Coal pyrolysis in a fluidized bed reactor simulating the process conditions of coal topping in CFB boiler
文献类型:期刊论文
| 作者 | Zhang, Xiaofang; Dong, Li; Zhang, Juwei; Tian, Yajun; Xu, Guangwen |
| 刊名 | JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS
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| 出版日期 | 2011-05-01 |
| 卷号 | 91期号:1页码:241-250 |
| 关键词 | Coal topping CFB boiler Fluidized bed Reaction atmosphere Pyrolysis oil TG-FTIR |
| ISSN号 | 0165-2370 |
| 通讯作者 | Xu, GW |
| 英文摘要 | Simulating the conditions of pyrolytic topping in a fluidized bed reactor integrated into a CFB boiler, the study was devoted to the reaction fundamentals of coal pyrolysis in terms of the production characteristics of pyrolysis oil in fluidized bed reactors, including pyrolysis oil yield, required reaction time and the chemical species presented in the pyrolysis oil. The results demonstrated that the maximal pyrolysis oil yield occurred on conditions of 873K, with a reaction time of 3 min and in a reaction atmosphere gas simulating the composition of pyrolysis gas. Adding H(2) and CO(2) into the reaction atmosphere decreased the pyrolysis oil yield, while the oil yield increased with increasing the CO and CH(4) contents in the atmosphere. TG-FTIR analysis was conducted to reveal the effects of reaction atmosphere on the chemical species present in the pyrolysis oil. The results clarified that the pyrolysis oil yield reached its maximum when the simulated pyrolysis gas was the reaction atmosphere, but there were slightly fewer volatile matters in the pyrolysis oil than the oil generated in the N(2) atmosphere. All of these results are expected not only to reveal the composition characteristics of the pyrolysis oil from different conditions of the coal topping process but also to optimize the pyrolysis conditions in terms of maximizing the light pyrolysis oil yield and quality. (C) 2011 Elsevier B.V. All rights reserved. |
| WOS标题词 | Science & Technology ; Physical Sciences ; Technology |
| 类目[WOS] | Chemistry, Analytical ; Spectroscopy |
| 研究领域[WOS] | Chemistry ; Spectroscopy |
| 关键词[WOS] | PRESSURE ; HYDROPYROLYSIS ; TEMPERATURE ; RATES |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000290779600028 |
| 公开日期 | 2013-11-05 |
| 版本 | 出版稿 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/4881] ![]() |
| 专题 | 过程工程研究所_多相复杂系统国家重点实验室 |
| 作者单位 | Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100080, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhang, Xiaofang,Dong, Li,Zhang, Juwei,et al. Coal pyrolysis in a fluidized bed reactor simulating the process conditions of coal topping in CFB boiler[J]. JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS,2011,91(1):241-250. |
| APA | Zhang, Xiaofang,Dong, Li,Zhang, Juwei,Tian, Yajun,&Xu, Guangwen.(2011).Coal pyrolysis in a fluidized bed reactor simulating the process conditions of coal topping in CFB boiler.JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS,91(1),241-250. |
| MLA | Zhang, Xiaofang,et al."Coal pyrolysis in a fluidized bed reactor simulating the process conditions of coal topping in CFB boiler".JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS 91.1(2011):241-250. |
入库方式: OAI收割
来源:过程工程研究所
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