Sub-millisecond lithiothermal synthesis of graphitic meso-microporous carbon
文献类型：期刊论文
| 作者 | Zhang, Huimin1; Qiu, Jingyi1; Pang, Jie2; Cao, Gaoping1; Zhang, Bingsen3; Wang, Li4; He, Xiangming4; Feng, Xuning4; Ma, Shizhou1; Zhang, Xinggao1 |
| 刊名 | NATURE COMMUNICATIONS
 |
| 出版日期 | 2024-04-25 |
| 卷号 | 15期号:1页码:9 |
| DOI | 10.1038/s41467-024-47916-y |
| 通讯作者 | Li, Feng(fli@imr.ac.cn) ; Zhang, Hao(dr.h.zhang@hotmail.com) |
| 英文摘要 | Porous carbons with concurrently high specific surface area and electronic conductivity are desirable by virtue of their desirable electron and ion transport ability, but conventional preparing methods suffer from either low yield or inferior quality carbons. Here we developed a lithiothermal approach to bottom-up synthesize highly meso-microporous graphitized carbon (MGC). The preparation can be finished in a few milliseconds by the self-propagating reaction between polytetrafluoroethylene powder and molten lithium (Li) metal, during which instant ultra-high temperature (>3000 K) was produced. This instantaneous carbon vaporization and condensation at ultra-high temperatures and in ultra-short duration enable the MGC to show a highly graphitized and continuously cross-coupled open pore structure. MGC displays superior electrochemical capacitor performance of exceptional power capability and ultralong-term cyclability. The processes used to make this carbon are readily scalable to industrial levels. |
| 资助项目 | Funders: The Natural Science Foundation of China Grant Reference Number (22075320 and 52202336y[22075320] ; Funders: The Natural Science Foundation of China Grant Reference Number (22075320 and 52202336y[52202336] ; Natural Science Foundation of China |
| WOS研究方向 | Science & Technology - Other Topics |
| 语种 | 英语 |
| WOS记录号 | WOS:001211008800021 |
| 出版者 | NATURE PORTFOLIO |
| 资助机构 | Funders: The Natural Science Foundation of China Grant Reference Number (22075320 and 52202336y ; Natural Science Foundation of China |
| 源URL |  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Li, Feng; Zhang, Hao |
| 作者单位 | 1.Res Inst Chem Def, Beijing Key Lab Adv Chem Energy Storage Technol &, Beijing, Peoples R China 2.Henan Univ, Sch Energy Sci & Technol, Zhengzhou, Peoples R China 3.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang, Peoples R China 4.Tsinghua Univ, Inst Nucl & New Energy Technol, Beijing, Peoples R China 5.Univ Cambridge, Dept Mat Sci & Met, Cambridge, England |
| 推荐引用方式 GB/T 7714 | Zhang, Huimin,Qiu, Jingyi,Pang, Jie,et al. Sub-millisecond lithiothermal synthesis of graphitic meso-microporous carbon[J]. NATURE COMMUNICATIONS,2024,15(1):9. |
| APA | Zhang, Huimin.,Qiu, Jingyi.,Pang, Jie.,Cao, Gaoping.,Zhang, Bingsen.,...&Zhang, Hao.(2024).Sub-millisecond lithiothermal synthesis of graphitic meso-microporous carbon.NATURE COMMUNICATIONS,15(1),9. |
| MLA | Zhang, Huimin,et al."Sub-millisecond lithiothermal synthesis of graphitic meso-microporous carbon".NATURE COMMUNICATIONS 15.1(2024):9. |
入库方式： OAI收割
来源：金属研究所
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