Insights on Fabrication Strategies and Energy Storage Mechanisms of Transition Metal Dichalcogenides Cathodes for Aqueous Zn-Based Batteries
文献类型：期刊论文
| 作者 | Li, Shengwei1; Das, Pratteek1; Wang, Xiao1; Li, Chenyang1; Wu, Zhong-Shuai1; Cheng, Hui-Ming2,3,4 |
| 刊名 | SMALL
 |
| 出版日期 | 2025-01-24 |
| 页码 | 16 |
| 关键词 | aqueous Zn-based battery cathode fabrication strategy transition metal dichalcogenides |
| ISSN号 | 1613-6810 |
| DOI | 10.1002/smll.202410036 |
| 通讯作者 | Wu, Zhong-Shuai(wuzs@dicp.ac.cn) ; Cheng, Hui-Ming(hm.cheng@siat.ac.cn) |
| 英文摘要 | Aqueous zinc-based batteries (AZBs) are gaining widespread attention owing to their intrinsic safety, relatively low electrode potential, and high theoretical capacity. Transition metal dichalcogenides (TMDs) have convenient 2D ion diffusion channels, so they have been identified as promising host materials for AZBs, but face several key challenges such as the narrow interlayer spacing and the lack of in-deep understanding energy storage mechanisms. This review presents a comprehensive summary and discussion of the intrinsic structure, charge storage mechanisms, and key fabrication strategies of TMD-based cathodes for AZBs. Firstly, the structural features including phase types and electrical properties of TMDs are underscored. Then, the charge storage mechanisms and activation principles in TMDs are elaborated along with the discussions about their influence on electrochemical performance. Afterward, specific attention is focused on the fabrication strategies of high-performance TMD cathodes, including interlayer expansion, defect creation, phase transition, and heteroatom doping. Finally, the key challenges are considered and potential effective strategies are proposed to design high-performance aqueous Zn-TMDs batteries. |
| 资助项目 | National Natural Science Foundation of China ; Basic Science Center Project of the National Natural Science Foundation of China[52188101] ; China National Postdoctoral Program for Innovative Talents[BX20240361] ; Natural Science Foundation of Liaoning Province[2024-BSBA-31] ; DICP[DICP I202471] ; State Key Laboratory of Catalysis[2024SKL-A-001] ; Energy Revolution S&T Program of Yulin Innovation Institute of Clean Energy[E412010508] ; Energy Revolution S&T Program of Yulin Innovation Institute of Clean Energy[E411050316] ; [22125903] ; [22439003] ; [22309176] ; [22209173] ; [22409196] ; [W2433043] |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| 语种 | 英语 |
| WOS记录号 | WOS:001403213800001 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 资助机构 | National Natural Science Foundation of China ; Basic Science Center Project of the National Natural Science Foundation of China ; China National Postdoctoral Program for Innovative Talents ; Natural Science Foundation of Liaoning Province ; DICP ; State Key Laboratory of Catalysis ; Energy Revolution S&T Program of Yulin Innovation Institute of Clean Energy |
| 源URL |  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Wu, Zhong-Shuai; Cheng, Hui-Ming |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China 2.Chinese Acad Sci, Shenzhen Inst Adv Technol, Shenzhen Key Lab Energy Mat Carbon Neutral, Shenzhen 518055, Peoples R China 3.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 4.Shenzhen Univ Adv Technol, Fac Mat Sci & Energy Engn, Shenzhen 518055, Peoples R China |
| 推荐引用方式 GB/T 7714 | Li, Shengwei,Das, Pratteek,Wang, Xiao,et al. Insights on Fabrication Strategies and Energy Storage Mechanisms of Transition Metal Dichalcogenides Cathodes for Aqueous Zn-Based Batteries[J]. SMALL,2025:16. |
| APA | Li, Shengwei,Das, Pratteek,Wang, Xiao,Li, Chenyang,Wu, Zhong-Shuai,&Cheng, Hui-Ming.(2025).Insights on Fabrication Strategies and Energy Storage Mechanisms of Transition Metal Dichalcogenides Cathodes for Aqueous Zn-Based Batteries.SMALL,16. |
| MLA | Li, Shengwei,et al."Insights on Fabrication Strategies and Energy Storage Mechanisms of Transition Metal Dichalcogenides Cathodes for Aqueous Zn-Based Batteries".SMALL (2025):16. |
入库方式： OAI收割
来源：金属研究所
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