Deep desulfurization of hydrodesulfurized diesel oil by Pseudomonas delafieldii R-8
文献类型:期刊论文
作者 | Shan, GB; Xing, JM; Zhang, HY; Liu, HZ |
刊名 | JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY
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出版日期 | 2005-04-01 |
卷号 | 80期号:4页码:420-424 |
关键词 | biodesulfurization hydrodesulfurized diesel oil Pseudomonas delafieldii alkylated dibenzothiophenes |
ISSN号 | 0268-2575 |
其他题名 | J. Chem. Technol. Biotechnol. |
中文摘要 | Biodesulfurization is a promising technology for deep desulfurization. The remaining alkylated DBTs (dibenzothiophenes) in the HDS-treated (hydrodesulfurized-treated) diesel oil could be selectively and efficiently desulfurized by resting cells of Pseudomonas delafieldii R-8, a Gram-negative bacterium. The desulfurization activities of resting cells were greatly affected by W/O ratio (the volume ratio of aqueous phase to oil phase) and cell concentration. The desulfurization activity increased with the increase in the W/O ratio. When the W/O ratio and cell concentration were 2 and 25 mg cm(-3), the desulfurization activity was as high as 0.41 mg (total sulfur) g(-1) (dry cell weight, DCW) h(-1), ie higher than that reported previously. GC-AED (gas chromatography with an atomic emission detector) analysis showed that the total reductions for all the C1DBTs and C2DBTs were approximately 100%, 94.63% for C3DBT, and 97.09% for C4DBT (designated CxDBT, where x is the number of alkyl groups attached). The rates of biodesulfurization relate to the number and position of alkyl groups attached to the DBT. (c) 2005 Society of Chemical Industry. |
英文摘要 | Biodesulfurization is a promising technology for deep desulfurization. The remaining alkylated DBTs (dibenzothiophenes) in the HDS-treated (hydrodesulfurized-treated) diesel oil could be selectively and efficiently desulfurized by resting cells of Pseudomonas delafieldii R-8, a Gram-negative bacterium. The desulfurization activities of resting cells were greatly affected by W/O ratio (the volume ratio of aqueous phase to oil phase) and cell concentration. The desulfurization activity increased with the increase in the W/O ratio. When the W/O ratio and cell concentration were 2 and 25 mg cm(-3), the desulfurization activity was as high as 0.41 mg (total sulfur) g(-1) (dry cell weight, DCW) h(-1), ie higher than that reported previously. GC-AED (gas chromatography with an atomic emission detector) analysis showed that the total reductions for all the C1DBTs and C2DBTs were approximately 100%, 94.63% for C3DBT, and 97.09% for C4DBT (designated CxDBT, where x is the number of alkyl groups attached). The rates of biodesulfurization relate to the number and position of alkyl groups attached to the DBT. (c) 2005 Society of Chemical Industry. |
WOS标题词 | Science & Technology ; Life Sciences & Biomedicine ; Physical Sciences ; Technology |
类目[WOS] | Biotechnology & Applied Microbiology ; Chemistry, Multidisciplinary ; Engineering, Chemical |
研究领域[WOS] | Biotechnology & Applied Microbiology ; Chemistry ; Engineering |
关键词[WOS] | MICROBIAL DESULFURIZATION ; MIDDLE-DISTILLATE ; CRUDE-OIL ; BIODESULFURIZATION ; DIBENZOTHIOPHENE ; PETROLEUM ; SULFUR ; STRAIN ; BACTERIA ; MODEL |
收录类别 | SCI |
原文出处 | |
语种 | 英语 |
WOS记录号 | WOS:000228019100009 |
公开日期 | 2013-10-25 |
版本 | 出版稿 |
源URL | [http://ir.ipe.ac.cn/handle/122111/4140] ![]() |
专题 | 过程工程研究所_研究所(批量导入) |
作者单位 | Chinese Acad Sci, State Key Lab Biochem Engn, Inst Proc Engn, Lab Seperat Sci & Engn, Beijing 100080, Peoples R China |
推荐引用方式 GB/T 7714 | Shan, GB,Xing, JM,Zhang, HY,et al. Deep desulfurization of hydrodesulfurized diesel oil by Pseudomonas delafieldii R-8[J]. JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY,2005,80(4):420-424. |
APA | Shan, GB,Xing, JM,Zhang, HY,&Liu, HZ.(2005).Deep desulfurization of hydrodesulfurized diesel oil by Pseudomonas delafieldii R-8.JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY,80(4),420-424. |
MLA | Shan, GB,et al."Deep desulfurization of hydrodesulfurized diesel oil by Pseudomonas delafieldii R-8".JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY 80.4(2005):420-424. |
入库方式: OAI收割
来源:过程工程研究所
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