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Organochlorine Pesticides in the Atmosphere and Surface Water from the Equatorial Indian Ocean: Enantiomeric Signatures, Sources, and Fate

文献类型：期刊论文

作者Huang, Yumei1,3; Xu, Yue1; Li, Jun1; Xu, Weihai2; Zhang, Gan1; Cheng, Zhineng1,3; Liu, Junwen1,3; Wang, Yan1; Tian, Chongguo4,5
刊名ENVIRONMENTAL SCIENCE & TECHNOLOGY
出版日期2013-12-03
卷号47期号:23页码:13395-13403
关键词PERSISTENT ORGANIC POLLUTANTS NORTH-ATLANTIC ARCTIC-OCEAN SOUTH CHINA ALPHA-HEXACHLOROCYCLOHEXANE CLIMATE-CHANGE GAS-EXCHANGE AIR SEA HCH
ISSN号0013-936X
其他题名Potentiometric Determination of Dopamine Using a Solid-Contact Polymeric Membrane Ion-Selective Electrode.pdf
产权排序[Huang, Yumei; Xu, Yue; Li, Jun; Zhang, Gan; Cheng, Zhineng; Liu, Junwen; Wang, Yan] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China; [Xu, Weihai] Chinese Acad Sci, South China Sea Inst Oceanol, CAS Key Lab Marginal Sea Geol, Guangzhou 510301, Guangdong, Peoples R China; [Huang, Yumei; Cheng, Zhineng; Liu, Junwen] Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China; [Tian, Chongguo] Chinese Acad Sci, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai Inst Coastal Zone Res, Yantai 264003, Shandong, Peoples R China; [Tian, Chongguo] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Shandong Prov Key Lab Coastal Zone Environm Proc, Yantai 264003, Shandong, Peoples R China
通讯作者Xu, Y (reprint author), Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China. xuyue@gig.ac.cn
中文摘要Nineteen pairs of gaseous and surface seawater samples were collected along the cruise from Malaysia to the south of Bay of Bengal passing by Sri Lanka between April 12 and May 4, 2011 on the Chinese research vessel Shiyan I to investigate the latest OCP pollution status over the equatorial Indian Ocean. Significant decrease of alpha-HCH and gamma-HCH was found in the air and dissolved water phase owing to global restriction for decades. Substantially high levels of p,p'-DDT, o,p'-DDT, trans-chlordane (TC), and cis-chlordane (CC) were observed in the water samples collected near Sri Lanka, indicating fresh continental riverine input of these compounds. Fugacity fractions suggest equilibrium of alpha-HCH at most sampling sites, while net volatilization for DDT isomers, TC and CC in most cases. Enantiomer fractions (EFs) of alpha-HCH and o,p'-DDT in the air and water samples were determined to trace the source of these compounds in the air. Racemic or close to racemic composition was found for atmospheric alpha-HCH and o,p'-DDT, while significant depletion of (+) enantiomer was found in the water phase, especially for o,p'-DDT (EFs = 0.310 + 0.178). 24% of alpha-HCH in the lower air over the open sea of the equatorial Indian Ocean is estimated to be volatilized from local seawater, indicating that long-range transport is the main source.
英文摘要Nineteen pairs of gaseous and surface seawater samples were collected along the cruise from Malaysia to the south of Bay of Bengal passing by Sri Lanka between April 12 and May 4, 2011 on the Chinese research vessel Shiyan I to investigate the latest OCP pollution status over the equatorial Indian Ocean. Significant decrease of alpha-HCH and gamma-HCH was found in the air and dissolved water phase owing to global restriction for decades. Substantially high levels of p,p'-DDT, o,p'-DDT, trans-chlordane (TC), and cis-chlordane (CC) were observed in the water samples collected near Sri Lanka, indicating fresh continental riverine input of these compounds. Fugacity fractions suggest equilibrium of alpha-HCH at most sampling sites, while net volatilization for DDT isomers, TC and CC in most cases. Enantiomer fractions (EFs) of alpha-HCH and o,p'-DDT in the air and water samples were determined to trace the source of these compounds in the air. Racemic or close to racemic composition was found for atmospheric alpha-HCH and o,p'-DDT, while significant depletion of (+) enantiomer was found in the water phase, especially for o,p'-DDT (EFs = 0.310 + 0.178). 24% of alpha-HCH in the lower air over the open sea of the equatorial Indian Ocean is estimated to be volatilized from local seawater, indicating that long-range transport is the main source.
学科主题Engineering, Environmental ; Environmental Sciences
研究领域[WOS]Engineering ; Environmental Sciences & Ecology
关键词[WOS]PERSISTENT ORGANIC POLLUTANTS ; NORTH-ATLANTIC ; ARCTIC-OCEAN ; SOUTH CHINA ; ALPHA-HEXACHLOROCYCLOHEXANE ; CLIMATE-CHANGE ; GAS-EXCHANGE ; AIR ; SEA ; HCH
收录类别SCI
资助信息Chinese Academy of Sciences [KZCX2-YW-GJ02]; Natural Science Foundation of China (NSFC) [41125014, 41073080]
原文出处http://dx.doi.org/10.1021/es403138p
语种英语
WOS记录号WOS:000327999400026
公开日期2014-07-08
源URL[http://ir.yic.ac.cn/handle/133337/6927]  
专题烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
作者单位1.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
2.Chinese Acad Sci, South China Sea Inst Oceanol, CAS Key Lab Marginal Sea Geol, Guangzhou 510301, Guangdong, Peoples R China
3.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
4.Chinese Acad Sci, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai Inst Coastal Zone Res, Yantai 264003, Shandong, Peoples R China
5.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Shandong Prov Key Lab Coastal Zone Environm Proc, Yantai 264003, Shandong, Peoples R China
推荐引用方式
GB/T 7714		 Huang, Yumei,Xu, Yue,Li, Jun,et al. Organochlorine Pesticides in the Atmosphere and Surface Water from the Equatorial Indian Ocean: Enantiomeric Signatures, Sources, and Fate[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2013,47(23):13395-13403.
APA Huang, Yumei.,Xu, Yue.,Li, Jun.,Xu, Weihai.,Zhang, Gan.,...&Tian, Chongguo.(2013).Organochlorine Pesticides in the Atmosphere and Surface Water from the Equatorial Indian Ocean: Enantiomeric Signatures, Sources, and Fate.ENVIRONMENTAL SCIENCE & TECHNOLOGY,47(23),13395-13403.
MLA Huang, Yumei,et al."Organochlorine Pesticides in the Atmosphere and Surface Water from the Equatorial Indian Ocean: Enantiomeric Signatures, Sources, and Fate".ENVIRONMENTAL SCIENCE & TECHNOLOGY 47.23(2013):13395-13403.

入库方式： OAI收割

来源：烟台海岸带研究所

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