Spatial confinement effects of cage-type SAPO molecular sieves on product distribution and coke formation in methanol-to-olefin reaction
文献类型：期刊论文
| 作者 | Chen, Jingrun1,2; Li, Jinzhe1; Wei, Yingxu1; Yuan, Cuiyu1,2; Li, Bing1,2; Xu, Shutao1; Zhou, You1,2; Wang, Jinbang1; Zhang, Mozhi1,2; Liu, Zhongmin1 |
| 刊名 | catalysis communications
 |
| 出版日期 | 2014-02-10 |
| 卷号 | 46页码:36-40 |
| 关键词 | Methanol to olefin Silicoaluminophosphate Deactivation Adamantane hydrocarbons Spatial confinement |
| 产权排序 | 待补充 |
| 通讯作者 | 刘中民 |
| 合作状况 | 英 |
| 英文摘要 | three kinds of 8-membered ring silicoaluminophosphate (sapo) molecular sieves with different cage structures, sapo-34, sapo-18 and sapo-35, were employed in methanol-to-olefin (mto) reaction. the main products over sapo-34 and sapo-18 were propene and butenes, whereas ethene and propene especially ethene were predominantly generated over sapo-35. coke species formation greatly depended on reaction temperature and varied systematically with cage size. the differences in production distribution and generated coke species in the mto reaction suggest great spatial confinement effects imposed by cage structure of sapo catalysts. (c) 2013 elsevier b.v. all rights reserved. |
| WOS标题词 | science & technology ; physical sciences |
| 学科主题 | 物理化学 |
| 类目[WOS] | chemistry, physical |
| 研究领域[WOS] | chemistry |
| 关键词[WOS] | zeolite deactivation ; reaction centers ; conversion ; hydrocarbons ; catalysis ; selectivity ; hsapo-34 ; size ; mechanism |
| 收录类别 | SCI |
| 资助信息 | 1，1 |
| 原文出处 | 40 |
| 语种 | 英语 |
| WOS记录号 | WOS:000331504600008 |
| 公开日期 | 2014-09-11 |
| 源URL | [http://159.226.238.44/handle/321008/119729]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Natl Engn Lab Methanol Olefins, Dalian 116023, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Chen, Jingrun,Li, Jinzhe,Wei, Yingxu,et al. Spatial confinement effects of cage-type SAPO molecular sieves on product distribution and coke formation in methanol-to-olefin reaction[J]. catalysis communications,2014,46:36-40. |
| APA | Chen, Jingrun.,Li, Jinzhe.,Wei, Yingxu.,Yuan, Cuiyu.,Li, Bing.,...&Liu, Zhongmin.(2014).Spatial confinement effects of cage-type SAPO molecular sieves on product distribution and coke formation in methanol-to-olefin reaction.catalysis communications,46,36-40. |
| MLA | Chen, Jingrun,et al."Spatial confinement effects of cage-type SAPO molecular sieves on product distribution and coke formation in methanol-to-olefin reaction".catalysis communications 46(2014):36-40. |
入库方式： OAI收割
来源：大连化学物理研究所
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