Semiclassical approach to plasmon-electron coupling and Landau damping of surface plasmons
文献类型:期刊论文
作者 | Gao, Y ; Yuan, Z ; Gao, SW |
刊名 | JOURNAL OF CHEMICAL PHYSICS
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出版日期 | 2011 |
卷号 | 134期号:13 |
关键词 | OPTICAL-PROPERTIES GOLD NANOSHELLS SILVER FILMS NANOPARTICLES HYBRIDIZATION SCATTERING LIFETIME MODEL |
ISSN号 | 0021-9606 |
通讯作者 | Gao, Y (reprint author), Chinese Acad Sci, Inst Phys, Beijing 10190, Peoples R China. |
中文摘要 | A semiclassical model is developed to describe plasmon-electron coupling and electronic damping of surface plasmons. It is compared with the ab initio linear response calculations for metallic thin films in the jellium approximation and for a realistic crystalline Mg(0001) surface. The semiclassical model is able to reproduce the quantum oscillations of plasmon linewidth, which was obtained in the previous ab initio calculations. In addition, state-resolved analysis reveals the origin of these oscillations, which result from superposition of the short-period oscillations of individual electron-hole pair transitions. The semiclassical model is further applied to a crystalline Mg(0001) surface, where linewidth dispersion of the surface plasmon is calculated and shows good agreement with earlier ab initio calculation and experiment. Our results suggest that this semiclassical approach is quite promising for the quantitative description of plasmon-electron coupling and associated processes such as surface-enhanced Raman scattering, light emission, and fluorescence. (C) 2011 American Institute of Physics. [doi: 10.1063/1.3575185] |
收录类别 | SCI |
资助信息 | NSFC; MOST, China; STINT, Sweden |
语种 | 英语 |
公开日期 | 2013-09-24 |
源URL | [http://ir.iphy.ac.cn/handle/311004/52470] ![]() |
专题 | 物理研究所_物理所公开发表论文_物理所公开发表论文_期刊论文 |
推荐引用方式 GB/T 7714 | Gao, Y,Yuan, Z,Gao, SW. Semiclassical approach to plasmon-electron coupling and Landau damping of surface plasmons[J]. JOURNAL OF CHEMICAL PHYSICS,2011,134(13). |
APA | Gao, Y,Yuan, Z,&Gao, SW.(2011).Semiclassical approach to plasmon-electron coupling and Landau damping of surface plasmons.JOURNAL OF CHEMICAL PHYSICS,134(13). |
MLA | Gao, Y,et al."Semiclassical approach to plasmon-electron coupling and Landau damping of surface plasmons".JOURNAL OF CHEMICAL PHYSICS 134.13(2011). |
入库方式: OAI收割
来源:物理研究所
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