Novel Alkane Dehydrogenation Routes via Tailored Catalysts
文献类型：期刊论文
| 作者 | Dai, Xueya1,2; Qi, Wei1,2 |
| 刊名 | CHEMCATCHEM
 |
| 出版日期 | 2024-05-02 |
| 页码 | 7 |
| 关键词 | alkane dehydrogenation reaction routes non-mental catalysts reaction mechanisms structure-function relations |
| ISSN号 | 1867-3880 |
| DOI | 10.1002/cctc.202400410 |
| 通讯作者 | Qi, Wei(wqi@imr.ac.cn) |
| 英文摘要 | Alkane dehydrogenation to alkene represents a promising alternative route for conventional petroleum cracking processes heavily reliant on fossil resources. This Concept outlines the latest advancements of novel alkane dehydrogenation routes that offer potential solutions to intrinsic problems existing in routine direct dehydrogenation or oxidative dehydrogenation reactions, including CO2 assisted alkane dehydrogenation, chemical looping alkane oxidative dehydrogenation, dual-path dehydrogenation and auto-accelerated multiple alkane dehydrogenation route. These novel reaction routes exhibit unique advantages in enhancing the activity, selectivity and stability of the alkane dehydrogenation reaction system. The rational design of novel catalysts and proper choice of the reaction condition that well-fitted these reaction routes is the key for achieving highly efficient and stable alkane dehydrogenation process. These present examples in this manuscript also highlight the importance of fundamental in-depth understandings on the mechanism and structure-function relations, which is the foundation for developing novel alkane dehydrogenation routes for practical applications. Novel alkane dehydrogenation routes, including CO2 assisted dehydrogenation, chemical looping oxidative dehydrogenation, dual-path dehydrogenation and auto-accelerated multiple alkane dehydrogenation routes, are highlighted in this Concept. Rational design of corresponding catalysts, proper choice of reaction conditions and the in depth understandings on the reaction mechanism and structure-function relations are summarized as the key in these reaction routes. image |
| 资助项目 | NSFC of China ; Natural Science Foundation of Liaoning Province of China[2020-YQ-02] ; Baowu Low Carbon Metallurgy Innovation Foudation[BWLCF202113] ; [22072163] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:001214528800001 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 资助机构 | NSFC of China ; Natural Science Foundation of Liaoning Province of China ; Baowu Low Carbon Metallurgy Innovation Foudation |
| 源URL |  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Qi, Wei |
| 作者单位 | 1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 2.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Peoples R China |
| 推荐引用方式 GB/T 7714 | Dai, Xueya,Qi, Wei. Novel Alkane Dehydrogenation Routes via Tailored Catalysts[J]. CHEMCATCHEM,2024:7. |
| APA | Dai, Xueya,&Qi, Wei.(2024).Novel Alkane Dehydrogenation Routes via Tailored Catalysts.CHEMCATCHEM,7. |
| MLA | Dai, Xueya,et al."Novel Alkane Dehydrogenation Routes via Tailored Catalysts".CHEMCATCHEM (2024):7. |
入库方式： OAI收割
来源：金属研究所
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