中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Semiclassical approach to plasmon-electron coupling and Landau damping of surface plasmons

文献类型:期刊论文

作者Gao, Y ; Yuan, Z ; Gao, SW
刊名JOURNAL OF CHEMICAL PHYSICS
出版日期2011
卷号134期号:13
关键词OPTICAL-PROPERTIES GOLD NANOSHELLS SILVER FILMS NANOPARTICLES HYBRIDIZATION SCATTERING LIFETIME MODEL
ISSN号0021-9606
通讯作者Gao, Y (reprint author), Chinese Acad Sci, Inst Phys, Beijing 10190, Peoples R China.
中文摘要A semiclassical model is developed to describe plasmon-electron coupling and electronic damping of surface plasmons. It is compared with the ab initio linear response calculations for metallic thin films in the jellium approximation and for a realistic crystalline Mg(0001) surface. The semiclassical model is able to reproduce the quantum oscillations of plasmon linewidth, which was obtained in the previous ab initio calculations. In addition, state-resolved analysis reveals the origin of these oscillations, which result from superposition of the short-period oscillations of individual electron-hole pair transitions. The semiclassical model is further applied to a crystalline Mg(0001) surface, where linewidth dispersion of the surface plasmon is calculated and shows good agreement with earlier ab initio calculation and experiment. Our results suggest that this semiclassical approach is quite promising for the quantitative description of plasmon-electron coupling and associated processes such as surface-enhanced Raman scattering, light emission, and fluorescence. (C) 2011 American Institute of Physics. [doi: 10.1063/1.3575185]
收录类别SCI
资助信息NSFC; MOST, China; STINT, Sweden
语种英语
公开日期2013-09-24
源URL[http://ir.iphy.ac.cn/handle/311004/52470]  
专题物理研究所_物理所公开发表论文_物理所公开发表论文_期刊论文
推荐引用方式
GB/T 7714
Gao, Y,Yuan, Z,Gao, SW. Semiclassical approach to plasmon-electron coupling and Landau damping of surface plasmons[J]. JOURNAL OF CHEMICAL PHYSICS,2011,134(13).
APA Gao, Y,Yuan, Z,&Gao, SW.(2011).Semiclassical approach to plasmon-electron coupling and Landau damping of surface plasmons.JOURNAL OF CHEMICAL PHYSICS,134(13).
MLA Gao, Y,et al."Semiclassical approach to plasmon-electron coupling and Landau damping of surface plasmons".JOURNAL OF CHEMICAL PHYSICS 134.13(2011).

入库方式: OAI收割

来源:物理研究所

浏览0
下载0
收藏0
其他版本

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。