The Use of Levoglucosan and Radiocarbon for Source Apportionment of PM2.5 Carbonaceous Aerosols at a Background Site in East China
文献类型：期刊论文
| 作者 | Liu, Di1,4; Li, Jun1; Zhang, Yanlin1; Xu, Yue1; Liu, Xiang1; Ding, Ping2; Shen, Chengde2; Chen, Yingjun3; Tian, Chongguo3 ; Zhang, Gan1
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| 刊名 | ENVIRONMENTAL SCIENCE & TECHNOLOGY
 |
| 出版日期 | 2013-09-17 |
| 卷号 | 47期号:18页码:10454-10461 |
| 关键词 | BIOMASS BURNING SMOKE AMBIENT AEROSOL BLACK CARBON C-14 MEASUREMENTS SOUTHEAST CHINA ORGANIC AEROSOL FOSSIL SOURCES RURAL SITE TRANSPORT SYSTEM |
| ISSN号 | 0013-936X |
| 产权排序 | [Liu, Di; Li, Jun; Zhang, Yanlin; Xu, Yue; Liu, Xiang; Zhang, Gan] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China; [Ding, Ping; Shen, Chengde] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Isotope Geochem, Guangzhou 510640, Guangdong, Peoples R China; [Chen, Yingjun; Tian, Chongguo] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China; [Liu, Di] Chinese Acad Sci, Grad Univ, Beijing 100039, Peoples R China |
| 通讯作者 | Li, J (reprint author), Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China. junli@gig.ac.cn |
| 中文摘要 | Samples of fine particulate matter (PM2.5) were collected during July 2009 to March 2010 at a regional background site in East China. The mass concentrations of organic carbon (OC) and elemental carbon (EC) were characterized by the highest levels in winter (December to February) and the lowest abundances in summer (June to August). Conversely, the concentrations of levoglucosan were higher in summer than in winter. The observations were associated to the anthropogenic air pollutions (predominantly fossil-fuel combustions) transport from the center and north China with the northwest winds in winter and large contribution of the open biomass burning activities in South China and East China in summer, which was evident by air-mass trajectories and MODIS satellite fire counts. To assign fossil and nonfossil contributions of carbonaceous matters, the radiocarbon contents in water-insoluble OC (WINSOC) and EC in 4 combined samples representing four seasons were analyzed using the isolation system established in China. The results indicated that biomass burning and biogenic sources (59%) were the major contribution to the WINSOC, whereas fossil fuel (78%) was the dominant contributor to the refractory EC at this site. The source variation obtained by radiocarbon was consistent with other indicators, such as the OC/EC ratios and the levoglucosan concentration. Biomass burning and biogenic emissions were found to predominate in the summer and autumn, whereas fossil fuel emissions predominate in winter and spring. |
| 英文摘要 | Samples of fine particulate matter (PM2.5) were collected during July 2009 to March 2010 at a regional background site in East China. The mass concentrations of organic carbon (OC) and elemental carbon (EC) were characterized by the highest levels in winter (December to February) and the lowest abundances in summer (June to August). Conversely, the concentrations of levoglucosan were higher in summer than in winter. The observations were associated to the anthropogenic air pollutions (predominantly fossil-fuel combustions) transport from the center and north China with the northwest winds in winter and large contribution of the open biomass burning activities in South China and East China in summer, which was evident by air-mass trajectories and MODIS satellite fire counts. To assign fossil and nonfossil contributions of carbonaceous matters, the radiocarbon contents in water-insoluble OC (WINSOC) and EC in 4 combined samples representing four seasons were analyzed using the isolation system established in China. The results indicated that biomass burning and biogenic sources (59%) were the major contribution to the WINSOC, whereas fossil fuel (78%) was the dominant contributor to the refractory EC at this site. The source variation obtained by radiocarbon was consistent with other indicators, such as the OC/EC ratios and the levoglucosan concentration. Biomass burning and biogenic emissions were found to predominate in the summer and autumn, whereas fossil fuel emissions predominate in winter and spring. |
| 学科主题 | Engineering, Environmental ; Environmental Sciences |
| 研究领域[WOS] | Engineering ; Environmental Sciences & Ecology |
| 关键词[WOS] | BIOMASS BURNING SMOKE ; AMBIENT AEROSOL ; BLACK CARBON ; C-14 MEASUREMENTS ; SOUTHEAST CHINA ; ORGANIC AEROSOL ; FOSSIL SOURCES ; RURAL SITE ; TRANSPORT ; SYSTEM |
| 收录类别 | SCI |
| 资助信息 | Chinese Academy of Sciences [XDB05040503]; Natural Science Foundation of China (NSFC) [41125014, 41273117]; Earmarked Fund of the State Key Laboratory of Organic Geochemistry [OGL-200804] |
| 原文出处 | http://dx.doi.org/10.1021/es401250k |
| 语种 | 英语 |
| WOS记录号 | WOS:000330096000048 |
| 公开日期 | 2014-07-08 |
| 源URL | [http://ir.yic.ac.cn/handle/133337/6950]  |
| 专题 | 烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室 |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Isotope Geochem, Guangzhou 510640, Guangdong, Peoples R China 3.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China 4.Chinese Acad Sci, Grad Univ, Beijing 100039, Peoples R China |
| 推荐引用方式 GB/T 7714 | Liu, Di,Li, Jun,Zhang, Yanlin,et al. The Use of Levoglucosan and Radiocarbon for Source Apportionment of PM2.5 Carbonaceous Aerosols at a Background Site in East China[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2013,47(18):10454-10461. |
| APA | Liu, Di.,Li, Jun.,Zhang, Yanlin.,Xu, Yue.,Liu, Xiang.,...&Zhang, Gan.(2013).The Use of Levoglucosan and Radiocarbon for Source Apportionment of PM2.5 Carbonaceous Aerosols at a Background Site in East China.ENVIRONMENTAL SCIENCE & TECHNOLOGY,47(18),10454-10461. |
| MLA | Liu, Di,et al."The Use of Levoglucosan and Radiocarbon for Source Apportionment of PM2.5 Carbonaceous Aerosols at a Background Site in East China".ENVIRONMENTAL SCIENCE & TECHNOLOGY 47.18(2013):10454-10461. |
入库方式： OAI收割
来源：烟台海岸带研究所
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