Ultrafast Graphene Oxide-Lignin Biopolymer Nanocomposite Membranes for Separation of Biomolecules, Dyes, and Salts
文献类型：期刊论文
| 作者 | Ali, Akbar1; Vohra, Muhammad Ismail2; Nadeem, Ahmed3; Al-Anzi, Bader S.8; Iqbal, Muzaffar4; Memon, Ayaz Ali5; Jatoi, Ashique Hussain6; Akhtar, Javeed7; Yang, Jun1; Thebo, Khalid Hussain7,9 |
| 刊名 | ACS APPLIED POLYMER MATERIALS
 |
| 出版日期 | 2024-04-10 |
| 页码 | 9 |
| 关键词 | graphene oxide lignin biopolymer separation membrane biomolecules |
| ISSN号 | 2637-6105 |
| DOI | 10.1021/acsapm.4c00285 |
| 通讯作者 | Al-Anzi, Bader S.(bader.alanzi@ku.edu.kw) ; Yang, Jun(jyang@ipe.ac.cn) ; Thebo, Khalid Hussain(khalidthebo@yahoo.com) |
| 英文摘要 | Graphene oxide offers a promising opportunity to fabricate highly efficient and pressure-endurable membranes in terms of water permeability while demonstrating a high level of solute rejection. However, achieving higher permeance with an excellent separation capability is still challenging. Herein, we report a class of graphene oxide-lignin biopolymer (GOLB) membranes for the first time prepared by functionalizing GO nanosheets with lignin biopolymer extracted from plant pulp. Lignin biopolymer is the most abundant, green, low-cost, and environmentally friendly material with a variety of oxygen functional groups. The as-prepared GOLB membranes have a unique laminated structure that provides an excellent rejection (>99%) for several organic dyes, proteins, and biomolecules with variable molecular weight and exhibits ultrawater permeance similar to 1300 L m(-2) h(-1) bar(-1), more than that of reported GO-based membranes. It is interesting that due to larger interlayer spacing, such membranes show less rejection (<10%) for salts, i.e., NaCl, MgCl2, Na2SO4, etc. Furthermore, these membranes are highly stable up to 37 days in an aqueous environment and 28 days in acidic and basic solutions compared to pristine GO-based membranes. |
| 资助项目 | King Saud University, Riyadh, Saudi Arabia[RSP2024R124] ; National Natural Science Foundation of China[22272179] ; National Natural Science Foundation of China[22075290] ; Beijing Natural Science Foundation[Z200012] ; State Key Laboratory of Multiphase Complex Systems, Institute of Process Engineering, Chinese Academy of Sciences[MPCS-2021-A-05] |
| WOS研究方向 | Materials Science ; Polymer Science |
| 语种 | 英语 |
| WOS记录号 | WOS:001201351800001 |
| 出版者 | AMER CHEMICAL SOC |
| 资助机构 | King Saud University, Riyadh, Saudi Arabia ; National Natural Science Foundation of China ; Beijing Natural Science Foundation ; State Key Laboratory of Multiphase Complex Systems, Institute of Process Engineering, Chinese Academy of Sciences |
| 源URL |  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Al-Anzi, Bader S.; Yang, Jun; Thebo, Khalid Hussain |
| 作者单位 | 1.Chinese Acad Sci, Inst Proc Engn IPE, State Key Lab Multiphase Complex Syst, 100F190, Beijing, Peoples R China 2.One Hlth Lab, Res & Dev Karachi, Karachi 76000, Pakistan 3.King Saud Univ, Coll Pharm, Dept Pharmacol & Toxicol, Riyadh 11451, Saudi Arabia 4.Univ Haripur, Fac Phys & Appl Sci, Dept Chem, Haripur 22620, Khyber Pakhtunk, Pakistan 5.Univ Sindh, Natl Ctr Excellence Analyt Chem, Jamshoro 76080, Pakistan 6.Shaheed Benazir Bhutto Univ, Dept Chem, Shaheed Benazirabad 67480, Pakistan 7.Chinese Acad Sci, Inst Met Res, Shenyang 110016, Peoples R China 8.Kuwait Univ, Dept Environm Sci, Safat 13060, Kuwait 9.Mirpur Univ Sci & Technol MUST, Dept Chem, Funct Nano Mat Lab, Mirpur 10250, Pakistan |
| 推荐引用方式 GB/T 7714 | Ali, Akbar,Vohra, Muhammad Ismail,Nadeem, Ahmed,et al. Ultrafast Graphene Oxide-Lignin Biopolymer Nanocomposite Membranes for Separation of Biomolecules, Dyes, and Salts[J]. ACS APPLIED POLYMER MATERIALS,2024:9. |
| APA | Ali, Akbar.,Vohra, Muhammad Ismail.,Nadeem, Ahmed.,Al-Anzi, Bader S..,Iqbal, Muzaffar.,...&Thebo, Khalid Hussain.(2024).Ultrafast Graphene Oxide-Lignin Biopolymer Nanocomposite Membranes for Separation of Biomolecules, Dyes, and Salts.ACS APPLIED POLYMER MATERIALS,9. |
| MLA | Ali, Akbar,et al."Ultrafast Graphene Oxide-Lignin Biopolymer Nanocomposite Membranes for Separation of Biomolecules, Dyes, and Salts".ACS APPLIED POLYMER MATERIALS (2024):9. |
入库方式： OAI收割
来源：金属研究所
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