Recent progress in methane dehydroaromatization: From laboratory curiosities to promising technology
文献类型：期刊论文
| 作者 | Ma, Shuqi1,2 ; Guo, Xiaoguang1; Zhao, Lingxiao1; Scott, Susannah3,4; Bao, Xinhe1
|
| 刊名 | journal of energy chemistry
 |
| 出版日期 | 2013 |
| 卷号 | 22期号:1页码:1-20 |
| 关键词 | direct conversion methane methane dehydroaromatization Mo-based catalyst |
| 产权排序 | 待补充 |
| 通讯作者 | 包信和 |
| 合作状况 | 英 |
| 英文摘要 | direct conversion of methane to benzene or other valuable chemicals is a very promising process for the efficient application of natural gas. compared with conversion processes that require oxidants, non-oxidative direct conversion is more attractive due to high selectivity to the target product. in this paper, an alternative route for methane dehydrogenation and selective conversion to benzene and hydrogen without the participation of oxygen is discussed. a brief review of the catalysts used in methane dehydroaromatization (mda) is first given, followed by our current understanding of the location and the active phase of mo species, the reaction mechanism, the mechanism of carbonaceous deposit and the deactivation of mo/zeolite catalysts are systematically discussed. ways to improve the catalytic activity and stability are described in detail based on catalyst and reaction as well as reactor design. future prospects for methane dehydroaromatization process are also presented. |
| WOS标题词 | science & technology ; physical sciences ; technology |
| 学科主题 | 物理化学 |
| 类目[WOS] | chemistry, applied ; chemistry, physical ; energy & fuels ; engineering, chemical |
| 研究领域[WOS] | chemistry ; energy & fuels ; engineering |
| 关键词[WOS] | mo-based catalysts ; hydrothermal post-synthesis ; bronsted acid sites ; temperature nonoxidative activation ; galloaluminosilicate mfi zeolite ; impregnated hzsm-5 catalysts ; highly stable performance ; supersonic jet expansion ; single-pass conversion ; mo-95 nmr-spectroscopy |
| 收录类别 | SCI |
| 资助信息 | 1，1 |
| 原文出处 | 20 |
| 语种 | 英语 |
| WOS记录号 | WOS:000318050700002 |
| 公开日期 | 2014-09-11 |
| 源URL | [http://159.226.238.44/handle/321008/119624]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China 2.Henan Polytech Univ, Sch Phys & Chem, Jiaozuo 454000, Henan, Peoples R China 3.Univ Calif Santa Barbara, Dept Chem & Biochem, Santa Barbara, CA 93106 USA 4.Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA |
| 推荐引用方式 GB/T 7714 | Ma, Shuqi,Guo, Xiaoguang,Zhao, Lingxiao,et al. Recent progress in methane dehydroaromatization: From laboratory curiosities to promising technology[J]. journal of energy chemistry,2013,22(1):1-20. |
| APA | Ma, Shuqi,Guo, Xiaoguang,Zhao, Lingxiao,Scott, Susannah,&Bao, Xinhe.(2013).Recent progress in methane dehydroaromatization: From laboratory curiosities to promising technology.journal of energy chemistry,22(1),1-20. |
| MLA | Ma, Shuqi,et al."Recent progress in methane dehydroaromatization: From laboratory curiosities to promising technology".journal of energy chemistry 22.1(2013):1-20. |
入库方式： OAI收割
来源：大连化学物理研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。