中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Amino Group-Driven Adsorption of Sodium p-Perfluorous Nonenoxybenzene Sulfonate in Water by the Modified Graphene Oxide

文献类型:期刊论文

作者Lu, Mengyuan1; Liu, Yang1; Zheng, Xinning2; Liu, Wenjuan3; Liu, Yang1; Bao, Jia1; Feng, Ao1; Bao, Yueyao1; Diao, Jiangyong5; Liu, Hongyang5
刊名TOXICS
出版日期2024-05-01
卷号12期号:5页码:14
关键词sodium p-perfluorinated nonenoxybenzene sulfonate (OBS) chitosan-modified amino-driven graphene oxide (CS-GO) removal adsorption mechanism electrostatic interaction
DOI10.3390/toxics12050343
通讯作者Liu, Yang(liuyang@sut.edu.cn) ; Bao, Jia(baojia@sut.edu.cn)
英文摘要Sodium p-perfluorous nonenoxybenzene sulfonate (OBS) is one of the key alternatives to perfluoroalkyl substances (PFASs). Its widespread tendency has increased extensive contamination in the aquatic environment. However, the present treatment technology for OBS exhibited insignificant adsorption capacity and long adsorption time. In this study, three proportions (1:5, 3:5, and 10:1) of chitosan-modified amino-driven graphene oxide (CS-GO) were innovated to strengthen the OBS adsorption capacity, compared with graphene oxide (GO) and graphene (GH). Through the characterization of SEM, BET, and FTIR, it was discovered that CS was synthetized on GO surfaces successfully with a low specific surface area. Subsequently, batch single influence factor studies on OBS removal from simulated wastewater were investigated. The optimum removal efficiency of OBS could be achieved up to 95.4% within 2 h when the adsorbent was selected as CS-GO (10:1), the dosage was 2 mg, and the pH was 3. The addition of inorganic ions could promote the adsorption efficiency of OBS. In addition, CS-GO presented the maximum adsorption energy due to additional functional groups of -NH3, and electrostatic interaction was the foremost motive for improving the adsorption efficiency of OBS. Moreover, OBS exhibited the fastest diffusion coefficient in the CS-GO-OBS solution, which is consistent with the fitting results of adsorption kinetics.
资助项目National Key R&D Program of China
WOS研究方向Environmental Sciences & Ecology ; Toxicology
语种英语
WOS记录号WOS:001231557500001
出版者MDPI
资助机构National Key R&D Program of China
源URL  
专题金属研究所_中国科学院金属研究所
通讯作者Liu, Yang; Bao, Jia
作者单位1.Shenyang Univ Technol, Sch Environm & Chem Engn, Shenyang 110870, Peoples R China
2.Shenyang Zhenxing Sewage Treatment Co Ltd, Shenyang 110143, Peoples R China
3.Dalian Xigang Dist Ctr Dis Control & Prevent, Dalian 116021, Peoples R China
4.Shenyang Hoper Grp Co Ltd, Shenyang 110112, Peoples R China
5.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
推荐引用方式
GB/T 7714
Lu, Mengyuan,Liu, Yang,Zheng, Xinning,et al. Amino Group-Driven Adsorption of Sodium p-Perfluorous Nonenoxybenzene Sulfonate in Water by the Modified Graphene Oxide[J]. TOXICS,2024,12(5):14.
APA Lu, Mengyuan.,Liu, Yang.,Zheng, Xinning.,Liu, Wenjuan.,Liu, Yang.,...&Liu, Hongyang.(2024).Amino Group-Driven Adsorption of Sodium p-Perfluorous Nonenoxybenzene Sulfonate in Water by the Modified Graphene Oxide.TOXICS,12(5),14.
MLA Lu, Mengyuan,et al."Amino Group-Driven Adsorption of Sodium p-Perfluorous Nonenoxybenzene Sulfonate in Water by the Modified Graphene Oxide".TOXICS 12.5(2024):14.

入库方式: OAI收割

来源:金属研究所

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