An efficient CuZr-based metallic glasses electrode material for electrocatalytic degradation of azo dyes
文献类型：期刊论文
| 作者 | Deng, Zhiwang1,2; Zhao, Bowen2; Li, Songtao2; Li, Zhengkun2,3; Zhang, Shiming4; Zhang, Kewei1; Zhu, Zhengwang2,3 |
| 刊名 | JOURNAL OF ENVIRONMENTAL SCIENCES
 |
| 出版日期 | 2024-02-01 |
| 卷号 | 136页码:537-546 |
| 关键词 | Metallic glasses Azo dyes Electrocatalytic Degradation Oxidized copper |
| ISSN号 | 1001-0742 |
| DOI | 10.1016/j.jes.2022.09.0101001-0742 |
| 通讯作者 | Zhang, Kewei(drzkw@126.com) ; Zhu, Zhengwang(zwzhu@imr.ac.cn) |
| 英文摘要 | Metallic glasses have received a lot of attention on wastewater treatment due to their unique atomic structure, and the use of metallic glasses as electrodes has produced unexpected electrocatalytic degradation effects for many pollutants through combining with electrochemical technology. However, it still is a formidable challenge to find a metallic glass electrode material with both efficient and clean for the catalytic degradation of pollutants. In this work, the Cu 55 Zr 45 metallic glassy ribbons are used as an electrode to degrade azo dyes and show the excellent degradation effect, which can reach 95.6% within 40 min. In the degradation process, almost no additives are produced and Cu 55 Zr 45 metallic glassy ribbons have excellent effects under different pH conditions. Meanwhile, it exhibits good stability for degradation efficiency during the 8 cycle degradation tests of the amorphous alloy electrode. When the copper nanoparticles are exposed on the surface of the ribbons, the oxidized copper obtained synergistically produce activated radicals is the primary degradation mechanism, where the auxiliary degradation mechanisms include electron transfer and the promotion of active chlorine. This research develops a new type of electrode material for wastewater treatment, and the economy and high efficiency of Cu 55 Zr 45 metallic glass endow it the expandable functional applications. (c) 2023 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V. |
| 资助项目 | National Natural Science Foundation of China[51801209] ; National Natural Science Foundation of China[52074257] ; Fund of Qingdao[19-9-2-1-wz] |
| WOS研究方向 | Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:001146147100001 |
| 出版者 | SCIENCE PRESS |
| 资助机构 | National Natural Science Foundation of China ; Fund of Qingdao |
| 源URL |  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Zhang, Kewei; Zhu, Zhengwang |
| 作者单位 | 1.Taiyuan Univ Sci & Technol, Sch Mat Sci & Engn, Taiyuan 030024, Peoples R China 2.Chinese Acad Sci, Inst Met Res, Shi Changxu Innovat Ctr Adv Mat, Shenyang 110016, Peoples R China 3.Chinese Acad Sci, Inst Met Res, Key Lab Nucl Mat & Safety Assessment, Shenyang 110016, Peoples R China 4.Qingdao Yunlu Adv Mat Technol Co Ltd, Qingdao 266232, Peoples R China |
| 推荐引用方式 GB/T 7714 | Deng, Zhiwang,Zhao, Bowen,Li, Songtao,et al. An efficient CuZr-based metallic glasses electrode material for electrocatalytic degradation of azo dyes[J]. JOURNAL OF ENVIRONMENTAL SCIENCES,2024,136:537-546. |
| APA | Deng, Zhiwang.,Zhao, Bowen.,Li, Songtao.,Li, Zhengkun.,Zhang, Shiming.,...&Zhu, Zhengwang.(2024).An efficient CuZr-based metallic glasses electrode material for electrocatalytic degradation of azo dyes.JOURNAL OF ENVIRONMENTAL SCIENCES,136,537-546. |
| MLA | Deng, Zhiwang,et al."An efficient CuZr-based metallic glasses electrode material for electrocatalytic degradation of azo dyes".JOURNAL OF ENVIRONMENTAL SCIENCES 136(2024):537-546. |
入库方式： OAI收割
来源：金属研究所
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