In situ Preparation and Visible-light-driven Photocatalytic Degradation Performance of Nano 3C-SiC@Multilayer Graphene Oxide Heterostructure
文献类型：期刊论文
| 作者 | Yang, Xiaodan1; Guo, Ziqi1,2; Xu, Yichen1; Li, Ziliang3; Zhou, Yangtao1; Yang, Zhenming1; Zhou, Zishuai4; Gao, Yong1; Zhang, Jinsong1 |
| 刊名 | CHEMICAL RESEARCH IN CHINESE UNIVERSITIES
 |
| 出版日期 | 2024-05-25 |
| 页码 | 12 |
| 关键词 | Photocatalysis Multilayer graphene oxide Nano 3C-SiC Visible light degradation |
| ISSN号 | 1005-9040 |
| DOI | 10.1007/s40242-024-4076-7 |
| 通讯作者 | Yang, Xiaodan(xdyang@imr.ac.cn) ; Gao, Yong(ygao@imr.ac.cn) |
| 英文摘要 | Nano 3C-SiC@multilayer graphene oxide (NS@MGO) heterostructure was in situ prepared by carbothermal reduction of pyrolyzed precursor composed of highly dispersed cured phenolic resin and silicon dioxide derived from tetraethyl orthosilicate. The heterojunction interface, number of layers of MGO, and defect content in graphene are the three most important factors for promoting photocatalytic activity. Direct contact between 3C-SiC nanograins and MGO layers facilitates the photogenerated electrons to migrate across the heterojunction interface and avoid the formation of SiO2 nanolayers on the surface of SiC nanograins. The number of MGO layers is supposed to be less than ten instead of over-thick MGO. The concentrations of oxygenated components, considered the defect contents, decrease with the increase of sintering temperature for NS@MGO 0.175-T-150, and relative carbon content in the multilayer graphene increases. According to the heterostructures, properties, and photocatalytic reaction performance of the NS@MGO materials, the highest photocatalytic kinetic rate constant of 0.00891/min for NS@MGO 0.175-1500-150 shows that the significant enhancement in photocatalytic degradation activity under visible light (>420 nm) irradiation is ascribed to the advantageous synergistic effects between the nano 3C-SiC particles and the direct contact multilayer graphene oxide with appropriate layers and sufficient oxygen content of 3.51% (atomic fraction) in MGO. |
| 资助项目 | National Key Research and Development Program of China[2021YFB3801301] ; Shenyang National Laboratory for Materials Science (SYNL, China) Program for Youth Talent[L2022F39] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:001236308100001 |
| 出版者 | HIGHER EDUCATION PRESS |
| 资助机构 | National Key Research and Development Program of China ; Shenyang National Laboratory for Materials Science (SYNL, China) Program for Youth Talent |
| 源URL |  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Yang, Xiaodan; Gao, Yong |
| 作者单位 | 1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 2.Univ Sci & Technol China, Nano Sci & Technol Inst, Suzhou 215123, Peoples R China 3.Shenyang SCIENCREAT Chem Co Ltd, Shenyang 110144, Peoples R China 4.Northeastern Univ, Sch Mat Sci & Engn, Shenyang 110819, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yang, Xiaodan,Guo, Ziqi,Xu, Yichen,et al. In situ Preparation and Visible-light-driven Photocatalytic Degradation Performance of Nano 3C-SiC@Multilayer Graphene Oxide Heterostructure[J]. CHEMICAL RESEARCH IN CHINESE UNIVERSITIES,2024:12. |
| APA | Yang, Xiaodan.,Guo, Ziqi.,Xu, Yichen.,Li, Ziliang.,Zhou, Yangtao.,...&Zhang, Jinsong.(2024).In situ Preparation and Visible-light-driven Photocatalytic Degradation Performance of Nano 3C-SiC@Multilayer Graphene Oxide Heterostructure.CHEMICAL RESEARCH IN CHINESE UNIVERSITIES,12. |
| MLA | Yang, Xiaodan,et al."In situ Preparation and Visible-light-driven Photocatalytic Degradation Performance of Nano 3C-SiC@Multilayer Graphene Oxide Heterostructure".CHEMICAL RESEARCH IN CHINESE UNIVERSITIES (2024):12. |
入库方式： OAI收割
来源：金属研究所
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