Oxygen-Vacancy-Induced Antiferromagnetism to Ferromagnetism Transformation in Eu0.5Ba0.5TiO3-delta Multiferroic Thin Films
文献类型:期刊论文
作者 | Li, WW ; Zhao, R ; Wang, L ; Tang, RJ ; Zhu, YY ; Lee, JH ; Cao, HX ; Cai, TY ; Guo, HZ ; Wang, C ; Ling, LS ; Pi, L ; Jin, KJ ; Zhang, YH ; Wang, HY ; Wang, YQ ; Ju, S ; Yang, H |
刊名 | SCIENTIFIC REPORTS
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出版日期 | 2013 |
卷号 | 3 |
ISSN号 | 2045-2322 |
通讯作者 | Yang, H (reprint author), Soochow Univ, Sch Phys Sci & Technol, Jiangsu Key Lab Thin Films, Suzhou 215006, Peoples R China. |
中文摘要 | Oxygen vacancies (V-O) effects on magnetic ordering in Eu0.5Ba0.5TiO3-delta (EBTO3-delta) thin films have been investigated using a combination of experimental measurements and first-principles density-functional calculations. Two kinds of EBTO3-delta thin films with different oxygen deficiency have been fabricated. A nuclear resonance backscattering spectrometry technique has been used to quantitatively measure contents of the V-O. Eu0.5Ba0.5TiO3 ceramics have been known to exhibit ferroelectric (FE) and G-type antiferromagnetic (AFM) properties. While, a ferromagnetic (FM) behavior with a Curie temperature of 1.85 K has been found in the EBTO3-delta thin films. Spin-polarized Ti3+ ions, which originated from the V-O, has been proven to mediate a FM coupling between the local Eu 4f spins and were believed to be responsible for the great change of the magnetic ordering. Considering the easy formation of V-O, our work opens up a new avenue for achieving co-existence of FM and FE orders in oxide materials. |
资助信息 | National Natural Science Foundation of China [11004145, 11274237, 11134012, 11104193, 51228201, 51202153]; Natural Science Foundation of Jiangsu Province [SBK201021263]; Scientific Research Foundation for the Returned Overseas Chinese Scholars (State Education Ministry of China); Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD); US National Science Foundation [NSF-0846504] |
语种 | 英语 |
公开日期 | 2014-01-16 |
源URL | [http://ir.iphy.ac.cn/handle/311004/57312] ![]() |
专题 | 物理研究所_物理所公开发表论文_物理所公开发表论文_期刊论文 |
推荐引用方式 GB/T 7714 | Li, WW,Zhao, R,Wang, L,et al. Oxygen-Vacancy-Induced Antiferromagnetism to Ferromagnetism Transformation in Eu0.5Ba0.5TiO3-delta Multiferroic Thin Films[J]. SCIENTIFIC REPORTS,2013,3. |
APA | Li, WW.,Zhao, R.,Wang, L.,Tang, RJ.,Zhu, YY.,...&Yang, H.(2013).Oxygen-Vacancy-Induced Antiferromagnetism to Ferromagnetism Transformation in Eu0.5Ba0.5TiO3-delta Multiferroic Thin Films.SCIENTIFIC REPORTS,3. |
MLA | Li, WW,et al."Oxygen-Vacancy-Induced Antiferromagnetism to Ferromagnetism Transformation in Eu0.5Ba0.5TiO3-delta Multiferroic Thin Films".SCIENTIFIC REPORTS 3(2013). |
入库方式: OAI收割
来源:物理研究所
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