Noncollinear optical parametric amplifier based femtosecond time-resolved transient fluorescence spectra: characterization and correction
文献类型:期刊论文
作者 | Chen, HL ; Weng, YX ; Zhang, JY |
刊名 | JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS
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出版日期 | 2009 |
卷号 | 26期号:8页码:1627 |
关键词 | PULSE GENERATION RELAXATION PROCESSES UP-CONVERSION LUMINESCENCE SPECTROSCOPY LIGHT-PULSES AMPLIFICATION GATE SPECTROMETER PROTEINS SYSTEM |
ISSN号 | 0740-3224 |
通讯作者 | Weng, YX (reprint author), Chinese Acad Sci, Lab Soft Matter Phys, Beijing 100190, Peoples R China. |
中文摘要 | Spectral distortion frequently occurs in a recently developed femtosecond time-resolved fluorescence spectroscopy based on noncollinear optical parametric amplification, which would limit its applications if it is not treated appropriately. We report the mechanism for broadening and distortion of the amplified spectrum, and it was found that the amplified fluorescence spectral width and the corresponding pulse duration were limited by the uncertainty principle. We demonstrated that the nonuniform gain curve of nonlinear optical crystal in the wide spectral region is the main cause leading to the distorted spectrum. Theoretical analysis shows that by carefully adjusting the experimental parameters, such as propagation and noncollinear angles, the spectral fidelity can be achieved in a broad region. Moreover, we also proposed a method for retrieving the genuine spectrum from the distorted amplified spectrum by experimentally measuring the gain curve encoded in the spectrum of the parametric superfluorescence, which is collected during propagation at noncollinear angles the same as those for amplified fluorescence. (C) 2009 Optical Society of America |
收录类别 | SCI |
资助信息 | Natural Science Foundation of China (NSFC) [60438020, 60321003]; National Basic Research Program of China [2009CB930700]; CAS innovative projects [KJCX2SWW14]; Georgia Southern University |
语种 | 英语 |
公开日期 | 2013-09-24 |
源URL | [http://ir.iphy.ac.cn/handle/311004/49942] ![]() |
专题 | 物理研究所_物理所公开发表论文_物理所公开发表论文_期刊论文 |
推荐引用方式 GB/T 7714 | Chen, HL,Weng, YX,Zhang, JY. Noncollinear optical parametric amplifier based femtosecond time-resolved transient fluorescence spectra: characterization and correction[J]. JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS,2009,26(8):1627. |
APA | Chen, HL,Weng, YX,&Zhang, JY.(2009).Noncollinear optical parametric amplifier based femtosecond time-resolved transient fluorescence spectra: characterization and correction.JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS,26(8),1627. |
MLA | Chen, HL,et al."Noncollinear optical parametric amplifier based femtosecond time-resolved transient fluorescence spectra: characterization and correction".JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS 26.8(2009):1627. |
入库方式: OAI收割
来源:物理研究所
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