Intercalating Architecture for the Design of Charge Density Wave in Metallic MA2Z4 Materials
文献类型：期刊论文
| 作者 | Wang, Lei1,2; Wang, Shuaiyu1; Niu, Yuekun1; Liu, Xiuying1; Wu, Yapeng1; Zhang, Bing1; Liu, Zhifeng1; Li, Xiao-Ping1; Chen, Xing-Qiu3 |
| 刊名 | NANO LETTERS
 |
| 出版日期 | 2024-08-15 |
| 页码 | 7 |
| 关键词 | Charge Density Wave MA(2)Z(4) Materials Intercalating Architecture Approach Phase Diagram Mott Transition Star of David |
| ISSN号 | 1530-6984 |
| DOI | 10.1021/acs.nanolett.4c02998 |
| 通讯作者 | Wang, Lei(lwang@imu.edu.cn) ; Li, Xiao-Ping(xpli@imu.edu.cn) ; Chen, Xing-Qiu(xingqiu.chen@imr.ac.cn) |
| 英文摘要 | We present a novel approach to induce charge density waves (CDWs) in metallic MA(2)Z(4) materials, resembling the behavior observed in transition metal dichalcogenides (TMDCs). This method leverages the intercalating architecture to maintain the same crystal field and Fermi surface topologies. Our investigation reveals that CDW instability in these materials arises from electron-phonon coupling (EPC) between the d band and longitudinal acoustic (LA) phonons, mirroring TMDC's behavior. By combining alpha-MA(2)Z(4) with 1H-MX2 materials in a predictive CDW phase diagram using critical EPC constants, we demonstrate the feasibility of extending CDW across material families with comparable crystal fields and reveal the crucial role in CDW instability of the competition between ionic charge transfer and electron correlation. We further uncover a strain-induced Mott transition in beta(2)-NbGe2N4 monolayer featuring star-of-David patterns. This work highlights the potential of intercalating architecture to engineer CDW materials, expanding our understanding of CDW instability and correlation physics. |
| 资助项目 | National Natural Science Foundation of China[12304165] ; National Natural Science Foundation of China[12304086] ; Natural Science Foundation of Inner Mongolia Autonomous Region[2023QN01003] ; Inner Mongolia autonomous region[21200-242920] ; Startup Project of Inner Mongolia University[21200-5223733] |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| 语种 | 英语 |
| WOS记录号 | WOS:001292266000001 |
| 出版者 | AMER CHEMICAL SOC |
| 资助机构 | National Natural Science Foundation of China ; Natural Science Foundation of Inner Mongolia Autonomous Region ; Inner Mongolia autonomous region ; Startup Project of Inner Mongolia University |
| 源URL |  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Wang, Lei; Li, Xiao-Ping; Chen, Xing-Qiu |
| 作者单位 | 1.Inner Mongolia Univ, Sch Phys Sci & Technol, Hohhot 010021, Peoples R China 2.Inner Mongolia Univ, Inner Mongolia Key Lab Nanosci & Nanotechnol, Hohhot 010021, Peoples R China 3.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Lei,Wang, Shuaiyu,Niu, Yuekun,et al. Intercalating Architecture for the Design of Charge Density Wave in Metallic MA2Z4 Materials[J]. NANO LETTERS,2024:7. |
| APA | Wang, Lei.,Wang, Shuaiyu.,Niu, Yuekun.,Liu, Xiuying.,Wu, Yapeng.,...&Chen, Xing-Qiu.(2024).Intercalating Architecture for the Design of Charge Density Wave in Metallic MA2Z4 Materials.NANO LETTERS,7. |
| MLA | Wang, Lei,et al."Intercalating Architecture for the Design of Charge Density Wave in Metallic MA2Z4 Materials".NANO LETTERS (2024):7. |
入库方式： OAI收割
来源：金属研究所
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