Amino Group-Driven Adsorption of Sodium p-Perfluorous Nonenoxybenzene Sulfonate in Water by the Modified Graphene Oxide
文献类型:期刊论文
| 作者 | Lu, Mengyuan1; Liu, Yang1; Zheng, Xinning2; Liu, Wenjuan3; Liu, Yang1; Bao, Jia1; Feng, Ao1; Bao, Yueyao1; Diao, Jiangyong5; Liu, Hongyang5 |
| 刊名 | TOXICS
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| 出版日期 | 2024-05-01 |
| 卷号 | 12期号:5页码:14 |
| 关键词 | sodium p-perfluorinated nonenoxybenzene sulfonate (OBS) chitosan-modified amino-driven graphene oxide (CS-GO) removal adsorption mechanism electrostatic interaction |
| DOI | 10.3390/toxics12050343 |
| 通讯作者 | Liu, Yang(liuyang@sut.edu.cn) ; Bao, Jia(baojia@sut.edu.cn) |
| 英文摘要 | Sodium p-perfluorous nonenoxybenzene sulfonate (OBS) is one of the key alternatives to perfluoroalkyl substances (PFASs). Its widespread tendency has increased extensive contamination in the aquatic environment. However, the present treatment technology for OBS exhibited insignificant adsorption capacity and long adsorption time. In this study, three proportions (1:5, 3:5, and 10:1) of chitosan-modified amino-driven graphene oxide (CS-GO) were innovated to strengthen the OBS adsorption capacity, compared with graphene oxide (GO) and graphene (GH). Through the characterization of SEM, BET, and FTIR, it was discovered that CS was synthetized on GO surfaces successfully with a low specific surface area. Subsequently, batch single influence factor studies on OBS removal from simulated wastewater were investigated. The optimum removal efficiency of OBS could be achieved up to 95.4% within 2 h when the adsorbent was selected as CS-GO (10:1), the dosage was 2 mg, and the pH was 3. The addition of inorganic ions could promote the adsorption efficiency of OBS. In addition, CS-GO presented the maximum adsorption energy due to additional functional groups of -NH3, and electrostatic interaction was the foremost motive for improving the adsorption efficiency of OBS. Moreover, OBS exhibited the fastest diffusion coefficient in the CS-GO-OBS solution, which is consistent with the fitting results of adsorption kinetics. |
| 资助项目 | National Key R&D Program of China |
| WOS研究方向 | Environmental Sciences & Ecology ; Toxicology |
| 语种 | 英语 |
| WOS记录号 | WOS:001231557500001 |
| 出版者 | MDPI |
| 资助机构 | National Key R&D Program of China |
| 源URL | ![]() |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Liu, Yang; Bao, Jia |
| 作者单位 | 1.Shenyang Univ Technol, Sch Environm & Chem Engn, Shenyang 110870, Peoples R China 2.Shenyang Zhenxing Sewage Treatment Co Ltd, Shenyang 110143, Peoples R China 3.Dalian Xigang Dist Ctr Dis Control & Prevent, Dalian 116021, Peoples R China 4.Shenyang Hoper Grp Co Ltd, Shenyang 110112, Peoples R China 5.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China |
| 推荐引用方式 GB/T 7714 | Lu, Mengyuan,Liu, Yang,Zheng, Xinning,et al. Amino Group-Driven Adsorption of Sodium p-Perfluorous Nonenoxybenzene Sulfonate in Water by the Modified Graphene Oxide[J]. TOXICS,2024,12(5):14. |
| APA | Lu, Mengyuan.,Liu, Yang.,Zheng, Xinning.,Liu, Wenjuan.,Liu, Yang.,...&Liu, Hongyang.(2024).Amino Group-Driven Adsorption of Sodium p-Perfluorous Nonenoxybenzene Sulfonate in Water by the Modified Graphene Oxide.TOXICS,12(5),14. |
| MLA | Lu, Mengyuan,et al."Amino Group-Driven Adsorption of Sodium p-Perfluorous Nonenoxybenzene Sulfonate in Water by the Modified Graphene Oxide".TOXICS 12.5(2024):14. |
入库方式: OAI收割
来源:金属研究所
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