Butene catalytic cracking to ethylene and propylene on fluorinated ZSM-5-based catalyst
文献类型：期刊论文
| 作者 | Tang ZC(唐志诚)1 ; Zhang P(张朋)1; Han WL(韩维亮)1; Lu GX(吕功煊)1; Lu JY(陆江银)2,3; Tang ZC(唐志诚)
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| 刊名 | Reaction Kinetics, Mechanisms and Catalysis
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| 出版日期 | 2013 |
| 卷号 | 108期号:1页码:231-239 |
| 关键词 | Fluorinated treatment Catalytic cracking Ethylene and propylene Micropore ZSM-5 zeolite |
| ISSN号 | 1878-5190 |
| 通讯作者 | 唐志诚 |
| 英文摘要 | In this paper, fluorine-containing ZSM-5 catalysts were first prepared and applied for butene catalytic cracking. Fluorinated ZSM-5 was obtained by treating the ZSM-5 zeolite with NH4F solutions at 85 C. XRD showed that the intrinsic mordenite framework inverted structure of ZSM-5 zeolite was preserved and the corresponding crystallinity remained unchanged. The N2 adsorption/desorption measure indicated the generation of a number of new micropores. The experiment of butene catalytic cracking showed that catalytic performances can be greatly improved after fluorination treatment. The highest yield of ethylene plus propylene was obtained when the treated concentration of NH4F solution is 0.1 M. |
| 学科主题 | 物理化学与绿色催化 |
| 收录类别 | SCI |
| 资助信息 | West Light Foundation of The Chinese Academy of Sciences;Science and Technique Program of Lanzhou City, Science-Technology Foundation for Middle-Aged and Young Scientist of Gansu Province;Key Laboratory of Oil & Gas Fine Chemicals, Ministry of Education & Xinjiang Uyghur Autonomous Region, Xinjiang University (XJDX0908-2011-03) |
| 语种 | 英语 |
| WOS记录号 | WOS:000313370800020 |
| 公开日期 | 2013-12-02 |
| 源URL | [http://210.77.64.217/handle/362003/4232]  |
| 专题 | 兰州化学物理研究所_ERC国家工程研究中心 兰州化学物理研究所_OSSO国家重点实验室 |
| 通讯作者 | Tang ZC(唐志诚) |
| 作者单位 | 1.Chinese Acad Sci, State Key Lab Oxo Synth & Select Oxidat, Natl Engn Res Ctr Fine Petrochem Intermediates, Lanzhou Inst Chem Phys, Lanzhou 730000, Peoples R China 2.Xinjiang Univ, Key Lab Oil & Gas Fine Chem, Minist Educ, Urumqi 830046, Xinjiang, Peoples R China 3.Xinjiang Univ, Xinjiang Uyghur Autonomous Reg, Urumqi 830046, Xinjiang, Peoples R China |
| 推荐引用方式 GB/T 7714 | Tang ZC,Zhang P,Han WL,et al. Butene catalytic cracking to ethylene and propylene on fluorinated ZSM-5-based catalyst[J]. Reaction Kinetics, Mechanisms and Catalysis,2013,108(1):231-239. |
| APA | Tang ZC,Zhang P,Han WL,Lu GX,Lu JY,&唐志诚.(2013).Butene catalytic cracking to ethylene and propylene on fluorinated ZSM-5-based catalyst.Reaction Kinetics, Mechanisms and Catalysis,108(1),231-239. |
| MLA | Tang ZC,et al."Butene catalytic cracking to ethylene and propylene on fluorinated ZSM-5-based catalyst".Reaction Kinetics, Mechanisms and Catalysis 108.1(2013):231-239. |
入库方式： OAI收割
来源：兰州化学物理研究所
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