Influence of Deoxyribose Group on Self-Assembly of Thymidine on Au(111)
文献类型：期刊论文
| 作者 | Yang, B ; Wang, YL ; Li, G ; Cun, HY ; Ma, Y ; Du, SX ; Xu, MC ; Song, YL ; Gao, HJ |
| 刊名 | JOURNAL OF PHYSICAL CHEMISTRY C
 |
| 出版日期 | 2009 |
| 卷号 | 113期号:41页码:17590 |
| 关键词 | SCANNING-TUNNELING-MICROSCOPY SINGLE-CRYSTAL ELECTRODES DNA BASES ADENINE ADSORPTION THYMINE URACIL SURFACES MONOLAYERS INTERFACE |
| ISSN号 | 1932-7447 |
| 通讯作者 | Gao, HJ: Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. |
| 中文摘要 | Using scanning tunneling microscopy (STM), we investigate the self-assembled structures and current-induced phase transition of one nucleoside species, thymidine (TD) on Au(111). By comparing the previous work on DNA nucleic acid base thymine on the same surface, we find that the deoxyribose groups of TD molecules remarkably enhance the intermolecular interaction and drive the formation of a dimer structure even at low temperature. At room temperature, TD molecules aggregate into well-ordered dimer islands. A two-dimensional (2D3) gas-like phase of mobile TD molecules is also found surrounding the islands, and it can be transformed into the dimer structure. Furthermore, a new phase, a parallel-line structure, was observed gradually developing around the dimer domains under consecutive scanning. These molecular lines can be produced from both the gas-like phase and the dimer. First-principle calculations illustrate the optimized molecular superstructures in both phases. |
| 收录类别 | SCI |
| 资助信息 | National Science Foundation of China [10674159, 10874219]; '863' and '973' projects; Supercomputing Center, CNIC, in China |
| 语种 | 英语 |
| 公开日期 | 2013-09-17 |
| 源URL | [http://ir.iphy.ac.cn/handle/311004/39799]  |
| 专题 | 物理研究所_物理所公开发表论文_物理所公开发表论文_期刊论文 |
| 推荐引用方式 GB/T 7714 | Yang, B,Wang, YL,Li, G,et al. Influence of Deoxyribose Group on Self-Assembly of Thymidine on Au(111)[J]. JOURNAL OF PHYSICAL CHEMISTRY C,2009,113(41):17590. |
| APA | Yang, B.,Wang, YL.,Li, G.,Cun, HY.,Ma, Y.,...&Gao, HJ.(2009).Influence of Deoxyribose Group on Self-Assembly of Thymidine on Au(111).JOURNAL OF PHYSICAL CHEMISTRY C,113(41),17590. |
| MLA | Yang, B,et al."Influence of Deoxyribose Group on Self-Assembly of Thymidine on Au(111)".JOURNAL OF PHYSICAL CHEMISTRY C 113.41(2009):17590. |
入库方式： OAI收割
来源：物理研究所
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