Production of Gasoline and Diesel from Coal Tar via Its Catalytic Hydrogenation in Serial Fixed Beds
文献类型:期刊论文
作者 | Kan, Tao; Sun, Xiaoyan; Wang, Hongyan; Li, Chunshan; Muhammad, Usman |
刊名 | ENERGY & FUELS
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出版日期 | 2012-06-01 |
卷号 | 26期号:6页码:3604-3611 |
关键词 | HYDROTREATING CATALYSTS HYDRODESULFURIZATION OIL DIBENZOTHIOPHENE AROMATICS TETRALIN INSIGHT |
ISSN号 | 0887-0624 |
通讯作者 | Li, CS |
英文摘要 | Clean liquid fuel was produced from the catalytic hydrogenation of coal tar using two serial fixed beds. Hydrofining catalyst of MoNi/gamma-Al2O3 and hydrocracking catalyst of WNiP/gamma-Al2O3-USY were filled in the first and second fixed beds, respectively. In the initial catalyst screening tests, the typical fixed experimental conditions were as follows: hydrogen pressure of 8 MPa, liquid hourly space velocity of 0.8 h(-1), hydrogen-to-tar volume ratio of 1600, temperature in first fixed bed at 360 degrees C, and temperature in second fixed bed at 380 degrees C. Gasoline (<= 180 degrees C) and diesel (180-360 degrees C) fractions were then separated from the effluent oil. Their fuel indexes were determined to assess the hydrogenation performance. The effect of pressure (6-10 MPa) on the hydrogenation performance was also investigated by keeping other experimental conditions constant. The catalysts showed good stability in activity in the test of catalyst life. The analysis results of the products indicated that raw coal tar could be promisingly upgraded by catalytic hydrogenation in the serial fixed beds. Nitrogen and sulfur contents were greatly reduced from 1.69 and 0.96 wt % in the feed to less than 10 and 50 ppm, respectively, in the products. |
WOS标题词 | Science & Technology ; Technology |
类目[WOS] | Energy & Fuels ; Engineering, Chemical |
研究领域[WOS] | Energy & Fuels ; Engineering |
关键词[WOS] | HYDROTREATING CATALYSTS ; HYDRODESULFURIZATION ; OIL ; DIBENZOTHIOPHENE ; AROMATICS ; TETRALIN ; INSIGHT |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000305444400053 |
公开日期 | 2013-10-16 |
版本 | 出版稿 |
源URL | [http://ir.ipe.ac.cn/handle/122111/3584] ![]() |
专题 | 过程工程研究所_多相复杂系统国家重点实验室 |
作者单位 | Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing Key Lab Ion Liquids Clean Proc, Beijing 100190, Peoples R China |
推荐引用方式 GB/T 7714 | Kan, Tao,Sun, Xiaoyan,Wang, Hongyan,et al. Production of Gasoline and Diesel from Coal Tar via Its Catalytic Hydrogenation in Serial Fixed Beds[J]. ENERGY & FUELS,2012,26(6):3604-3611. |
APA | Kan, Tao,Sun, Xiaoyan,Wang, Hongyan,Li, Chunshan,&Muhammad, Usman.(2012).Production of Gasoline and Diesel from Coal Tar via Its Catalytic Hydrogenation in Serial Fixed Beds.ENERGY & FUELS,26(6),3604-3611. |
MLA | Kan, Tao,et al."Production of Gasoline and Diesel from Coal Tar via Its Catalytic Hydrogenation in Serial Fixed Beds".ENERGY & FUELS 26.6(2012):3604-3611. |
入库方式: OAI收割
来源:过程工程研究所
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