Atomically dispersed metal cocatalysts for solar energy conversion
文献类型：期刊论文
| 作者 | Kong, Kejian1; Zhang, Hao2; Han, Ali1,3; Li, Feng2; Wang, Dingsheng1 |
| 刊名 | ENERGY & ENVIRONMENTAL SCIENCE
 |
| 出版日期 | 2024-09-04 |
| 页码 | 32 |
| ISSN号 | 1754-5692 |
| DOI | 10.1039/d4ee03065f |
| 通讯作者 | Han, Ali(hanali@mail.ustc.edu.cn) ; Li, Feng(li_feng@fudan.edu.cn) ; Wang, Dingsheng(wangdingsheng@mail.tsinghua.edu.cn) |
| 英文摘要 | The pursuit of clean and sustainable energy has become more urgent than ever. Photocatalysis is a potential approach to convert highly sustainable solar energy into promising fuels. Additionally, effective and robust cocatalysts are crucial factors in facilitating rapid photogenerated charge separation/charge transfer, widespread absorption and highly photoactive reactions and achieving efficient solar-to-chemical energy conversion. In this review, we summarize the recent advances in efficient cocatalysts provided with atomic metal sites, including single-atom metal cocatalysts (SAMCs) and atomic cluster metal cocatalysts (ACMCs). First, we present a general definition of atomic metal sites to improve our understanding of the structure-activity correlations at the atomic scale. Then, a brief description of advanced characterization techniques is given to distinguish the atomic metal sites. After introducing the atomic metal sites, regulating strategies for the enhancement of photocatalysis, such as electronic metal-support interaction (EMSI), atomic alloy strategy and confinement strategy, the advantages and disadvantages of each type of atomic metal sites and the solar energy conversion applications (water splitting, CO2 reduction, N2 reduction, etc.) are highlighted. Finally, the prospective and a summary of the comparison of different atomic metal sites as well as the potential development direction of photocatalysts in the future are outlined. This review explores the role of atomic metal site cocatalysts in photocatalysis for solar energy conversion, focusing on the recent advances in single-atom and atomic cluster cocatalysts, their structure-activity relationships, and key applications. |
| 资助项目 | National Natural Science Foundation of China[QXH2203003] ; National Natural Science Foundation of China[22375048] ; National Natural Science Foundation of China[22202214] ; National Natural Science Foundation of China[JIH2203013Y] ; Fudan University[2022-YQ-02] ; Natural Science Foundation of Liaoning Province-Outstanding Youth Foundation |
| WOS研究方向 | Chemistry ; Energy & Fuels ; Engineering ; Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:001316150800001 |
| 出版者 | ROYAL SOC CHEMISTRY |
| 资助机构 | National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fudan University ; Natural Science Foundation of Liaoning Province-Outstanding Youth Foundation |
| 源URL |  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Han, Ali; Li, Feng; Wang, Dingsheng |
| 作者单位 | 1.Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China 2.Fudan Univ, Lab Adv Mat, Shanghai Key Lab Mol Catalysis & Innovat Mat, 220 Handan, Shanghai 200433, Peoples R China 3.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China |
| 推荐引用方式 GB/T 7714 | Kong, Kejian,Zhang, Hao,Han, Ali,et al. Atomically dispersed metal cocatalysts for solar energy conversion[J]. ENERGY & ENVIRONMENTAL SCIENCE,2024:32. |
| APA | Kong, Kejian,Zhang, Hao,Han, Ali,Li, Feng,&Wang, Dingsheng.(2024).Atomically dispersed metal cocatalysts for solar energy conversion.ENERGY & ENVIRONMENTAL SCIENCE,32. |
| MLA | Kong, Kejian,et al."Atomically dispersed metal cocatalysts for solar energy conversion".ENERGY & ENVIRONMENTAL SCIENCE (2024):32. |
入库方式： OAI收割
来源：金属研究所
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