Thermodynamic Modeling and Assessment of Ionic Liquid-Based CO2 Capture Processes
文献类型：期刊论文
| 作者 | Huang, Ying1,2; Zhang, Xiangping1; Zhang, Xin1,2; Dong, Haifeng1; Zhang, Suojiang1 |
| 刊名 | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
 |
| 出版日期 | 2014-07-23 |
| 卷号 | 53期号:29页码:11805-11817 |
| 关键词 | CARBON-DIOXIDE ABSORPTION POWER-PLANTS VAPOR-PRESSURE NATURAL-GAS 1-BUTYL-3-METHYLIMIDAZOLIUM TETRAFLUOROBORATE STRIPPER CONFIGURATIONS TECHNOECONOMIC ANALYSIS MONOETHANOLAMINE MEA AQUEOUS-SOLUTIONS TERNARY-SYSTEMS |
| ISSN号 | 0888-5885 |
| 其他题名 | Ind. Eng. Chem. Res. |
| 中文摘要 | Ionic liquid (IL)-amine hybrid solvents have been experimentally proved to be effective for CO2 capture. This Article provided rigorous thermodynamic models, process simulation, and cost estimation of a potential design of IL-based CO2 capture processes. Three lLs ([Bmim][BF4], [Bmim][DCA], and [Bpy][BF4]) were investigated to blend with MEA aqueous solution. The physicochemical properties of the ILs were predicted by several temperature-dependent correlations. Phase equilibria were modeled based on Henry's law and NRTL equation, and the calculated values were in good agreement with the experimental data. The simulation results show that the [Bpy][BF4]-MEA process can save about 15% regeneration heat duty as compared to the conventional MEA process, which is attributed to the reduction of sensible and latent heat. Moreover, a modified [Bpy][BF4]-MEA process via adding intercooling and lean vapor recompression presents 12% and 13.5% reduction in overall equivalent energy penalty and capture cost as compared to the conventional MEA process, respectively. |
| 英文摘要 | Ionic liquid (IL)-amine hybrid solvents have been experimentally proved to be effective for CO2 capture. This Article provided rigorous thermodynamic models, process simulation, and cost estimation of a potential design of IL-based CO2 capture processes. Three lLs ([Bmim][BF4], [Bmim][DCA], and [Bpy][BF4]) were investigated to blend with MEA aqueous solution. The physicochemical properties of the ILs were predicted by several temperature-dependent correlations. Phase equilibria were modeled based on Henry's law and NRTL equation, and the calculated values were in good agreement with the experimental data. The simulation results show that the [Bpy][BF4]-MEA process can save about 15% regeneration heat duty as compared to the conventional MEA process, which is attributed to the reduction of sensible and latent heat. Moreover, a modified [Bpy][BF4]-MEA process via adding intercooling and lean vapor recompression presents 12% and 13.5% reduction in overall equivalent energy penalty and capture cost as compared to the conventional MEA process, respectively. |
| WOS标题词 | Science & Technology ; Technology |
| 类目[WOS] | Engineering, Chemical |
| 研究领域[WOS] | Engineering |
| 关键词[WOS] | CARBON-DIOXIDE ABSORPTION ; POWER-PLANTS ; VAPOR-PRESSURE ; NATURAL-GAS ; 1-BUTYL-3-METHYLIMIDAZOLIUM TETRAFLUOROBORATE ; STRIPPER CONFIGURATIONS ; TECHNOECONOMIC ANALYSIS ; MONOETHANOLAMINE MEA ; AQUEOUS-SOLUTIONS ; TERNARY-SYSTEMS |
| 收录类别 | SCI |
| 原文出处 | |
| 语种 | 英语 |
| WOS记录号 | WOS:000339471500025 |
| 公开日期 | 2014-08-28 |
| 版本 | 出版稿 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/10916]  |
| 专题 | 过程工程研究所_研究所（批量导入） |
| 作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, Key Lab Green Proc & Engn, Beijing Key Lab Ion Liquids Clean Proc,State Key, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Sch Chem & Chem Engn, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Huang, Ying,Zhang, Xiangping,Zhang, Xin,et al. Thermodynamic Modeling and Assessment of Ionic Liquid-Based CO2 Capture Processes[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2014,53(29):11805-11817. |
| APA | Huang, Ying,Zhang, Xiangping,Zhang, Xin,Dong, Haifeng,&Zhang, Suojiang.(2014).Thermodynamic Modeling and Assessment of Ionic Liquid-Based CO2 Capture Processes.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,53(29),11805-11817. |
| MLA | Huang, Ying,et al."Thermodynamic Modeling and Assessment of Ionic Liquid-Based CO2 Capture Processes".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 53.29(2014):11805-11817. |
入库方式： OAI收割
来源：过程工程研究所
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