中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Structure and magnetic properties of R2Co17-xSix (x = 0-3) compounds with R = Y and Pr

文献类型:期刊论文

作者Zhang, ZY ; Shen, BG ; Li, RW ; Ruan, XF ; Liang, B ; Zhang, HW ; Wang, FW ; Zhan, WS ; Zhang, LG
刊名JOURNAL OF PHYSICS-CONDENSED MATTER
出版日期1998
卷号10期号:11页码:2445
关键词MAGNETOCRYSTALLINE ANISOTROPY NEUTRON-DIFFRACTION GA-CONCENTRATION SOLID-SOLUTIONS SM2FE17-XSIX SI
ISSN号0953-8984
通讯作者Zhang, ZY (reprint author), Chinese Acad Sci, Inst Phys, State Key Lab Magnetism, POB 603, Beijing 100080, Peoples R China.
中文摘要The influence of Si substitution for Co or, the structure and magnetic properties of Y2Co17-xSix and Pr2Co17-xSix (x = 0-3) compounds were investigated by means of x-ray diffraction and magnetization measurements. X-ray diffraction patterns demonstrate that all samples are single phase with the hexagonal Th2Ni17-type structure for Y2Co17-xSix and the rhombohedral Th2Zn17-type structure for Pr2Co17-xSix compounds, except for Pr2Co14Si3 With a small amount of impurity phases. The unit-cell volume is found to decrease linearly with increasing Si concentration in both series. The Curie temperature decreases monotonically with increasing Si concentration at an approximate rate of 205 and 175 K per Si atom for the Y2Co17-xSix and Pr2Co17-xSix compounds, respectively. The saturation magnetic moments of R2Co17-xSix (R = Y, Pr) decrease with increasing Si content and the decline rates are larger than that expected as a simple dilution. For Y2Co17-xSix, the substitution of Si has a significant effect on the magnetocrystalline anisotropy of the Co sublattice, and changes the easy magnetization direction from the basal plane to the c-axis at room temperature. For Pr2Co17-xSix, the Si substitution has not changed the easy magnetization direction at room temperature. However, the spin-reorientation transitions from the basal plane to the c-axis for this series with 0.5 less than or equal to x less than or equal to 2.4 were observed above room temperature with increasing temperature. The spin-reorientation temperature TSR first decreases with increasing Si content and then increases at higher x values (x > 2). The origin of this spin reorientation is interpreted by the competition between the Pr sublattice anisotropy and the Co sublattice anisotropy. This has been confirmed by the magnetocrystalline anisotropy measurements on Y2Co17-xSix.
收录类别SCI
语种英语
公开日期2013-09-24
源URL[http://ir.iphy.ac.cn/handle/311004/53482]  
专题物理研究所_物理所公开发表论文_物理所公开发表论文_期刊论文
推荐引用方式
GB/T 7714
Zhang, ZY,Shen, BG,Li, RW,et al. Structure and magnetic properties of R2Co17-xSix (x = 0-3) compounds with R = Y and Pr[J]. JOURNAL OF PHYSICS-CONDENSED MATTER,1998,10(11):2445.
APA Zhang, ZY.,Shen, BG.,Li, RW.,Ruan, XF.,Liang, B.,...&Zhang, LG.(1998).Structure and magnetic properties of R2Co17-xSix (x = 0-3) compounds with R = Y and Pr.JOURNAL OF PHYSICS-CONDENSED MATTER,10(11),2445.
MLA Zhang, ZY,et al."Structure and magnetic properties of R2Co17-xSix (x = 0-3) compounds with R = Y and Pr".JOURNAL OF PHYSICS-CONDENSED MATTER 10.11(1998):2445.

入库方式: OAI收割

来源:物理研究所

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