Detailed Description of Coal Tar Hydrogenation Process Using the Kinetic Lumping Approach
文献类型：期刊论文
| 作者 | Dai, Fei1,2; Gao, Mingjie1; Li, Chunshan1; Xiang, Shuguang2; Zhang, Suojiang2 |
| 刊名 | ENERGY & FUELS
 |
| 出版日期 | 2011-11-01 |
| 卷号 | 25期号:11页码:4878-4885 |
| 关键词 | heavy oil hydrocracking model liquefaction pyrolysis catalyst residue gasoline |
| ISSN号 | 0887-0624 |
| 其他题名 | Energy Fuels |
| 中文摘要 | A new eight-lump kinetic model containing 19 kinetic constants is proposed to describe coal tar hydrogenation. The model contains lump 1 (> 300 degrees C), lump 2 (250-300 degrees C), lump 3 (200-250 degrees C), lump 4 (20-200 degrees C), diesel, gasoline, gas, and coke as lumps. The kinetic parameters were determined using least-squares regression analysis of the experimental data, obtained in two-stage fixed beds filled with the laboratory-made catalysts at various operating conditions. The proposed model was also validated. Comparisons between the experimental data and predictions using the lumping kinetic model showed good agreement. The variation in product yields and product distribution with operating conditions and feed properties was predicted. The effects of space velocity, hydrogen/oil ratio, temperature, initial hydrogen pressure, and other reaction conditions on hydrogenation performance were also investigated. |
| 英文摘要 | A new eight-lump kinetic model containing 19 kinetic constants is proposed to describe coal tar hydrogenation. The model contains lump 1 (> 300 degrees C), lump 2 (250-300 degrees C), lump 3 (200-250 degrees C), lump 4 (20-200 degrees C), diesel, gasoline, gas, and coke as lumps. The kinetic parameters were determined using least-squares regression analysis of the experimental data, obtained in two-stage fixed beds filled with the laboratory-made catalysts at various operating conditions. The proposed model was also validated. Comparisons between the experimental data and predictions using the lumping kinetic model showed good agreement. The variation in product yields and product distribution with operating conditions and feed properties was predicted. The effects of space velocity, hydrogen/oil ratio, temperature, initial hydrogen pressure, and other reaction conditions on hydrogenation performance were also investigated. |
| WOS标题词 | Science & Technology ; Technology |
| 类目[WOS] | Energy & Fuels ; Engineering, Chemical |
| 研究领域[WOS] | Energy & Fuels ; Engineering |
| 关键词[WOS] | HEAVY OIL ; HYDROCRACKING ; MODEL ; LIQUEFACTION ; PYROLYSIS ; CATALYST ; RESIDUE ; GASOLINE |
| 收录类别 | SCI |
| 原文出处 | |
| 语种 | 英语 |
| WOS记录号 | WOS:000297001400002 |
| 公开日期 | 2013-11-28 |
| 版本 | 出版稿 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/6302]  |
| 专题 | 过程工程研究所_研究所（批量导入） |
| 作者单位 | 1.Chinese Acad Sci, State Key Lab Multiphase Complex Syst, Inst Proc Engn, Beijing 100190, Peoples R China 2.Qingdao Univ Sci, Hitech Inst Petr, Qingdao 266042, Shandong, Peoples R China |
| 推荐引用方式 GB/T 7714 | Dai, Fei,Gao, Mingjie,Li, Chunshan,et al. Detailed Description of Coal Tar Hydrogenation Process Using the Kinetic Lumping Approach[J]. ENERGY & FUELS,2011,25(11):4878-4885. |
| APA | Dai, Fei,Gao, Mingjie,Li, Chunshan,Xiang, Shuguang,&Zhang, Suojiang.(2011).Detailed Description of Coal Tar Hydrogenation Process Using the Kinetic Lumping Approach.ENERGY & FUELS,25(11),4878-4885. |
| MLA | Dai, Fei,et al."Detailed Description of Coal Tar Hydrogenation Process Using the Kinetic Lumping Approach".ENERGY & FUELS 25.11(2011):4878-4885. |
入库方式： OAI收割
来源：过程工程研究所
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