Lanyu1; Ma, Guofeng1; Kou, Ronghui1; Wang, Ziyao1; Zhang, Hongling2; Yang, Yanhong3 |
| 刊名 | JOURNAL OF WATER PROCESS ENGINEERING
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| 出版日期 | 2025-02-01 |
| 卷号 | 70页码:8 |
| 关键词 | CoAl-LDH Fenton-like Dye degradation |
| ISSN号 | 2214-7144 |
| DOI | 10.1016/j.jwpe.2025.107018 |
| 通讯作者 | Ma, Guofeng(guofma@163.com) |
| 英文摘要 | The Fenton-like process is a highly efficient and widely applied advanced oxidation technology for degrading organic pollutants under dark conditions. However, its development is limited by low H2O2 utilization, incomplete mineralization, and limited optimal pH range. We developed a CoAl-LDH/porous g-C3N4 catalyst via high-temperature thermal polymerization with NH4HCO3 as a dynamic gas template and urea as a precursor. The reaction rate constant of CoAl-LDH/porous g-C3N4-H2O2 system for degradation of Rhodamine B is 0.0199 min-1, which is about 1.58 times that of the CoAl-LDH-H2O2 system. Moreover, the catalyst sustained performance over four cycles and maintained high activity in degrading three different substrates. The high catalytic activity is attributed to the rich porous structure of g-C3N4, the presence of abundant active sites, and the synergistic interaction between the CoAl-LDH and g-C3N4, which promotes the generation of center dot OH, 1O2, center dot O2-, facilitating pollutant degradation. This study highlights the potential of this CoAl-LDH/porous g-C3N4-based Fenton-like system for applications in dye wastewater treatment. |
| 资助项目 | Innovative Talents Program of Colleges and Universities in Liaoning Province[2020-42] ; Shenyang Science and Technology Project[20-202-1-12] ; Shenyang Science and Technology Project[23-407-3-11] ; Shenyang Science and Technology Innovation Talent Project[RC210321] |
| WOS研究方向 | Engineering ; Water Resources |
| 语种 | 英语 |
| WOS记录号 | WOS:001402853900001 |
| 出版者 | ELSEVIER |
| 资助机构 | Innovative Talents Program of Colleges and Universities in Liaoning Province ; Shenyang Science and Technology Project ; Shenyang Science and Technology Innovation Talent Project |
| 源URL |  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Ma, Guofeng |
| 作者单位 | 1.Shenyang Univ, Shenyang Key Lab Microarc Oxidat Technol & Applica, Shenyang 110044, Peoples R China 2.Shenyang Univ, Key Lab Ecoremediat Reg Contaminated Environm, Minist Educ, Shenyang 110044, Peoples R China 3.Chinese Acad Sci, Shi Changxu Innovat Ctr Adv Mat, Inst Met Res, Shenyang 110016, Liaoning, Peoples R China |
| 推荐引用方式 GB/T 7714 | Qi, Lanyu,Ma, Guofeng,Kou, Ronghui,et al. Novel Fenton-like degradation via generation of hydrogen peroxide using CoAl-LDH/porous g-C3N4 catalyst[J]. JOURNAL OF WATER PROCESS ENGINEERING,2025,70:8. |
| APA | Qi, Lanyu,Ma, Guofeng,Kou, Ronghui,Wang, Ziyao,Zhang, Hongling,&Yang, Yanhong.(2025).Novel Fenton-like degradation via generation of hydrogen peroxide using CoAl-LDH/porous g-C3N4 catalyst.JOURNAL OF WATER PROCESS ENGINEERING,70,8. |
| MLA | Qi, Lanyu,et al."Novel Fenton-like degradation via generation of hydrogen peroxide using CoAl-LDH/porous g-C3N4 catalyst".JOURNAL OF WATER PROCESS ENGINEERING 70(2025):8. |
入库方式： OAI收割
来源：金属研究所
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